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Phonon interactions are inevitable in cavity quantum electrodynamical systems based on solid-state emitters or fluorescent molecules, where vibrations of the lattice or chemical bonds couple to the electronic degrees of freedom. Due to the…

量子物理 · 物理学 2021-06-16 Matias Bundgaard-Nielsen , Jesper Mørk , Emil Vosmar Denning

In this work we develop a theory of correlated many-electron dynamics dressed by the presence of a finite-temperature harmonic bath. The theory is based on the ab-initio Hamiltonian, and thus well-defined apart from any phenomenological…

量子物理 · 物理学 2015-06-05 John A. Parkhill , Thomas Markovich , David G. Tempel , Alan Aspuru-Guzik

Exciton polaritons in two-dimensional semiconductors inside microcavities are powerful platforms to explore hybrid light-matter quantum systems. Here, we study a macroscopic coherent population of the lowest energy state of…

介观与纳米尺度物理 · 物理学 2021-10-26 Aleksi Julku , Miguel. A. Bastarrachea-Magnani , Arturo Camacho-Guardian , Georg M. Bruun

When an optical emitter is strongly coupled to a vibrational bath the polaron transformation is often used to permit an accurate second-order Redfield master equation. However, the optical transition rates in the polaron frame are not…

量子物理 · 物理学 2022-01-19 Dominic M Rouse , Erik M Gauger , Brendon W Lovett

In the context of Frenkel exciton dynamics in aggregated molecules the polaron transformation technique facilitates a treatment where diagonal elements attributed to electronic excited-state populations are decoupled from fluctuations…

化学物理 · 物理学 2021-08-30 Joachim Seibt , Oliver Kühn

We study coherent transport through a double quantum dot. Its two electronic leads induce electronic matter and energy transport and a phonon reservoir contributes further energy exchanges. By treating the system-lead couplings…

统计力学 · 物理学 2015-04-07 Thilo Krause , Tobias Brandes , Massimiliano Esposito , Gernot Schaller

Understanding the dynamics of open quantum systems in strong coupling and non-Markovian regimes remains a formidable theoretical challenge. One popular and well-established method of approximation in these circumstances is provided by the…

量子物理 · 物理学 2024-07-16 Jake Iles-Smith , Owen Diba , Ahsan Nazir

Cascaded emission from the biexciton state of a quantum dot results in polarization entangled photon pairs. However, modelling this system becomes challenging when photon emission is cavity-mediated due to the large Hilbert space and…

量子物理 · 物理学 2026-03-24 Katy Snow , Mauro Paternostro

We have developed a non-Markovian theory of the polariton luminescence taking the molecular vibrations into account. The calculations were made in the polariton basis. We have shown that the frequency shift and the polariton spectral lines…

介观与纳米尺度物理 · 物理学 2022-04-19 B. D. Fainberg , V. Al. Osipov

Understanding interactions between excitons and correlated electronic states presents a fundamental challenge in quantum many-body physics. Here, we introduce a purely electronic model for the formation of exciton-polarons in moir\'e…

强关联电子 · 物理学 2026-05-12 Fabian Pichler , Mohammad Hafezi , Michael Knap

Non-Markovian and non-equilibrium phonon effects are believed to be key ingredients in the energy transfer in photosynthetic complexes, especially in complexes which exhibit a regime of intermediate exciton-phonon coupling. In this work, we…

量子物理 · 物理学 2011-07-08 Patrick Rebentrost , Alán Aspuru-Guzik

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

量子物理 · 物理学 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

Organic semiconductors have the remarkable property that their optical excitation not only generates charge-neutral electron-hole pairs (excitons) but also charge-separated polaron pairs with high yield. The microscopic mechanisms…

We investigate nonlinear magnetoelastic wave dynamics and electrically tunable soliton excitations in hexagonal multiferroic media. By varying the magnetoelastic coupling strength and using a coupled magnetoelastic-ferroelectric continuum…

介观与纳米尺度物理 · 物理学 2026-03-09 Saumen Acharjee , Kallol Kavas Hazarika , Rajneesh Kakoti

Vibrational motions in electronically excited states can be observed by either time and frequency resolved infrared absorption or by off resonant stimulated Raman techniques. Multipoint correlation function expressions are derived for both…

量子物理 · 物理学 2017-09-13 Konstantin E. Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

Multi-configurational electronic structure theory delivers the most versatile approximations to many-electron wavefunctions, flexible enough to deal with all sorts of transformations, ranging from electronic excitations, to open-shell…

化学物理 · 物理学 2024-05-07 Kalman Szenes , Maximilian Moerchen , Paul Fischill , Markus Reiher

Non-Markovian quantum evolution of the electronic subsystem in a laser-driven molecule is characterized through the appearance of negative decoherence rates in the canonical form of the electronic master equation. For a driven molecular…

量子物理 · 物理学 2018-11-22 Mihaela Vatasescu

Following our recent numerical study [arXiv:2601.16299 (2026)], we investigate vibrational excitation induced by transient optical driving in molecular ensembles strongly coupled to a cavity mode using the field-driven…

When a quantum system couples strongly to multiple baths then it is generally no longer possible to describe the resulting system dynamics by simply adding the individual effects of each bath. However, capturing such multi-bath system…

Quantum information processing relies on how dynamics unfold in open quantum systems. In this work, we study the non-Markovian dynamics in the single mode spin-boson model at strong couplings. In order to apply perturbation theory, we…

量子物理 · 物理学 2025-01-03 Rayees A Mala , Mehboob Rashid , Muzaffar Qadir Lone
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