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Monolayer transition metal dichalcogenides (TMDs) hold great promise for future information processing applications utilizing a combination of electron spin and valley pseudospin. This unique spin system has led to observation of the valley…

介观与纳米尺度物理 · 物理学 2019-05-30 T. P. Lyons , S. Dufferwiel , M. Brooks , F. Withers , T. Taniguchi , K. Watanabe , K. S. Novoselov , G. Burkard , A. I. Tartakovskii

Zeeman effect induced by the magnetic field introduces a splitting between the two valleys at K$^+$ and K$^-$ points of the Brillouin zone in monolayer semiconducting transition metal dichalcogenides. In consequence, the photoluminescence…

介观与纳米尺度物理 · 物理学 2020-12-30 Tomasz Smoleński , Tomasz Kazimierczuk , Mateusz Goryca , Karol Nogajewski , Marek Potemski , Piotr Kossacki

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

介观与纳米尺度物理 · 物理学 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Transition metal dichalcogenide (TMD) monolayers present a singular coupling in their spin and valley degrees of freedom. Moreover, by applying an external magnetic field it is possible to break the energy degeneracy between their K and…

Coulomb interaction between electrons lies at the heart of magnetism in solids. In contrast to conventional two-dimensional (2D) systems, electrons in monolayer transition metal dichalcogenides (TMDs) possess coupled spin and valley degrees…

介观与纳米尺度物理 · 物理学 2018-02-14 Zefang Wang , Kin Fai Mak , Jie Shan

Two-dimensional transition metal dichalcogenide (TMD) semiconductors provide a unique possibility to access the electronic valley degree of freedom using polarized light, opening the way to valley information transfer between distant…

Charge carriers in two-dimensional transition metal dichalcogenides (TMDs), such as WSe$_2$, have their spin and valley-pseudospin locked into an optically-addressable index that is proposed as a basis for future information processing. The…

介观与纳米尺度物理 · 物理学 2021-03-17 Weijie Li , Xin Lu , Jiatian Wu , Ajit Srivastava

Atomically thin transition metal dichalcogenides (TMDs) possess coupling of spin and valley degrees of freedom, making them promising for spin-valleytronics. ln monolayer TMDs, the emission helicity is locked to the valleys as a consequence…

材料科学 · 物理学 2018-02-07 Chongyun Jiang , Fucai Liu , Jorge Cuadra , Zumeng Huang , Ke Li , Ajit Srivastava , Zheng Liu , Wei-bo Gao

Exploiting the valley degree of freedom to store and manipulate information provides a novel paradigm for future electronics. A monolayer transition metal dichalcogenide (TMDC) with broken inversion symmetry possesses two degenerate yet…

Valley pseudospin in two-dimensional (2D) transition-metal dichalcogenides (TMDs) allows optical control of spin-valley polarization and intervalley quantum coherence. Defect states in TMDs give rise to new exciton features and…

Monolayers and multilayers of semiconducting transition metal dichalcogenides (TMDCs) offer an ideal platform to explore valley-selective physics with promising applications in valleytronics and information processing. Here we manipulate…

In this letter we study the valley degeneracy splitting of the transition-metal dichalcogenides monolayer by first-principles calculations. The local magnetic moments are introduced into the system when the transition-metal atoms are…

材料科学 · 物理学 2016-09-06 Xiaofang Chen , Liangshuai Zhong , Xiao Li , Jingshan Qi

The spectral signatures associated with different negatively charged exciton complexes (trions) in a WS$_2$ monolayer encapsulated in hBN, are analyzed from low temperature and polarization resolved reflectance contrast (RC) and…

Breaking space-time symmetries in two-dimensional crystals (2D) can dramatically influence their macroscopic electronic properties. Monolayer transition-metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal…

介观与纳米尺度物理 · 物理学 2015-09-04 Edbert J. Sie , James W. McIver , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

We report circularly-polarized optical reflection spectroscopy of monolayer WS$_2$ and MoS$_2$ at low temperatures (4~K) and in high magnetic fields to 65~T. Both the A and the B exciton transitions exhibit a clear and very similar Zeeman…

介观与纳米尺度物理 · 物理学 2016-02-11 Andreas V. Stier , Kathleen M. McCreary , Berend T. Jonker , Junichiro Kono , Scott A. Crooker

Monolayer valley semiconductors, such as tungsten diselenide (WSe$_2$), possess valley pseudospin degrees of freedom that are optically addressable but degenerate in energy. Lifting the energy degeneracy by breaking time-reversal symmetry…

Electrons in monolayer transition metal dichalcogenides (TMDs) possess both the valley and spin degree of freedom. These internal quantum degrees of freedom have provided an ideal laboratory for exploring both new physical phenomena and…

介观与纳米尺度物理 · 物理学 2017-02-21 Zefang Wang , Jie Shan , kin Fai Mak

The emerging field of valleytronics aims to exploit the valley pseudospin of electrons residing near Bloch band extrema as an information carrier. Recent experiments demonstrating optical generation and manipulation of exciton valley…

介观与纳米尺度物理 · 物理学 2017-05-24 Kai Hao , Lixiang Xu , Fengcheng Wu , Philipp Nagler , Kha Tran , Xin Ma , Christian Schüller , Tobias Korn , Allan H. MacDonald , Galan Moody , Xiaoqin Li

We have measured circularly polarized photoluminescence in monolayer MoSe2 under perpendicular magnetic fields up to 10 T. At low doping densities, the neutral and charged excitons shift linearly with field strength at a rate of $\mp$ 0.12…

Lifting the valley degeneracy of monolayer transition metal dichalcogenides (TMD) would allow versatile control of the valley degree of freedom. We report a giant valley exciton splitting of 18 meV/T for monolayer WS2, using the proximity…

介观与纳米尺度物理 · 物理学 2019-10-09 Tenzin Norden , Chuan Zhao , Peiyao Zhang , Renat Sabirianov , Athos Petrou , Hao Zeng
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