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The efficiency of a coherent VUV source at 125 nm, based on 2-photon resonant four-wave mixing in mercury vapor, has been enhanced by up to 2 orders of magnitude. This enhancement was obtained by locally heating a liquid Hg surface with a…

We propose to generate continuous-wave vacuum ultraviolet (VUV) laser light at 148.4 nm using four-wave mixing in cadmium vapor for precision spectroscopy of the Th-229 isomer transition. Due to the large transition matrix elements of…

Tunable coherent light sources operating in the vacuum ultraviolet (VUV) region in 100-200-nm (6-12 eV) wavelength range have important spectroscopic applications in many research fields, including time-resolved angle-resolved photoemission…

A novel approach is used to enhance by nearly two orders of magnitude the conversion efficiency of a 125 nm-coherent source, based on four-wave mixing in room-temperature mercury vapor. Saturation issues are observed and discussed.

光学 · 物理学 2007-05-23 Sebastien Chenais , Sebastien Forget , Marie-Claude Castex

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of…

Cooling antihydrogen atoms is important for future experiments both to test the fundamental CPT symmetry by high-resolution laser spectroscopy and also to measure the gravitational acceleration of antimatter. Laser-cooling of antihydrogen…

VUV radiation around 159 nm is obtained toward direct excitation of a single trapped $^{115}$In$^{+}$ ion. An efficient fluoride-based VUV output-coupler is employed for intracavity high-harmonic generation of a Ti:S oscillator. Using this…

原子物理 · 物理学 2014-08-25 Kentaro Wakui , Kazuhiro Hayasaka , Tetsuya Ido

Vacuum ultraviolet (VUV) light at 118 nm has been shown to be a powerful tool to ionize molecules for various gas-phase chemical studies. A convenient table top source of 118 nm light can be produced by frequency tripling 355 nm light from…

We use two continuous-wave (CW) laser beams of 780 nm and 515 nm to optically drive $^{85}$Rb atoms in a heated vapor cell to a low-lying Rydberg state 10D$_{5/2}$. We observe a collimated ultraviolet (UV) beam at 311 nm, corresponding to…

原子物理 · 物理学 2019-05-31 Mark Lam , Sambit B. Pal , Thibault Vogt , Christian Gross , Martin Kiffner , Wenhui Li

Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies…

光学 · 物理学 2018-11-15 Manoj K. Mridha , Pooria Hosseini , David Novoa , Philip St. J. Russell

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large…

Continuous coherent radiation in the vacuum-ultraviolet at 122 nm (Lyman-alpha) can be generated using sum-frequency mixing of three fundamental laser beams in mercury vapour. One of the fundamental beams is at 254 nm wavelength, which is…

光学 · 物理学 2015-06-11 Daniel Kolbe , Martin Scheid , Jochen Walz

We report here a detailed study of the four-wave mixing process in the extreme ultraviolet (XUV) region around 30 nm by using two collinear incommensurate frequency laser pulses. The experimental results reveal evidence of the coherent…

光学 · 物理学 2019-04-03 Khoa Anh Tran , Khuong Ba Dinh , Peter Hannaford , Lap Van Dao

Frequency-modulation (FM) spectroscopy has been extended to the vacuum-ultraviolet (VUV) range of the electromagnetic spectrum. Coherent VUV laser radiation is produced by resonance-enhanced sum-frequency mixing…

The recent breakthroughs in laser-driving 229Th nuclear transition have created an urgent demand for coherent vacuum-ultraviolet (VUV) sources delivering high spectral brightness at the critical 148.38 nm isomer energy. However, generating…

Four-wave mixing can be used to generate coherent output beams, with frequencies difficult to acquire in commercial lasers. Here a single narrow ECDL locked to the two photon 5s-5d transition in rubidium is combined with a tapered amplifier…

原子物理 · 物理学 2016-04-13 E. Brekke , L. Alderson

Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…

光学 · 物理学 2020-06-11 Rinat Tyumenev , Philip St. J. Russell , David Novoa

We report on the generation of a three-octave-wide supercontinuum extending from the vacuum ultraviolet (VUV) to the near-infrared, spanning at least 113 to 1000 nm (i.e., 11 to 1.2 eV), in He-filled hollow-core kagome-style photonic…

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagom\'e-style photonic crystal fiber. By pumping with ultrashort, few $\mu$J, pulses…

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