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A method for the calculation of the conductance of nanoscale electrical junctions is extended to ab-initio electronic structure methods and applied to realistic models of metallic wires and break-junctions of sodium and gold. The method is…

材料科学 · 物理学 2014-05-13 Matthieu J. Verstraete , P. Bokes , R. W. Godby

We report on the fabrication, transport measurements, and density functional theory (DFT) calculations of atomic size contacts made out of gadolinium (Gd). Gd is known to have local moments mainly associated with $f$ electrons. These…

介观与纳米尺度物理 · 物理学 2017-02-15 B. Olivera , C. Salgado , J. L. Lado , A. Karimi , V. Henkel , E. Scheer , J. Fernández-Rossier , J. J. Palacios , C. Untiedt

Based on density functional theory (DFT), we have developed algorithms and a program code to investigate the electron transport characteristics for a variety of nanometer scaled devices in the presence of an external bias voltage. We…

介观与纳米尺度物理 · 物理学 2008-05-14 Woo Youn Kim , Kwang S. Kim

A first-principles approach based on Density Functional Theory and Non-Equilibrium Green's functions is used to study the molecular transport system consisting of benzenedithiolate connected with monoatomic gold and platinum electrodes.…

介观与纳米尺度物理 · 物理学 2017-10-10 M. Rumetshofer , G. Dorn , L. Boeri , E. Arrigoni , W. von der Linden

Electrical conductance through various nanocontacts between gold electrodes is studied by using the density functional theory, scalar-relativistic pseudopotentials, generalized gradient approximation for the exchange-correlation energy and…

材料科学 · 物理学 2009-11-13 O. Lopez-Acevedo , D. Koudela , H. Häkkinen

The recent fabrication of graphene nanoribbon (GNR) field-effect transistors poses a challenge for first-principles modeling of carbon nanoelectronics due to many thousand atoms present in the device. The state of the art quantum transport…

介观与纳米尺度物理 · 物理学 2010-04-28 Denis A. Areshkin , Branislav K. Nikolic

We describe a first-principles method for calculating electronic structure, vibrational modes and frequencies, electron-phonon couplings, and inelastic electron transport properties of an atomic-scale device bridging two metallic contacts…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Magnus Paulsson , Mads Brandbyge , Antti-Pekka Jauho

We investigate charge transport in C$_{60}$-based single-molecule junctions with graphene electrodes employing a combination of density functional theory (DFT) electronic structure calculations and Landauer transport theory. In particular,…

介观与纳米尺度物理 · 物理学 2017-01-12 Susanne Leitherer , Pedro B. Coto , Konrad Ullmann , Heiko B. Weber , Michael Thoss

Correlation effects within the GW approximation have been incorporated into the Keldysh non-equilibrium transport formalism. We show that GW describes the Kondo effect and the zero-temperature transport properties of the Anderson model…

材料科学 · 物理学 2015-06-25 Kristian S. Thygesen , Angel Rubio

Electronic transport properties for single-molecule junctions have been widely measured by several techniques, including mechanically controllable break junctions, electromigration break junctions or by means of scanning tunneling…

介观与纳米尺度物理 · 物理学 2020-07-22 Ferdinand Evers , Richard Korytár , Sumit Tewari , Jan M. van Ruitenbeek

We present a generalized approach for computing electron conductance and I-V characteristics in multiterminal junctions from first-principles. Within the framework of Keldysh theory, electron transmission is evaluated employing an O(N)…

材料科学 · 物理学 2015-05-13 Kamal K. Saha , Wenchang Lu , J. Bernholc , Vincent Meunier

The evolution of electron conductance in the presence of inelastic effects is studied as an atomic gold contact is formed evolving from a low-conductance regime (tunneling) to a high-conductance regime (contact). In order to characterize…

介观与纳米尺度物理 · 物理学 2007-06-25 Thomas Frederiksen , Nicolas Lorente , Magnus Paulsson , Mads Brandbyge

Electron-phonon interactions are of great importance to a variety of physical phenomena, and their accurate description is an important goal for first-principles calculations. Isolated examples of materials and molecular systems have…

The non-equilibrium Green's function method combined with density functional theory (NEGF-DFT) provides a rigorous framework for simulating nanoscale electronic transport, but its computational cost scales steeply with system size. Recent…

介观与纳米尺度物理 · 物理学 2025-10-21 Zili Tang , Xiaoxin Xie , Guanwen Yao , Ligong Zhang , Xiaoyan Liu , Xing Zhang , Liu Fei

We overview nonequilibrium Green function combined with density functional theory (NEGF-DFT) modeling of independent electron and phonon transport in nanojunctions with applications focused on a new class of thermoelectric devices where a…

介观与纳米尺度物理 · 物理学 2012-04-19 Branislav K. Nikolic , Kamal K. Saha , Troels Markussen , Kristian S. Thygesen

With the objective to understand microscopic principles governing thermal energy flow in nanojunctions, we study phononic heat transport through metal-molecule-metal junctions using classical molecular dynamics (MD) simulations. Considering…

介观与纳米尺度物理 · 物理学 2022-11-23 Jonathan J. Wang , Jie Gong , Alan J. H. McGaughey , Dvira Segal

Nonequilibrium Greens function techniques (NEGF) combined with density functional theory (DFT) calculations have become a standard tool for the description of electron transport through single molecule nanojunctions in the coherent…

介观与纳米尺度物理 · 物理学 2015-11-05 Victor Geskin , Robert Stadler , Jérôme Cornil

An integrated piecewise thermal equilibrium approach based on the first-principles calculation method has been developed to calculate bias dependent electronic structures and current- and differential conductance-voltage characteristics of…

其他凝聚态物理 · 物理学 2009-11-13 M. -H. Tsai , T. -H. Lu , Y. -H. Tang

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

介观与纳米尺度物理 · 物理学 2012-12-18 Muhammad Imran

We present a first-principles numerical implementation of Landauer formalism for electrical transport in nanostructures characterized down to the atomic level. The novelty and interest of our method lies essentially on two facts. First of…

材料科学 · 物理学 2009-11-07 J. J. Palacios , A. J. Perez-Jimenez , E. Louis , E. SanFabian , J. A. Verges