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In view of the important role helix-sheet transitions play in protein aggregation, we introduce a simple model to study secondary structural transitions of helix-coil-sheet systems using a Potts model starting with an effective Hamiltonian.…

生物物理 · 物理学 2011-11-09 John S. Schreck , Jian-Min Yuan

In this paper we summarize some results of our theoretical investigations of helix-coil transition both in single-strand (polypeptides) and two-strand (polynucleotides) macromolecules. The Hamiltonian does not contain any parameter designed…

We analyze the problem of the helix-coil transition in explicit solvents analytically by using spin-based models incorporating two different mechanisms of solvent action: explicit solvent action through the formation of solvent-polymer…

An exact analytical solution of generalized three-state double-chain Potts model with multi-spin interactions which are invariant under cyclic shift of all spin values is obtained. The partition function in a finite cyclically closed strip…

统计力学 · 物理学 2025-02-04 Pavel Khrapov , Grigory Skvortsov

We present the exact solution of a microscopic statistical mechanical model for the transformation of a long polypeptide between an unstructured coil conformation and an $\alpha$-helix conformation. The polypeptide is assumed to be adsorbed…

软凝聚态物质 · 物理学 2015-01-30 Ganga P. Sharma , Yana K. Reshetnyak , Oleg A. Andreev , Michael Karbach , Gerhard Müller

We analyze a model statistical description of the polypeptide chain helix-coil transition, where we take into account the specificity of its primary sequence, as quantified by the phase space volume ratio of the number of all accessible…

生物大分子 · 定量生物学 2015-07-15 Artem Badasyan , Yevgeni Sh. Mamasakhlisov , Rudolf Podgornik , V. Adrian Parsegian

The authors study the short-time dynamics of helix-forming polypeptide chains using an all-atom representation of the molecules and an implicit solvation model to approximate the interaction with the surrounding solvent. The results confirm…

其他定量生物学 · 定量生物学 2016-08-14 Everaldo Arashiro , J. R. Drugowich de Felício , Ulrich H. E. Hansmann

The similarity in the thermodynamic properties of two completely different theoretical models for the helix-coil transition is examined critically. The first model is an all-atomic representation for a poly-alanine chain, while the second…

化学物理 · 物理学 2009-11-06 Josh P. Kemp , Ulrich H. E. Hansmann , Zheng Y. Chen

A microscopic spin model is proposed for the phenomenological Zimm-Bragg model for the helix-coil transition in biopolymers. This model is shown to provide the same thermophysical properties of the original Zimm-Bragg model and it allows a…

软凝聚态物质 · 物理学 2012-08-22 A. V. Badasyan , A. Giacometti , Y. Sh. Mamasakhlisov , V. F. Morozov , A. S. Benight

A self-consistent-field theory (SCFT) in the grand canonical ensemble formulation is used to study transitions in a helix-coil multiblock copolymer globule. The helices are modeled as stiff rods. In addition to the established coil-globule…

软凝聚态物质 · 物理学 2007-05-23 Christian Nowak , Vakhtang G. Rostiashvili , Thomas A. Vilgis

In the present paper we present results of calculations obtained with the use of the theoretical method described in our preceding paper [1] and perform detail analysis of alpha helix-random coil transition in alanine polypeptides of…

Most helix-coil transition theories can be characterized by a set of three parameters: energetic, describing the (free) energy cost of forming a helical state in one repeating unit; entropic, accounting for the decrease of entropy due to…

In this paper we suggest a theoretical method based on the statistical mechanics for treating the alpha-helix-random coil transition in alanine polypeptides. We consider this process as a first-order phase transition and develop a theory…

Thermoresponsive polymers hold both fundamental and technological importance, but the essential physics driving their intriguing behavior is not wholly understood. We introduce a lattice framework that incorporates elements of Flory-Huggins…

软凝聚态物质 · 物理学 2024-03-04 Satyen Dhamankar , Michael A. Webb

The interactions between a group of components are commonly studied in several areas of science (social science, biology, material science, complex dynamical systems, among others) using the methods of thermodynamics and statistical…

统计力学 · 物理学 2021-07-28 Constanza Farías , Sergio Davis

We present a simple yet generic model for the behavior of a system of many surface-attached flexible polymers with rigid side chains. Beyond its potential application in describing the dynamics of the extracellular matrix of mammalian…

统计力学 · 物理学 2008-04-01 Marcel Hellmann , Youjin Deng , Matthias Weiss , Dieter W. Heermann

We consider the Potts model on a two-dimensional periodic rectangular lattice with general coupling constants $J_{ij}>0$, where $i,j\in\{1,2,3\}$ are the possible spin values (or colors). The resulting energy landscape is thus significantly…

概率论 · 数学 2024-05-09 Gianmarco Bet , Anna Gallo , Seonwoo Kim

We perform Monte Carlo simulations to study the elastic properties of the helix-coil worm-like chain model of alpha-helical polypeptides. In this model the secondary structure enters as a scalar (Ising like) variable that controls the local…

软凝聚态物质 · 物理学 2007-05-23 Buddhapriya Chakrabarti , Alex J. Levine

The coil-globule transition of an energy polydisperse chain, a model heteropolymer system where the number of monomer species is as large as the total number of monomers, is studied by means of computer simulations. In this study, we…

软凝聚态物质 · 物理学 2022-07-21 Thoudam Vilip Singh , Lenin S. Shagolsem

Many-body spin systems represent a paradigmatic platform for the realization of emergent states of matter in a strongly interacting regime. Spin models are commonly studied in one-dimensional periodic chains, whose lattice constant is on…

介观与纳米尺度物理 · 物理学 2019-10-08 J. L. Lado , Oded Zilberberg
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