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Understanding light-matter interactions using localized surface plasmons (LSPs) is of fundamental interest in classical and quantum plasmonics and has a wide range of applications. In order to understand the spatial properties of LSPs,…

介观与纳米尺度物理 · 物理学 2016-03-22 Rong-Chun Ge , Stephen Hughes

We present a formalism and numerical results for the energy loss of a charged particle scattered at an arbitrary angle from epitaxially grown multilayer graphene (MLG). It is compared with that of free-standing graphene layers.…

材料科学 · 物理学 2011-05-20 O. Roslyak , G. Gumbs , D. H. Huang

In this work we perform electron energy-loss spectroscopy (EELS) of freestanding graphene with high energy and momentum resolution to disentangle the quasielastic scattering from the excitation gap of Dirac electrons close to the optical…

A periodic arrangement of 2D conducting planes is known to host a (bulk) plasmon dispersion that interpolates between the typical, gapped behavior of 3D metals and a gapless, acoustic regime as a function of the out-of-plane wavevector. The…

强关联电子 · 物理学 2022-11-09 Christian Boyd , Luke Yeo , Philip W. Phillips

A simple procedure is developed to simultaneously eliminate multiple scattering contributions from two reflection electron energy loss spectra (REELS) measured at different energies or for different experimental geometrical configurations.…

材料科学 · 物理学 2009-11-11 Wolfgang S. M. Werner

In previous work a different and powerful, analytical, technique was used to get data, such as the absolute atom concentration (AAC), specimen thickness etc., from public domain boron nitride EELS spectrum collected under a collection…

材料科学 · 物理学 2020-09-24 Noureddine Hadji

The inelastic scattering of electrons is one route to study the vibrational and electronic properties of materials. Such experiments, also called electron energy-loss spectroscopy, are particularly useful for the investigation of the…

材料科学 · 物理学 2014-06-24 Friedrich Roth , Andreas König , Jörg Fink , Bernd Büchner , Martin Knupfer

High-resolution electron energy loss spectroscopy (HREELS) is one of the most powerful methods to detect the dispersion of plasmons. However, we find that in the HREELS measurement, the scattering geometric configuration will seriously…

介观与纳米尺度物理 · 物理学 2022-03-18 Jiade Li , Zijian Lin , Guangyao Miao , Weiliang Zhong , Siwei Xue , Yi Li , Zhiyu Tao , Weihua Wang , Jiandong Guo , Xuetao Zhu

We theoretically investigate electron energy loss spectroscopy (EELS) of metallic nanoparticles in the optical frequency domain. Using a quasistatic approximation scheme together with a plasmon eigenmode expansion, we show that EELS can be…

介观与纳米尺度物理 · 物理学 2015-06-16 Anton Hörl , Andreas Trügler , Ulrich Hohenester

A fully relativistic description of the electron energy loss and the induced radiation emission in arbitrary arrays of non-overlapping metallic cylinders is presented in terms of the multiple scattering method on the basis of vector…

材料科学 · 物理学 2009-11-10 T. Ochiai , K. Ohtaka

{\it Ab initio} calculations of relativistic electron energy loss spectra (REELS) are carried out using a generalization of the real-space Green's function code FEFF8 which is applicable to general aperiodic materials. Our approach…

材料科学 · 物理学 2007-09-04 K. Jorissen , J. J. Rehr

The results of a joint experimental and theoretical investigation of the C60 collective excitations in the process of inelastic scattering of electrons are presented. The shape of the electron energy loss spectrum is observed to vary when…

Electron microscopy prevalently uses energy-dispersive x-ray spectroscopy (EDS) and electron energy loss spectroscopy (EELS) for elemental analysis. EDS and EELS energy resolutions are commonly between 30-100 eV or 0.01-1 eV, respectively.…

In the quest for dynamic multimodal probing of a material's structure and functionality, it is critical to be able to quantify the chemical state on the atomic and nanoscale using element specific electronic and structurally sensitive tools…

Electron energy loss spectroscopy (EELS) and Cathodoluminescence (CL) play a pivotal role in many of the cutting edge experiments in plasmonics. EELS and CL experiments are usually supported by numerical simulations, which, whilst accurate,…

介观与纳米尺度物理 · 物理学 2016-07-18 Matthias Kraft , Yu Luo , J. B. Pendry

Swift electrons passing near or through metallic structures have proven to be an excellent tool for studying plasmons and other types of confined optical modes involving collective charge oscillations in the materials hybridized with…

We study the origin of the structure in the spin-polarized electron energy loss spectroscopy (SPEELS) spectra of ferromagnetic crystals. Our study is based on a 3d tight-binding Fe model, with constant onsite Coulomb repulsion U between…

材料科学 · 物理学 2009-10-31 R. Saniz , S. P. Apell

Electron energy loss (EEL) spectra have been obtained on materials with the nominal compositions of Na0.33CoO2_yH2O (y = 0, 0.6 and 1.3). Spectral analyses revealed systematic changes in the low-loss energy region (< 10eV) and the core…

超导电性 · 物理学 2007-05-23 J. Q. Li , H. X. Yang , R. J. Xiao , Y. G. Shi , H. R Zhang

We present it ab initio calculations of the electronic energy loss of charged particles moving outside a magnesium surface, from a realistic description of the one-electron band structure and a full treatment of the dynamical electronic…

材料科学 · 物理学 2009-11-13 M. G. Vergniory , V. M. Silkin , I. G. Gurtubay , J. M. Pitarke

Fine structure analysis of core electron excitation spectra is a cornerstone characterization technique across the physical sciences. Spectra are most commonly measured with synchrotron radiation and X-ray spot sizes on the {\mu}m to mm…