相关论文: Energy conversion in Purple Bacteria Photosynthesi…
The plant bioelectric potential is believed to be a suitable real-time and noninvasive method that can be used to evaluate plant activities, such as the photosynthetic reaction. The amplitude of the bioelectric potential response when…
For efficient photovoltaic conversion, it is important to understand how quantum entropy-related quantities evolve during the photovoltaic process. In this study, using a double quantum dot (DQD) photocell model, we explored the dynamic…
Using the reduced density matrix formalism the exciton scattering in light-harvesting systems of purple bacteria is calculated. The static disorder (fluctuations of the site energies) as well as the dynamic disorder (dissipation) is taken…
Photosystem II (PSII) can achieve near-unity quantum efficiency of light harvesting in ideal conditions and can dissipate excess light energy as heat to prevent formation of reactive oxygen species under light stress. Understanding how this…
We study the natural excitation of molecular systems, applicable to, for example, photosynthetic light-harvesting complexes, by natural incoherent light. In contrast with the conventional classical models, we show that the light need not…
Many living organisms can exploit quantum mechanical effects to gain distinct biological advantages. In plants, photosynthesis uses quantum coherence to achieve near 100% efficiency in energy transfer. With advances in experimental…
In natural and artificial light-harvesting complexes (LHC) the resonant energy transfer (RET) between chromophores enables an efficient and directional transport of solar energy between collection and reaction centers. The detailed…
The early steps of photosynthesis involve the photo-excitation of reaction centres (RCs) and light-harvesting (LH) units. Here, we show that the --historically overlooked-- excitonic delocalisation across RC and LH pigments results in a…
Photosynthesis is vital for the survival of entire ecosystems on Earth. While light is fundamental to this process, excessive exposure can be detrimental to plant cells. Chloroplasts, the photosynthetic organelles, actively move in response…
Large-scale simulations of light-matter interaction in natural photosynthetic antenna complexes of the Chlorobium Tepidum green sulfur bacteria (GSB) containing more than one hundred thousand chlorophyll molecules, comparable with natural…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
Randomly moving active particles can be herded into directed motion by asymmetric geometric structures. Although such a rectification process has been extensively studied due to its fundamental, biological, and technological relevance, a…
Photosynthesis is central to Earth's biosphere and a prime candidate for sustaining complex life on habitable exoplanets, yet a thermodynamically consistent treatment of the work potential of stellar radiation at planetary surfaces is still…
We perform a quantitative assessment for the potential for photosynthesis in hydrothermal vents in the deep ocean. The photosynthetically active radiation in this case is from geothermal origin: the infrared thermal radiation emitted by hot…
Photochromic molecular structures constitute a unique platform for constructing molecular switches, sensors and memory devices. One of their most promising applications is as light-switchable electron acceptor or donor units. Here, we…
This review article provides a specific example of recombinant cell and protocell technology, moving from what is presently known to suggesting how novel application of existing methodologies could be utilized to design a complex synthetic…
The energy sciences attempt to meet the increasing world-wide need for energy, as well as sustainability goals, by cleaner sources of energy, by new alternative sources of energy, and by more efficient uses of available energy. These goals…
Photosynthesis powers life on our planet. The basic photosynthetic architecture comprises antenna complexes to harvest solar energy and reaction centers to convert the energy into a stable charge separated state. In oxygenic photosynthesis,…
Photoluminescence (PL) is a fundamental light-matter interaction in which absorbed photons are re-emitted, playing a key role in science and engineering. It is commonly modeled by introducing a non-zero chemical potential into Planck's law…
With this paper we propose a model to simulate the functional aspects of light adaptation in retinal photoreceptors. Our model, however, does not link specific stages to the detailed molecular processes which are thought to mediate…