相关论文: Kapellasite: a kagome quantum spin liquid
The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…
We report the study of high quality samples of the frustrated S = 1/2 kagome antiferromagnet vesignieite, Cu3Ba(VO5H)2. Neutron powder diffraction measurements evidence the high quality of the kagome lattice and show no sign of a transition…
We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…
A clear thermal Hall signal ($\kappa_{xy}$) was observed in the spin liquid phase of the $S=1/2$ kagom\'e antiferromagnet Ca kapellasite (CaCu$_3$(OH)$_6$Cl$_2\cdot 0.6$H$_2$O). We found that $\kappa_{xy}$ is well reproduced, both…
We analyze recent heat capacity measurements in herbertsmithite $\rm ZnCu_3(OH)_6Cl_2$ single crystal samples subjected to strong magnetic fields. We show that the temperature dependence of specific heat $C_{mag}$ formed by quantum spin…
Recently, a novel material with bilayer kagome lattice Ca$_{10}$Cr$_7$O$_{28}$ was proposed to be a gapless quantum spin liquid, due to the lack of long-range magnetic order and the observation of broad diffuse excitations. Here, we present…
Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel…
Deuteronium jarosite, (D_3O)Fe_3(SO_4)_2(OD)_6, contains a kagome lattice of Heisenberg spins, S=5/2, with a coverage of 97+-1%. DC and AC susceptibility measurements show strong in-plane antiferromagnetic exchange (\theta_CW=-1500+-300K)…
Strongly correlated Fermi systems are among the most intriguing and fundamental systems in physics, whose realization in some compounds is still to be discovered. We show that herbertsmithite ZnCu_3(OH)_6Cl_2 can be viewed as a strongly…
We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…
We present a study of a simple model antiferromagnet consisting of a sum of nearest neighbor SO($N$) singlet projectors on the Kagome lattice. Our model shares some features with the popular $S=1/2$ Kagome antiferromagnet but is…
The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…
We argue that a relatively simple model containing only SU(2)-invariant chiral three-spin interactions on a Kagome lattice of S=1/2 spins can give rise to both a gapped and a gapless quantum spin liquid. Our arguments are rooted in a…
Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…
Quantum spin liquids are exotic quantum phases of matter that do not order even at zero temperature. While there are several toy models and simple Hamiltonians that could host a quantum spin liquid as their ground state, it is very rare to…
Herbertsmithite, ZnCu$_3$(OH)$_6$Cl$_2$, is a two dimensional kagom\'{e} lattice realization of a spin liquid, with evidence for fractionalized excitations and a gapped ground state. Such a quantum spin liquid has been proposed to underlie…
We present a thorough experimental investigation on single crystals of the rare-earth based frustrated quantum antiferromagnet Pr$_3$BWO$_9$, a purported spin-liquid candidate on the breathing kagome lattice. This material possesses a…
On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…
We present the results of first-principle calculations using the Vienna Ab-initio Simulation Package (VASP) for a new class of organometallics labeled TM3C6O6 (TM =Sc, Ti, V, Cr, Fe, Co, Ni and Cu) in the form of planar, two-dimensional,…
Dynamical magnetic correlations in the geometrically frustrated Nd$\_3$Ga$\_5$SiO$\_{14}$ compound were probed by inelastic neutron scattering on a single crystal. A scattering signal with a ring shape distribution in reciprocal space and…