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We demonstrate a simple technique for molecular ion spectroscopy. BaCl$^+$ molecular ions are trapped in a linear Paul trap in the presence of a room-temperature He buffer gas and photodissociated by driving an electronic transition from…

We demonstrate rotational cooling of the silicon monoxide cation via optical pumping by a spectrally filtered broadband laser. Compared with diatomic hydrides, SiO\+ is more challenging to cool because of its smaller rotational interval.…

A counterintuitive scheme to produce ultracold hydrogen via fragmentation of laser cooled diatomic hydrides is presented where the final atomic H temperature is inversely proportional to the mass of the molecular parent. In addition, the…

原子物理 · 物理学 2015-09-02 Ian Lane

Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…

The electronic structures of the manifold of potential energy surfaces generated in the lower energy range by the interaction of the MgH$^+$(X$^1\Sigma^+$) cationic molecule with Rb($^2$S), neutral atom are obtained over a broad range of…

化学物理 · 物理学 2009-11-13 Mario Tacconi , Franco A. Gianturco

Trapped Be+ ions are a leading platform for quantum information science [1], but reactions with background gas species, such as H2 and H2O, result in qubit loss. Our experiment reveals that the BeOH+ ion is the final trapped ion species…

化学物理 · 物理学 2021-11-17 Tiangang Yang , Bin Zhao , Gary K. Chen , Hua Guo , Wesley C. Campbell , Eric R. Hudson

We present high-resolution rovibronic spectroscopy of calcium monohydride molecular ions (CaH$^+$) co-trapped in a Coulomb crystal with calcium ions ($^{40}$Ca$^+$), focusing on rotational transitions in the $|X^1\Sigma^+, \nu" = 0>…

原子物理 · 物理学 2026-02-10 Swapnil Patel , Kenneth R. Brown

Intense positron beams can be prepared via electro production with the reaction $e^{-} + e^{-} \rightarrow e^{-}+e^{+}+e^{-}+e^{-}$ due to the availability of high current electron beams. Head on collisions inside of a magnetic field of a…

加速器物理 · 物理学 2016-07-14 Berthold Schoch

The extension of laser cooling and trapping techniques to polyatomic molecular ions would have advanced scientific applications such as search of physics outside of the Standard Model, ultracold chemistry etc. We apply the Fock space…

We demonstrate cryogenic buffer-gas cooling of gas-phase methyltrioxorhenium (MTO). This molecule is closely related to chiral organometallic molecules where the parity-violating energy differences between enantiomers may be measurable. The…

原子物理 · 物理学 2017-09-07 Sean Tokunaga , R. J. Hendricks , M. Tarbutt , B Darquié

The ability to cool single ions, atomic ensembles, and more recently macroscopic degrees of freedom down to the quantum groundstate has generated considerable progress and perspectives in Basic and Technological Science. These major…

介观与纳米尺度物理 · 物理学 2016-02-17 A. Niguès , A. Siria , P. Verlot

Cooling and detection schemes using laser cooling and methods of quantum logic can contribute to high precision CPT symmetry tests in the baryonic sector. This work introduces an experiment to sympathetically cool protons and antiprotons…

We report a detailed investigation on near-ground state cooling of one and two trapped atomic ions. We introduce a simple sideband cooling method for confined atoms and ions, using RF radiation applied to bare ionic states in a static…

原子物理 · 物理学 2018-04-04 Theeraphot Sriarunothai , Gouri Shankar Giri , Sabine Wölk , Christof Wunderlich

We demonstrate co-trapping and sideband cooling of a H$_2^+$ - $^9$Be$^+$ ion pair in a cryogenic Paul trap. We study the chemical lifetime of H$_2^+$ and its dependence on the apparatus temperature, achieving lifetimes of up to…

原子物理 · 物理学 2023-10-23 N. Schwegler , D. Holzapfel , M. Stadler , A. Mitjans , I. Sergachev , J. P. Home , D. Kienzler

A new, efficient method to produce ultracold negative muon ions is proposed. The muonium atom is made up of an antimuon and an electron and is given the chemical symbol Mu. A second electron with binding energy or electron affinity of 0.75…

仪器与探测器 · 物理学 2019-01-30 V. Dudnikov , A. Dudnikov

We have developed a source of cold LiH molecules for Stark deceleration and trapping experiments. Lithium metal is ablated from a solid target into a supersonically expanding carrier gas. The translational, rotational and vibrational…

原子物理 · 物理学 2009-11-13 S. K. Tokunaga , J. O. Stack , J. J. Hudson , B. E. Sauer , E. A. Hinds , M. R. Tarbutt

Plasma dynamics critically depends on density and temperature, thus well-controlled experimental realizations are essential benchmarks for theoretical models. The formation of an ultracold plasma can be triggered by ionizing a tunable…

We present a theoretical investigation of reactive and non-reactive collisions of Li and Rb atoms with C$_{2}^{-}$ molecular anions at low temperatures in the context of sympathetic cooling in hybrid trap experiments. Based on recently…

化学物理 · 物理学 2020-08-26 M. Kas , J. Liévin , N. Vaeck , J. Loreau

The low-temperature (up to about 100K) collisional (de)excitation cross sections are computed using the full coupled-channel (CC) quantum dynamics for both Li$_2$ and Li$_2^+$ molecular targets in collision with $^4$He. The interaction…

化学物理 · 物理学 2007-07-13 M. Wernli. E. Bodo , F. A. Gianturco

We study the motion of an undamped single-ion harmonic oscillator, resonantly driven with a pulsed radiation pressure force. We demonstrate that a barium ion, initially cooled to the Doppler limit, quickly phase locks to the drive and…

原子物理 · 物理学 2014-05-13 Y. -W. Lin , S. Williams , B. C. Odom