相关论文: Broadband sum frequency generation via chirped qua…
We theoretically propose a method for optical isolation based on adiabatic nonlinear sum frequency generation in a chirped quasi-phase-matching crystal with strong absorption at the generated sum frequency wave. The method does not suffer…
We introduce the concept of a quantum pulse gate (QPG), a method for accessing the intrinsic broadband spectral mode structure of ultrafast quantum states of light. This mode structure can now be harnessed for applications in quantum…
Vibrational sum frequency generation (SFG) is a nonlinear spectroscopic technique widely used to study the molecular structure and dynamics of surface systems. However, the spatial resolution achieved by far-field observations is…
We measure the time-energy correlation of broadband, spontaneously generated four wave mixing (FWM), and demonstrate novel time-frequency coupling effects; specifically, we observe a power-dependent splitting of the correlation in both…
Phase-matching of the third-harmonic generation process can be used to extend the emission of radiation from Kerr microresonators into new spectral regions far from the pump wavelength. Here, we present a theoretical mean-field model for…
Dense wavelength division multiplexing (DWDM) is one of the most successful methods for enhancing data transmission rates in both classical and quantum communication networks. Although signal multiplexing and demultiplexing are equally…
We present a 100 kHz broadband vibrational sum-frequency generation (VSFG) spectrometer operating in the 5.5-10.5 $\mu$m (950-1750 cm$^{-1}$) wavelength range. The mid-infrared beam of the system is obtained from a collinear, type-I…
Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes…
Appropriately designed dual-core fibers using coupling-length phase matching (CLPM) allow for phase-matched frequency downconversion over wide frequency intervals using the third-order optical nonlinearity of glass. By tuning the distance…
Quantum frequency conversion (QFC) between the visible and telecom is a key functionality to connect quantum memories over long distances in fiber-based quantum networks. Current QFC methods for linking such widely-separated frequencies,…
Difference-frequency generation (DFG) is a powerful technique for generating widely tunable infrared radiation. However, conventional phase-matching schemes may require tuning multiple parameters-such as the wavelengths, crystal…
We propose a computational framework to extract non-linear response functions from real-time simulations in the presence of more than one external field. We apply this approach to the calculation of sum frequency generation (SFG) and…
Sum-frequency generation (SFG) is a powerful second-order nonlinear spectroscopic technique that provides detailed insights into molecular structures and absolute orientations at surfaces and interfaces. However, conventional SFG based on…
We propose a method for generation of a single-cycle squeezed light by parametric down-conversion in a chirped quasi-phase-matched nonlinear crystal. We find an exact quantum solution for this process valid for an arbitrary parametric gain,…
High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…
Future quantum information networks operated on telecom channels require qubit transfer between different wavelengths while preserving quantum coherence and entanglement. Qubit transfer is a nonlinear optical process, but currently the…
Supercontinuum generation in integrated photonic waveguides is a versatile source of broadband light, and the generated spectrum is largely determined by the phase-matching conditions. Here we show that quasi-phase-matching via periodic…
Triple sum-frequency (TSF) spectroscopy is a recently-developed methodology that enables collection of multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. This work reports the…
We address theoretically the question of classical stochastic fields mimicking quantum states of light in the context of nonlinear spectroscopy and nonlinear optics, in particular two-photon absorption (TPA) and sum-frequency generation…
This study proposes and demonstrates a versatile method for near and mid-infrared optical frequency comb generation using multi-seeded femtosecond optical parametric generation. The method allows one to divide the repetition rate by an…