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We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

介观与纳米尺度物理 · 物理学 2015-05-13 I. V. Bondarev , K. Tatur , L. M. Woods

The optical absorption spectrum of the carbon (4,2) nanotube is computed using an ab-initio many-body approach which takes into account excitonic effects. We develop a new method involving a local basis set which is symmetric with respect…

材料科学 · 物理学 2009-11-10 Eric Chang , Giovanni Bussi , Alice Ruini , Elisa Molinari

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

材料科学 · 物理学 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

介观与纳米尺度物理 · 物理学 2015-05-13 I. V. Bondarev , L. M. Woods , K. Tatur

Exciton effects are studied in single-wall boron-nitride (BN) nanotubes. Linear absorption spectra are calculated with changing the chiral index of the zigzag nanotubes. We consider the extended Hubbard model with atomic energies at the…

材料科学 · 物理学 2009-07-07 Kikuo Harigaya

Exciton effects are studied in single-wall boron-nitride nanotubes. The Coulomb interaction dependence of the band gap, the optical gap, and the binding energy of excitons are discussed. The optical gap of the (5,0) nanotube is about 6eV at…

材料科学 · 物理学 2009-07-07 Kikuo Harigaya

We present a quantitative theory of optical absorption polarized transverse to the tube axes in semiconducting single-walled carbon nanotubes. Transverse optical absorption in semiconducting single-walled carbon nanotubes is to an exciton…

材料科学 · 物理学 2009-11-13 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

Exciton-exciton recombination in isolated semiconducting single-walled carbon nanotubes was studied using femtosecond transient absorption. Under sufficient excitation to saturate the optical absorption, we observed an abrupt transition…

统计力学 · 物理学 2015-06-17 J. Allam , M. T. Sajjad , R. Sutton , K. Litvinenko , Z. Wang , S. Siddique , Q-H. Yang , W. H. Loh , T. Brown

We use the macroscopic quantum electrodynamics approach suitable for absorbing and dispersing media to study the properties and role of collective surface excitations --- excitons and plasmons --- in single-wall and double-wall carbon…

介观与纳米尺度物理 · 物理学 2017-08-14 I. V. Bondarev , L. M. Woods , A. Popescu

We calculate the exciton binding energy in single-walled carbon nanotubes with narrow band gaps, accounting for the quasi-relativistic dispersion of electrons and holes. Exact analytical solutions of the quantum relativistic two-body…

介观与纳米尺度物理 · 物理学 2011-08-16 R. R. Hartmann , I. A. Shelykh , M. E. Portnoi

Electroabsorption spectroscopy of well-identified index-defined semiconducting carbon nanotubes is reported. The measurement of high definition electroabsorption spectra allows direct indexation with unique nanotube chirality. Results show…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

材料科学 · 物理学 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred…

材料科学 · 物理学 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

We present many-body \textit{ab initio} calculations of the electronic and optical properties of semiconducting zigzag carbon nanotubes under uniaxial strain. The GW approach is utilized to obtain the quasiparticle bandgaps and is combined…

材料科学 · 物理学 2015-06-16 Catalin D. Spataru , François Léonard

Light emission from carbon nanotubes is expected to be dominated by excitonic recombination. Here we calculate the properties of excitons in nanotubes embedded in a dielectric, for a wide range of tube radii and dielectric environments. We…

材料科学 · 物理学 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

We show that the absorption spectrum in semiconducting nanotubes can be determined using the bosonization technique combined with mean-field theory and a harmonic approximation. Our results indicate that a multiple band semiconducting…

介观与纳米尺度物理 · 物理学 2014-03-13 M. C. Sweeney , J. D. Eaves

We report benchmark calculations of electroabsorption in semiconducting single-walled carbon nanotubes to provide motivation to experimentalists to perform electroabsorption measurement on these systems. We show that electroabsorption can…

材料科学 · 物理学 2007-05-23 Hongbo Zhao , Sumit Mazumdar

We report correlated-electron calculations of optically excited states in ten semiconducting single-walled carbon nanotubes with a wide range of diameters. Optical excitation occurs to excitons whose binding energies decrease with the…

材料科学 · 物理学 2007-05-23 Hongbo Zhao , Sumit Mazumdar

The dipole-dipole interactions between excitons are of paramount importance in the nanoscale structures. When two excitons are placed together they can exchange the energy can manifest in the resonant Raman cross sections. We provide…

介观与纳米尺度物理 · 物理学 2024-04-09 Anna Wroblewska , Niclas S. Mueller , Mariusz Zdrojek , Stephanie Reich , Georgy Gordeev

We develop a scaling relationship between the exciton binding energy and the external dielectric function in carbon nanotubes. We show that the electron-electron and electron-hole interaction energies are strongly affected by screening yet…

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