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The temperature evolution of icosahedral medium-range order formed by interpenetrating icosahedra in CuZr metallic glass-forming liquids was investigated via molecular dynamics simulations. Scaling analysis based on percolation theory was…

无序系统与神经网络 · 物理学 2016-10-20 Z. W. Wu , F. X. Li , C. W. Huo , M. Z. Li , W. H. Wang , K. X. Liu

The atomic structure of the supercooled liquid has often been discussed as a key source of glass formation in metals. The presence of icosahedrally-coordinated clusters and their tendency to form networks have been identified as one…

材料科学 · 物理学 2013-10-30 Logan Ward , Dan Miracle , Wolfgang Windl , Oleg Senkov , Katharine Flores

Using molecular dynamics simulations with embedded atom model potential, we study structural evolution of ${\rm Cu_{64.5}Zr_{35.5}}$ alloy during the cooling in a wide range of cooling rates $\gamma\in(1.5\cdot 10^{9},10^{13})$ K/s.…

无序系统与神经网络 · 物理学 2016-08-03 R. E. Ryltsev , B. A. Klumov , N. M. Chtchelkatchev

Recent experimental results suggest that metallic liquids universally exhibit a high-temperature dynamical crossover, which is correlated with the glass transition temperature ($T_{g}$). We demonstrate, using molecular dynamics results for…

无序系统与神经网络 · 物理学 2016-03-24 Ryan Soklaski , Vy Tran , Zohar Nussinov , K. F. Kelton , Li Yang

Metallic glasses have so far attracted considerable attention for their applications as bulk materials. However, new physics and applications often emerge by dimensional reduction from three dimension (3D) to two dimension (2D). Here, we…

材料科学 · 物理学 2017-09-07 Yuan-Chao Hu , Hajime Tanaka , Wei-Hua Wang

The glass transition remains one of the great unsolved mysteries of contemporary condensed matter physics. When crystallization is bypassed by rapid cooling, a supercooled liquid, retaining amorphous particle arrangment, results. The…

材料科学 · 物理学 2016-10-12 Nicholas B. Weingartner , Zohar Nussinov

As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

软凝聚态物质 · 物理学 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

Development of reliable interatomic potentials is crucial for theoretical studies of relationship between chemical composition, structure and observable properties in glass-forming metallic alloys. Due to ambiguity of potential…

化学物理 · 物理学 2020-01-08 R. E. Ryltsev , N. M. Chtchelkatchev

Finding a suitably growing length scale that increases in tandem with the immense viscous slowdown of supercooled liquids is an open problem associated with the glass transition. Here, we define and demonstrate the existence of one such…

材料科学 · 物理学 2016-06-08 Nicholas B. Weingartner , Ryan Soklaski , K. F. Kelton , Zohar Nussinov

Zr-Cu-Al alloys belong to a commercially important family of CuZr-based alloys that form bulk metallic glasses on microalloying of Al. However, the identification of compositions with good glass-forming ability and desirable properties from…

材料科学 · 物理学 2025-09-18 Kamal G. Soni , Jayraj P. Anadani , Mitanshu B. Vahiya , Kirit N. Lad

Special role in computer simulations of supercooled liquid and glasses is played by few general models representing certain classes of real glass-forming systems. Recently, it was shown that one of the most widely used model glassformers --…

材料科学 · 物理学 2018-11-14 R. E. Ryltsev , B. A. Klumov , N. M. Chtchelkatchev , K. Yu. Shunyaev

The discovery of quasicrystals 30 years ago challenged our understanding of order at the atomic scale. While quasicrystals possess long-range orientational order they lack translation periodicity. Structurally complex, yet crystalline…

材料科学 · 物理学 2014-10-14 Wolfgang Hornfeck , Raphael Kobold , Matthias Kolbe , Dieter Herlach

Dynamic and structural heterogeneities play an important role in glass transition phenomena and in the formation of amorphous structures. Since structure and dynamics are mutually related, it is expected that there exists some relation…

To experimentally clarify the changes in structural and dynamic heterogeneities in a metallic glass (MG), Gd65Co35, by rejuvenation with a temperature cycling (cryogenic rejuvenation), high-energy x-ray diffraction (HEXRD), anomalous x-ray…

Solid-state amorphization of crystalline copper nanolayers embedded in a Cu64Zr36 metallic glass is studied by molecular dynamics simulations for different orientations of the crystalline layer. We show that solid-state amorphization is…

材料科学 · 物理学 2015-05-07 Tobias Brink , Daniel Şopu , Karsten Albe

Metallic glasses are promising materials with unique mechanical and thermal properties, but their atomic-scale dynamics remain challenging to understand. In this work, we develop a unified approach to investigate the glass transition and…

材料科学 · 物理学 2025-02-07 Anh D. Phan , Do T. Nga , Ngo T. Que , Hailong Peng , Thongchanh Norhourmour , Le M. Tu

We performed all-atom molecular dynamics simulations for bulk cyclohexane and analysed the short- and medium-range structures in supercooled and glassy states by using the Voronoi tessellation technique. From the analyses of both the…

无序系统与神经网络 · 物理学 2020-01-15 Tomoko Mizuguchi , Soichi Tatsumi , Susumu Fujiwara

The viscosity of glass-forming liquids increases by many orders of magnitude if their temperature is lowered by a mere factor of 2-3 [1,2]. Recent studies suggest that this widespread phenomenon is accompanied by spatially heterogeneous…

无序系统与神经网络 · 物理学 2015-05-28 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

Binary Cu-Zr system is a representative bulk glassformer demonstrating high glass forming ability due to pronounced icosahedral local ordering. From the first glance, Ni-Zr system is the most natural object to expect the same behavior…

无序系统与神经网络 · 物理学 2018-10-09 B. A. Klumov , R. E. Ryltsev , N. M. Chtchelkatchev

This paper presents computer simulations of Cu$_x$Zr$_{100-x}$ $(x=36,50,64)$ in the liquid and glass phases. The simulations are based on the effective-medium theory (EMT) potentials. We find good invariance of both structure and dynamics…

材料科学 · 物理学 2021-04-21 Laura Friedeheim , Nicholas P. Bailey , Jeppe C. Dyre
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