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As the simplest element in nature, unraveling the phase diagram of hydrogen is a primary task for condensed matter physics. As conjectured many decades ago, in the low-temperature and high-pressure part of the phase diagram, solid hydrogen…

超导电性 · 物理学 2023-11-14 Mehmet Dogan , Sehoon Oh , Marvin L. Cohen

Hydrogen-rich compounds have been extensively studied both theoretically and experimentally in the quest for novel high-temperature superconductors. Reports on sulfur-hydride attaining metallicity under pressure and exhibiting…

The dependence of the superconducting transition temperature Tc of CaC6 has been determined as a function of hydrostatic pressure in both helium-loaded gas and diamond-anvil cells to 0.6 and 32 GPa, respectively. Following an initial…

超导电性 · 物理学 2015-05-13 M. Debessai , J. J. Hamlin , J. S. Schilling , Y. Meng , D. Rosenmann , D. G. Hinks , H. Claus

Solid CS$_{2}$ is superficially similar to CO$_{2}$, with the same $Cmca$ molecular crystal structure at low pressures, which has suggested similar phases also at high pressures. We carried out an extensive first principles evolutionary…

材料科学 · 物理学 2015-06-23 S. Shahab Naghavi , Yanier Crespo , Roman Martonak , Erio Tosatti

It has been suggested that hydrogen may metallise at lower pressures if it is ``precompressed''. Here we introduce a search strategy for predicting high-pressure structures and apply it to silane using first-principles electronic structure…

材料科学 · 物理学 2009-11-11 Chris J. Pickard , R. J. Needs

Recent experimental developments in hydrogen-rich materials in high pressures have put this class of materials above others in the race toward room temperature superconductivity. As it is the basis of all the materials in this class, the…

超导电性 · 物理学 2022-02-03 Mehmet Dogan , Sehoon Oh , Marvin L. Cohen

Due to its low atomic mass hydrogen is the most promising element to search for high-temperature phononic superconductors. However, metallic phases of hydrogen are only expected at extreme pressures (400 GPa or higher). The measurement of a…

超导电性 · 物理学 2016-03-23 José A. Flores-Livas , Antonio Sanna , E. K. U. Gross

The dependence of the superconducting transition temperature T_{c} on nearly hydrostatic pressure has been determined to 67 GPa in an ac susceptibility measurement for a Li sample embedded in helium pressure medium. With increasing…

超导电性 · 物理学 2009-11-10 Shanti Deemyad , James S. Schilling

The transition metal dichalcogenide PdTe$_2$ has attractive features based on its classification as a type-II Dirac semimetal and the occurrence of type-I superconductivity, providing a platform for discussion of a topological…

Hydrogen-based compounds have attracted significant attention in recent years due to the discovery of conventional superconductivity with high critical temperature under high pressure, rekindling hopes for searching room temperature…

超导电性 · 物理学 2024-11-20 Yao Ma , Mingqi Li , Wenjia Shi , Vei Wang , Pugeng Hou , Mi Pang

Superconductivity in the recently proposed ground-state structures of atomic metallic hydrogen is investigated over the pressure range 500 GPa to 3.5 TPa. Near molecular dissociation, the electron--phonon coupling $\lambda$ and renormalized…

超导电性 · 物理学 2015-05-28 Jeffrey M. McMahon , David M. Ceperley

The compression of SH$_2$ and its subsequent decomposition to SH$_3$, presumably in a cubic Im$\overline{3}$m structure, has lead to the discovery of conventional superconductivity with the highest measured and confirmed $T_c$ to date, 203…

材料科学 · 物理学 2019-02-20 Maximilian Amsler

Following the idea that hydrogen-rich compounds might be high-T$_c$ superconductors at high pressures, and the very recent breakthrough in predicting and synthesizing hydrogen sulfide with record-high T$_c$ = 203 K, ab initio evolutionary…

超导电性 · 物理学 2017-04-19 M. M. Davari Esfahani , A. R. Oganov , H. Niu , J. Zhang

Ab initio molecular dynamic method within the framework of density functional theory is applied to analyze the structural and electronic properties of crystalline molecular hydrogen at temperature 100\,K. Pressure, pair correlation function…

材料科学 · 物理学 2022-01-12 I. Saitov

The search for high-temperature superconductors in hydrides under high pressure has always been a research hotspot. Hydrogen-based superconductors offer an avenue to achieve the long-sought goal of superconductivity at room temperature. We…

超导电性 · 物理学 2023-05-22 Ming Xu , Defang Duan , Wendi Zhao , Decheng An , Hao Song , Tian Cui

As a new type of topological materials, ZrTe5 shows many exotic properties under extreme conditions. Utilizing resistance and ac magnetic susceptibility measurements under high pressure, while the resistance anomaly near 128 K is completely…

We predicted a new ternary hydride Li$_2$SiH$_6$ at high pressures. A systematic structure search in Li$_2$SiH$_6$ compound reveals novel stable phases with intriguing electronic and phonon properties. It is found that Li$_2$SiH$_6$ is…

材料科学 · 物理学 2022-09-13 Sixuan Wu , Bin Li , Zhi Chen , Yu Hou , Yan Bai , Xiaofeng Hao , Yeqian Yang , Shengli Liu , Jie Cheng , Zhixiang Shi

Recently, the superconducting transition temperature Tc = 287 K has been experimentally obtained in the material composed of carbon, sulfur, and hydrogen under the high pressure of 267 GPa. The material structure is unknown yet, where the…

超导电性 · 物理学 2022-08-08 Zheng-Wei Liao , Zhen Zhang , Jing-Yang You , Bo Gu , Gang Su

The uniquely characteristic macrostructures of binary hydrogen-clathrate compounds $M$H$_\textrm{n}$ formed at high pressure, a cage of hydrogens surrounding a central-atom host, is theoretically predicted in various studies to include…

超导电性 · 物理学 2020-06-22 Dale R. Harshman , Anthony T. Fiory

The discovery of the high temperature superconducting state in compounds of hydrogen, carbon and sulfur with the critical temperature (Tc) of 288 K at high pressure is an important milestone towards room-temperature superconductors. Here,…

超导电性 · 物理学 2021-07-23 Mingyang Du , Zihan Zhang , Tian Cui , Defang Duan1
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