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Resonant Inelastic X-ray Scattering (RIXS), which probes the occupied and unoccupied electronic subspaces in an interrelated fashion, is one of the most detailed, complex and information-rich experimental techniques employed in the…

材料科学 · 物理学 2022-09-16 Subhayan Roychoudhury , David Prendergast

We discuss the calculation of resonant inelastic x-ray scattering (RIXS) with Xclaim, a multi-plaform code for the calculation of core-hole spectroscopy based on a ligand-field multiplet model. RIXS can be calcuated with a ligand-field…

强关联电子 · 物理学 2015-08-05 Javier Fernandez-Rodriguez , Brian Toby , Michel van Veenendaal

We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p…

强关联电子 · 物理学 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Jeroen van den Brink

We report a Cu $K$-edge resonant inelastic x-ray scattering (RIXS) study of spin excitations in the $S$=1/2 antiferromagnetic chain system Sr$_2$CuO$_3$. The spectral weight observed below the charge-transfer gap appears in two-spinon…

强关联电子 · 物理学 2025-10-31 Kenji Ishii , Kenji Tsutsui , Takayuki Kawamata , Yoji Koike

We use Ru $L_3$-edge resonant inelastic x-ray scattering (RIXS) to study the full range of excitations in Ca$_3$Ru$_2$O$_7$ from meV-scale magnetic dynamics through to the eV-scale interband transitions. This bilayer $4d$-electron…

强关联电子 · 物理学 2021-02-10 J. Bertinshaw , M. Krautloher , H. Suzuki , H. Takahashi , A. Ivanov , B. J. Kim , H. Gretarsson , B. Keimer

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender x-ray range and have recently become available for…

材料科学 · 物理学 2014-01-08 K. O. Kvashnina , S. M. Butorin

We have investigated the excitation spectra of $j_{eff}$=$\frac{1}{2}$ Mott insulator Na$_2$IrO$_3$. Taking into account a relativistic multiplet structure of Ir ions, we have calculated the optical conductivity $\sigma(\omega)$ and…

强关联电子 · 物理学 2014-02-25 Beom Hyun Kim , G. Khaliullin , B. I. Min

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

材料科学 · 物理学 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We study the resonant inelastic x-ray scattering (RIXS) features of vector chiral ordered kagome antiferromagnets. Utilizing a group theoretical formalism that respects lattice site symmetry, we calculated the $L$ -edge magnon contribution…

强关联电子 · 物理学 2024-01-05 Zijian Xiong , Trinanjan Datta , Dao-Xin Yao

The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we…

超导电性 · 物理学 2021-07-28 Da-Wei Yao , Tao Li

We present a detailed analysis of the incident-photon-energy and polarization dependences of the resonant inelastic x-ray scattering (RIXS) spectra at the Cu $K$ edge in La$_{2}$CuO$_{4}$. Our analysis is based on the formula developed by…

强关联电子 · 物理学 2009-11-13 Manabu Takahashi , Junichi Igarashi , Takuji Nomura

We show that Resonant Inelastic X-ray scattering (RIXS) is sensitive to three-magnon excitations in cuprates. Even if it requires three electrons to simultaneously flip their spin, the RIXS tri-magnon scattering amplitude is not small. At…

强关联电子 · 物理学 2010-02-22 Luuk J. P. Ament , Jeroen van den Brink

High-resolution resonant inelastic x-ray scattering (RIXS) measurements ($\Delta$E = 46 meV) have been performed on Cd$_2$Os$_2$O$_7$ through the metal-to-insulator transition (MIT). A magnetic excitation at 125 meV evolves continuously…

Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic…

化学物理 · 物理学 2024-03-19 Antonia Freibert , David Mendive-Tapia , Oriol Vendrell , Nils Huse

The low energy excitations in Na2IrO3 have been investigated using resonant inelastic x-ray scattering (RIXS). A magnetic excitation branch can be resolved, whose dispersion reaches a maximum energy of about 35 meV at the \Gamma-point. The…

Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitations of these materials hold great promise for understanding and…

强关联电子 · 物理学 2019-04-02 Y. Cao , D. G. Mazzone , D. Meyers , J. P. Hill , X. Liu , S. Wall , M. P. M. Dean

We present a comprehensive study of the spin excitations - as measured by the dynamical spin structure factor $S(q,\omega)$ - of the so-called block-magnetic state of low-dimensional orbital-selective Mott insulators. We realize this state…

强关联电子 · 物理学 2020-09-17 J. Herbrych , G. Alvarez , A. Moreo , E. Dagotto

We compute the $K$ and $L_{3}$ -edge resonant inelastic x-ray scattering (RIXS) spectrum of the columnar and the staggered quantum dimer states accessible to the square lattice Heisenberg magnet. Utilizing a bond operator representation…

强关联电子 · 物理学 2020-02-03 Meiyu He , Trinanjan Datta , Dao-Xin Yao

We examine the effect of core-hole lifetime on the spectral weight of resonant inelastic x-ray scattering (RIXS) in hole-doped cuprates. We calculate the spectral weight by using exact diagonalization technique for a 4x4 doped Hubbard…

强关联电子 · 物理学 2018-08-01 Takami Tohyama , Kenji Tsutsui