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We observe interfacial ferromagnetism in superlattices of the paramagnetic metal LaNiO3 and the antiferromagnetic insulator CaMnO3. LaNiO3 exhibits a thickness dependent metal-insulator transition and we find the emergence of ferromagnetism…

Perovskite solar cells (PSCs) based on methylammonium lead iodide (MAPbI3) exhibit remarkable photovoltaic performance, where interface engineering with hole transport layers (HTLs) is crucial for optimizing charge transfer and device…

材料科学 · 物理学 2025-12-30 Somayyeh Alidoust , V. Ongun Özçelik

Superconductivity in infinite layer nickelates Nd1-xSrxNiO2 has so far been achieved only in thin films raising questions on the role of substrates and interfaces. Given the challenges associated with their synthesis it is imperative to…

Strong resonant enhancements of the charge-order and spin-order superstructure-diffraction intensities in La1.8Sr0.2NiO4 are observed when x-ray energies in the vicinity of the Ni L2,3 absorption edges are used. The pronounced photon-energy…

Since the discovery of two-dimensional electron gas (2DEG) at the oxide interface of LaAlO3/SrTiO3, improving carrier mobility has become an important issue for device applications. In this paper, by using an alternate polar perovskite…

强关联电子 · 物理学 2016-03-29 Z. Huang , K. Han , S. W. Zeng , M. Motapothula , W. M. Lü , C. J. Li , W. X. Zhou , J. M. D. Coey , T. Venkatesan , Ariando

The present work theoretically studies the possibility to hinder the formation of a "dead" layer at the interfaces in manganite superlattices. We showed that this goal can be reached by using alkaline-earth simple oxides as alternating…

Epitaxial interfaces and superlattices comprised of polar and non-polar perovskite oxides have generated considerable interest because they possess a range of desirable properties for functional devices. In this work, emergent polarization…

La0.7Ce0.3MnO3 is a relatively new addition in the family of colossal magnetoresistive manganites where the cerium ion is believed to be in the Ce4+ state. In this paper we report an extensive study the magnetotransport properties of laser…

材料科学 · 物理学 2007-05-23 P. Raychaudhuri , S. Mukherjee , A. K. Nigam , J. John , U. D. Vaisnav , R. Pinto

The nature of superconductivity and its interplay with strong spin-orbit coupling at the KTaO3(111) interfaces remains a subject of debate. To address this problem, we grew epitaxial LaMnO3/KTaO3(111) heterostructures. We show that…

Superlattices of correlated oxides have been used to explore interfacial effects and to achieve additional control over the physical properties of individual constituents. In this work, we present a first-principles perspective of the…

强关联电子 · 物理学 2024-02-02 V. A. M. Lima , M. C. O. Aguiar , N. C. Plumb , M. Radovic , W. H. Brito

We investigate the effect of oxygen vacancies and hydrogen dopants at the surface and inside slabs of LaAlO3, SrTiO3, and LaAlO3/SrTiO3 heterostructures on the electronic properties by means of electronic structure calculations as based on…

强关联电子 · 物理学 2019-05-03 I. I. Piyanzina , V. Eyert , Yu. V. Lysogorskiy , D. A. Tayurskii , T. Kopp

The modulation of charge density and spin order in (LaMnO$_3$)$_{2n}$/(SrMnO$_3$)$_n$ ($n$=1-4) superlattices is studied via Monte Carlo simulations of the double-exchange model. G-type antiferromagnetic barriers in the SrMnO$_{3}$ regions…

强关联电子 · 物理学 2008-11-24 Shuai Dong , Rong Yu , Seiji Yunoki , Gonzalo Alvarez , J. -M. Liu , Elbio Dagotto

We report strong localization of 2D electron gas in LaAlO3 / SrTiO3 epitaxial thin-film heterostructures grown on (LaAlO3)0.3-(Sr2AlTaO3)0.7 substrates by using pulsed laser deposition with in-situ reflection high-energy electron…

强关联电子 · 物理学 2015-05-30 T. Hernandez , C. W. Bark , D. A. Felker , C. B. Eom , M. S. Rzchowski

The gating effect achieved by an ionic liquid and its electric double layer allows for charge transfer which can be an order of magnitude larger than with conventional dielectrics. However, the large charged ions also causes inevitable…

介观与纳米尺度物理 · 物理学 2019-04-26 Chunhai Yin , Kumar Prateek , Wouter Gelling , Jan Aarts

Nickel-based superconductors provide a long-awaited experimental platform to explore possible cuprate-like superconductivity. Despite similar crystal structure and $d$ electron filling, these systems exhibit several differences. Nickelates…

Interface engineering in complex oxide heterostructures has developed into a flourishing field as various intriguing physical phenomena can be demonstrated which are otherwise absent in their constituent bulk compounds. Here we present…

材料科学 · 物理学 2023-04-03 Snehal Mandal , Sandip Halder , Biswarup Satpati , Kalpataru Pradhan , I. Das

At interfaces between complex oxides it is possible to generate electronic systems with unusual electronic properties, which are not present in the isolated oxides. One important example is the appearance of superconductivity at the…

超导电性 · 物理学 2016-07-13 D. Di Castro , C. Cantoni , F. Ridolfi , C. Aruta , A. Tebano , N. Yang , G. Balestrino

We report transport measurements of infinite-layer cuprate Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ films with controlled electron (by trivalent europium) and hole (by interstitial apical oxygen) carriers grown on SrTiO$_3$(001) with molecular beam…

超导电性 · 物理学 2024-12-12 Hang Yan , Ze-Xian Deng , Xue-Qing Yu , Yan-Ling Xiong , Qun Zhu , Ding Zhang , Can-Li Song , Xu-Cun Ma , Qi-Kun Xue

Driven quantum materials with on demand properties controlled by external stimuli are critical for emergent quantum technology. In optically tunable superconducting heterostructures, the lattice responses at the buried interface may hold…

To study digital Mott insulator LaTiO3 and band insulator SrTiO3 interfaces, we apply correlated band theory (LDA+U) to (n,m) multilayers, 1<n,m<9. If the on-site repulsion on Ti is large enough to model the magnetic insulating behavior of…

材料科学 · 物理学 2007-05-23 Rossitza Pentcheva , Warren E. Pickett