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A range of chemical reactions occurring on the surfaces of metal nanoparticles exhibit enhanced rates under plasmonic excitation. Recent analyses based on Arrhenius law fitting have argued in favor of a purely photothermal mechanism of…

化学物理 · 物理学 2020-06-11 Prashant K. Jain

The behavior of a particle in a solvent has been framed using stochastic dynamics since the early theory of Kramers. A particle in a chemical reaction reacts slower in a diluted solvent because of the lack of energy transfer via collisions.…

We consider a molecular junction immersed in a solvent where the electron transfer is dominated by Marcus-type steps. However, the successive nature of the charge transfer through the junction does not imply that the solvent reach thermal…

统计力学 · 物理学 2022-03-23 Henning Kirchberg , Abraham Nitzan

One considers the motion of a test particle in an homogeneous fluid in equilibrium at temperature $T$, undergoing dissipative collisions with the fluid particles. It is shown that the corresponding linear Boltzmann equation still posseses a…

统计力学 · 物理学 2007-05-23 Ph. A. Martin , J. Piasecki

Recently, we have shown that thermal effects play a crucial role in speeding up the rate of bond-dissociation reactions. This was done by applying a simple temperature-shifted Arrhenius Law to the experimental data, corroborated with…

化学物理 · 物理学 2023-03-31 Ieng Wai Un , Yonatan Sivan

It is shown that thermally excited plasmon-polariton modes can strongly mediate, enhance and \emph{tune} the near-field radiation transfer between two closely separated graphene sheets. The dependence of near-field heat exchange on doping…

介观与纳米尺度物理 · 物理学 2013-05-30 Ognjen Ilic , Marinko Jablan , John D. Joannopoulos , Ivan Celanovic , Hrvoje Buljan , Marin Soljačić

Ionic conductivity in solid electrolytes is commonly expected to exhibit Arrhenius dependence on temperature, determined by a well-defined activation energy. Consequently, a standard approach involves calculating this energy using…

介观与纳米尺度物理 · 物理学 2024-04-11 Keian Noori , Ben A. Olsen , Aleksandr Rodin

The emergent photoactive materials through photochemistry make it possible to directly convert photon energy to mechanical work. There is much recent work in developing appropriate materials and a promising new system is semi-crystalline…

软凝聚态物质 · 物理学 2021-03-24 Ruobing Bai , Eric Ocegueda , Kaushik Bhattacharya

[Abridged] Photoionization, whether by starlight or other sources, has difficulty in accounting for the observed spectra of the optical filaments that often surround central galaxies in large clusters. Our first paper examined whether…

We use large scale molecular dynamics simulations of the isomerizations of azobenzene molecules diluted inside a simple molecular material, to investigate the effect of a modification of the cis isomer shape on the induced diffusion…

软凝聚态物质 · 物理学 2017-12-05 Victor Teboul

Employing a previously derived formulation, and extending the treatment from purely transverse modes to wave vectors having a longitudinal component, we discuss the prospects for the occurrence of Weibel-type color-current filamentation in…

核理论 · 物理学 2008-11-26 Jorgen Randrup , Stanislaw Mrowczynski

Interpretations of the very rich second solar spectrum of the MgH molecule face serious problems owing to the complete lack of any information about rates of collisions between the MgH and hydrogen atoms. This work seeks to begin the…

太阳与恒星天体物理 · 物理学 2021-07-27 Saleh Qutub , Yulia Kalugina , Moncef Derouich

This work inspects the thermally activated transfer of solute particles across the interface between two interstitial solid solution phases that equilibrate internally by fast diffusion on conserved arrays of sites. When each phase is…

材料科学 · 物理学 2026-01-30 Jörg Weissmüller

We study C70 fullerene matter waves in a Talbot-Lau interferometer as a function of their temperature. While the ideal fringe visibility is observed at moderate molecular temperatures, we find a gradual degradation of the interference…

量子物理 · 物理学 2007-05-23 Klaus Hornberger , Lucia Hackermueller , Markus Arndt

We propose a theoretical approach to quantitatively determine the photothermally driven enhancement of molecular mobility of graphene-indomethacin mixtures under infrared laser irradiation. Graphene plasmons absorb incident electromagnetic…

介观与纳米尺度物理 · 物理学 2022-04-13 Anh D. Phan , Nguyen K. Ngan , Do T. Nga , Nam B. Le , Chu Viet Ha

For a detailed understanding of chemical processes in nature and industry, we need accurate models of chemical reactions in complex environments. While Eyring transition state theory is commonly used for modeling chemical reactions, it is…

化学物理 · 物理学 2023-12-19 Simon Ghysbrecht , Bettina G. Keller

The broadening of the hydrogen lines during flares is thought to result from increased charge (electron, proton) density in the flare chromosphere. However, disagreements between theory and modeling prescriptions have precluded an accurate…

Graphene supports strongly confined transverse-magnetic sheet plasmons whose spectral characteristics depend on the energetic distribution of Dirac particles. The question arises whether plasmons can become amplified when graphene is pumped…

介观与纳米尺度物理 · 物理学 2015-02-05 A. Freddie Page , Fouad Ballout , Ortwin Hess , Joachim M. Hamm

Plasmas in an accretion flow are heated by MHD turbulence generated through the magneto-rotational instability. The viscous stress driving the accretion is intimately connected to the microscopic processes of turbulence dissipation. We show…

天体物理学 · 物理学 2007-07-04 Siming Liu , Christopher L. Fryer , Hui Li

Context. In dffuse interstellar clouds the excitation temperature derived from the lowest levels of H$^+_3$ is systematically lower than that derived from H2. The differences may be attributed to the lack of state-specific formation and…

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