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In recent years, a number of dynamical density functional theories (DDFTs) have been developed for describing the dynamics of the one-body density of both colloidal and atomic fluids. In the colloidal case, the particles are assumed to have…

软凝聚态物质 · 物理学 2009-08-10 A. J. Archer

By computer simulations of systems of ellipsoids, we study the influence of the isotropic/nematic phase transition on the direct correlation functions (DCF) in anisotropic fluids. The DCF is determined from the pair distribution function by…

材料科学 · 物理学 2009-11-10 Nguyen H. Phuong , Friederike Schmid

We present a real-space formulation and higher-order finite-difference implementation of periodic Orbital-free Density Functional Theory (OF-DFT). Specifically, utilizing a local reformulation of the electrostatic and kernel terms, we…

计算物理 · 物理学 2015-12-23 Swarnava Ghosh , Phanish Suryanarayana

The thermal conductivity of organic liquids is a vital parameter influencing various industrial and environmental applications, including energy conversion, electronics cooling, and chemical processing. However, atomistic simulation of…

The exact 1+3 covariant dynamical fluid equations for a multi-component plasma, together with Maxwell's equations are presented in such a way as to make them suitable for a gauge-invariant analysis of linear density and velocity…

广义相对论与量子宇宙学 · 物理学 2009-11-07 Mattias Marklund , Peter K. S. Dunsby , Gerold Betschart , Martin Servin , Christos Tsagas

Orbital-free molecular dynamics simulations are used to benchmark two popular models for hot dense plasmas: the one component plasma (OCP) and the Yukawa model. A unified concept emerges where an effective OCP (eOCP) is constructed from the…

等离子体物理 · 物理学 2020-11-19 Jean Clérouin , Philippe Arnault , Christopher Ticknor , Joel D. Kress , Lee A. Collins

Modeling nuclear quantum effects is required for accurate molecular dynamics (MD) simulations of molecules. The community has paid special attention to water and other biomolecules that show hydrogen bonding. Standard methods of modeling…

化学物理 · 物理学 2020-07-06 Vikram Sundar , David Gelbwaser-Klimovsky , Alan Aspuru-Guzik

We present a parametrization of the pair correlation function and the static structure factor of the Coulomb one component plasma (OCP) from the weakly coupled regime to the strongly coupled regime. Recent experiments strongly suggest that…

等离子体物理 · 物理学 2016-11-03 Nicolas Desbiens , Philippe Arnault , Jean Clérouin

Results for the dynamic structure factor of a one-component plasma are presented for the situations of strong coupling and weak degeneracy and strong degeneracy and weak coupling. Possibilities to obtain rigorous results when both, coupling…

统计力学 · 物理学 2009-11-07 M. Bonitz , V. Golubnichiy , N. H. Kwong , D. Semkat , D. Kremp , V. S. Filinov , M. Schlanges

Three dimensional implementations of liquid state theories offer an efficient alternative to computer simulations for the atomic-level description of aqueous solutions in complex environments. In this context, we present a (classical)…

化学物理 · 物理学 2013-02-13 Guillaume Jeanmairet , Maximilien Levesque , Rodolphe Vuilleumier , Daniel Borgis

The frequency-dependent response of a one-dimensional fermion system is investigated using Current Density Functional Theory (CDFT) within the local approximation (LDA). DFT-LDA, and in particular CDFT-LDA, reproduces very well the…

强关联电子 · 物理学 2010-04-01 Michael Dzierzawa , Ulrich Eckern , Stefan Schenk , Peter Schwab

Dynamical density functional theory (DDFT) is a powerful variational framework to study the nonequilibrium properties of colloids by only considering a time-dependent one-body number density. Despite the large number of recent successes,…

软凝聚态物质 · 物理学 2021-01-13 René Wittmann , Hartmut Löwen , Joseph M. Brader

The dynamical structure factor (DSF) represents a measure of dynamical density-density correlations in a quantum many-body system. Due to the complexity of many-body correlations and quantum fluctuations in a system of an infinitely large…

量子气体 · 物理学 2023-08-15 Run-Tian Li , Song Cheng , Yang-Yang Chen , Xi-Wen Guan

A fundamental problem in applying machine learning techniques for chemical problems is to find suitable representations for molecular and crystal structures. While the structure representations based on atom connectivities are prevalent for…

机器学习 · 统计学 2016-08-23 Dipti Jasrasaria , Edward O. Pyzer-Knapp , Dmitrij Rappoport , Alan Aspuru-Guzik

The velocity autocorrelation function (VACF) encapsulates extensive information about a fluid's molecular-structural and hydrodynamic properties. We address the following fundamental question: How well can a purely hydrodynamic description…

软凝聚态物质 · 物理学 2024-04-22 Sean L Seyler , Charles E Seyler

We present a new code, RCF("Radiative-Collisional code based on FAC"), which is used to simulate steady-state plasmas under non local thermodynamic equilibrium condition, especially photoinization dominated plasmas. RCF takes almost all of…

原子物理 · 物理学 2015-06-24 Bo Han , Feilu Wang , David Salzmann , Gang Zhao

The manuscript reports the observation of time dependent localized and non-propagating structures in the coupled laser plasma system through 1-D fluid and PIC simulations. It is reported that such structures form spontaneously as a result…

等离子体物理 · 物理学 2018-01-17 Deepa Verma , Ratan Kumar Bera , Atul Kumar , Bhavesh Patel , Amita Das

The aim of this work is the investigation of the statistical properties of local electric fields in an ion-electron two component plasmas for coupled conditions. The stochastic fields at a charged or at a neutral point in plasmas involve…

Classical molecular dynamics simulations of hydrogen plasmas have been performed with emphasis on the analysis of equilibration process. Theoretical basis of simulation model as well as numerically relevant aspects -- such as the proper…

等离子体物理 · 物理学 2024-02-07 M. A. Gigosos , D. Gonzalez-Herrero , R. Florido , A. Calisti , S. Ferri , B. Talin

Structural and thermodynamic properties of ionic fluids are related to those of a simpler ``mimic'' system with short ranged intermolecular interactions in a spatially varying effective field by use of Local Molecular Field (LMF) theory,…

统计力学 · 物理学 2007-05-23 Yng-gwei Chen , Charanbir Kaur , John D. Weeks