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First-principles calculations of the magnetic anisotropy energy for Mn- and Fe-atoms on CuN/Cu(001) surface are performed making use of the torque method. The easy magnetization direction is found to be different for Mn and Fe atoms in…

材料科学 · 物理学 2015-05-13 A. B. Shick , F. Máca , A. I. Lichtenstein

First-principles calculations were conducted to investigate the structural, electronic and magnetic properties of single Fe atoms and Fe dimers on Cu2N/Cu(100). Upon adsorption of an Fe atom onto Cu2N/Cu(100), robust Fe-N bonds form,…

材料科学 · 物理学 2024-09-13 Jiale Chen , Jun Hu

Both quantum and classical behavior of single atomic spins on surfaces is determined by the local anisotropy of adatoms and their coupling to the immediate electronic environment. Yet adatoms seldom reside on surfaces alone and it is…

材料科学 · 物理学 2015-11-04 P. Ruiz-Díaz , O. V. Stepanyuk , V. S. Stepanyuk

The magnetism of single atoms and molecules is governed by the atomic scale environment. In general, the reduced symmetry of the surrounding splits the $d$ states and aligns the magnetic moment along certain favorable directions. Here, we…

介观与纳米尺度物理 · 物理学 2015-11-30 Benjamin W. Heinrich , Lukas Braun , Jose I. Pascual , Katharina J. Franke

CeAu2Ge2 single crystals (tetragonal ThCr2Si2 structure) have been grown in Au-Ge flux (AGF) as well as in Sn flux (SF). X-ray powder-diffraction and EDX measurements indicate that in the latter case Sn atoms from the flux are incorporated…

强关联电子 · 物理学 2011-10-05 V. Fritsch , P. Pfundstein , P. Schweiss , E. Kampert , B. Pilawa , H. v. L öhneysen

This study demonstrates how the spin quantum dynamics of a single Fe atom adsorbed on Cu(001) can be controlled and manipulated by the vibrations of a nearby copper tip attached to a nano cantilever by virtue of the dynamic magnetic…

The magnetic anisotropy energy of Fe and Co monatomic nanowires both free-standing and at the step edge of a Pt surface is investigated within the framework of the density-functional theory and local-spin-density (LSDA) approximation.…

材料科学 · 物理学 2007-05-23 Matej Komelj Daniel Steiauf Manfred Faehnle

We have investigated the upper critical field anisotropy and magnetotransport properties of Fe1.14(1)Te0.91(2)S0.09(2) single crystals in stable magnetic fields up to 35 T. The results show that u0Hc2(T) along the c axis and in the ab-plane…

超导电性 · 物理学 2010-05-21 Hechang Lei , Rongwei Hu , E. S. Choi , J. B. Warren , C. Petrovic

Sizable single crystals of $BaFe_2As_2$ have been grown with self-flux method. The crystals are plate-like with c-axis perpendicular to the plane. The size can be as large as 3 x 5 x 0.2 $mm^3$. The resistivity anisotropy…

超导电性 · 物理学 2009-11-13 X. F. Wang , T. Wu , G. Wu , H. Chen , Y. L. Xie , J. J. Ying , Y. J. Yan , R. H. Liu , X. H. Chen

Interest in creating magnetic metamaterials has led to methods for growing superstructures of magnetic nanoparticles. Mesoscopic crystals of maghemite ($\gamma\text{-Fe}_2\text{O}_3$) nanoparticles can be arranged into highly ordered…

介观与纳米尺度物理 · 物理学 2021-01-05 B. Gross , S. Philipp , E. Josten , J. Leliaert , E. Wetterskog , L. Bergström , M. Poggio

The large saturation magnetization in conventional dense moment ferromagnets offers flexible means of manipulating the ordered state through demagnetizing shape anisotropy fields but these dipolar fields, in turn, limit the integrability of…

In intercalated transition metal dichalcogenide $Fe_xTaS_2$ (0.2 $\leq$ x $\leq$ 0.4) single crystals, large magnetic anisotropy is observed. Transport property measurements indicate that heavy Fe-doping leads to a large anisotropy of…

强关联电子 · 物理学 2017-05-10 G. Wu , B. L. Kang , Y. L. Li , T. Wu , N. Z. Wang , X. G. Luo , Z. Sun , L. J. Zou , X. H. Chen

We reversibly switch the polar environment of an individual magnetic atom with an electric field to control the energy barrier for reversal of magnetization. By applying an electric field in the gap between the tip and sample of a scanning…

介观与纳米尺度物理 · 物理学 2023-03-01 Jose Martinez-Castro , Cyrus F. Hirjibehedin , David Serrate

A detailed study of the electronic transport and magnetic properties of Fe$_{1-x}$Cu$_x$Cr$_2$S$_4$ ($x \leq 0.5$) on single crystals is presented. The resistivity is investigated for $2 \leq T \leq 300$ K in magnetic fields up to 14 Tesla…

We have measured quantum transport through an individual Fe$_4$ single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are…

Magnetocrystalline anisotropy is a fundamental property of magnetic materials that determines the dynamics of magnetic precession, the frequency of spin waves, the thermal stability of magnetic domains, and the efficiency of spintronic…

Magnetic adatoms on surfaces are exchange coupled to their environment, inducing fast relaxation of excited spin states and decoherence. These interactions can be suppressed by inserting decoupling layers between the magnetic adsorbate and…

介观与纳米尺度物理 · 物理学 2022-04-01 Sergey Trishin , Christian Lotze , Nils Bogdanoff , Felix von Oppen , Katharina J. Franke

The local magnetic anisotropy of a typical crystalline compound is usually attributed to the combined effect of crystal electric fields and spin-orbit coupling. We show that this simple local picture is transformed in heavy-fermion…

强关联电子 · 物理学 2025-08-05 Ewan Scott , Michal Kwasigroch

The electronic structure and magnetic properties of a single Fe adatom on a CuN surface have been studied using density functional theory in the local spin density approximation (LSDA), the LSDA+U approach and the local density…

强关联电子 · 物理学 2016-04-20 S. K. Panda , I. Di Marco , O. Grånäs , O. Eriksson , J. Fransson

We present a theoretical approach to calculate the molecular magnetic anisotropy parameters, $D_M$ and $E_M$ for single molecule magnets in any eigenstate of the exchange Hamiltonian, treating the anisotropy Hamiltonian as a perturbation.…

强关联电子 · 物理学 2009-11-13 Rajamani Raghunathan , S. Ramasesha , Diptiman Sen
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