A continuous-wave vacuum ultraviolet laser for the nuclear clock
Abstract
The exceptionally low-energy isomeric transition in Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large ensembles of Th nuclei in transparent crystals and the development of pulsed vacuum-ultraviolet (VUV) lasers, have enabled initial laser spectroscopy of this transition. However, the lack of an intense, narrow-linewidth VUV laser has precluded coherent nuclear manipulation. Here we introduce and demonstrate the first continuous-wave laser at 148.4 nm, generated via four-wave mixing (FWM) in cadmium vapor. The source delivers 100 nW of power with a linewidth well below 100 Hz and supports broad wavelength tunability. This represents a five-orders-of-magnitude improvement in linewidth over all previous single-frequency lasers below 190 nm, marking a major advance in laser technology. We develop a spatially resolved homodyne technique to place a stringent upper bound on the phase noise induced by the FWM process and demonstrate sub-hertz linewidth capability. These results eliminate the final technical hurdle to a Th-based nuclear clock, opening new directions in quantum metrology, nuclear quantum optics and precision tests of the Standard Model. More broadly, they establish a widely tunable, ultranarrow-linewidth laser platform for applications across quantum information science, condensed matter physics, and high-resolution VUV spectroscopy.
Cite
@article{arxiv.2507.19449,
title = {A continuous-wave vacuum ultraviolet laser for the nuclear clock},
author = {Qi Xiao and Gleb Penyazkov and Xiangliang Li and Beichen Huang and Wenhao Bu and Juanlang Shi and Haoyu Shi and Tangyin Liao and Gaowei Yan and Haochen Tian and Yixuan Li and Jiatong Li and Bingkun Lu and Li You and Yige Lin and Yuxiang Mo and Shiqian Ding},
journal= {arXiv preprint arXiv:2507.19449},
year = {2025}
}
Comments
Submitted on June 26, 2025