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Graphene is at the centre of nanotechnology research. In order to fully exploit its outstanding properties, a mass production method is necessary. Two main routes are possible: large-scale growth or large-scale exfoliation. Here, we…

Liquid phase exfoliation (LPE) is the most promising method for the low-cost, scalable production of two-dimensional nanosheets from their bulk counterparts. Extensive exfoliation occurs in most solvents due to the huge amount of energy…

材料科学 · 物理学 2023-10-27 Urvesh Patil , Nuala M. Caffrey

Synthesis of graphene with reduced use of chemical reagents is essential for manufacturing scale-up and to control its structure and properties. In this paper, we report on a novel chemical-free mechanism of graphene exfoliation from…

We report the exfoliation of graphite in aqueous solutions under high shear rate [$\sim10^8s^{-1}$] turbulent flow conditions, with a 100\% exfoliation yield. The material is stabilized without centrifugation at concentrations up to 100 g/L…

We investigated the effect of surfactants and their concentration (Csur) on the final graphene concentration (CG) via the liquid-phase exfoliation method. Six typical surfactants including ionic and non-ionic ones were explored and the…

材料科学 · 物理学 2016-06-14 Shuai Wang , Min Yi , Shuaishuai Liang , Zhigang Shen , Xiaojing Zhang , Shulin Ma

Owing to wide variety of applications of graphene, high-quality and economical way of synthesizing graphene is highly desirable. In this study, we report a cost effective and simple approach to production of high-quality graphene. Here the…

材料科学 · 物理学 2013-10-29 Prashant Tripathi , Ch. Ravi Prakash Patel , M. A. Shaz , O. N. Srivastava

Bulk quantities of graphene nanosheets and nanodots have been selectively fabricated by mechanical grinding exfoliation of natural graphite in a small quantity of ionic liquids. The resulting graphene sheets and dots are solvent free with…

Graphene stands as a promising material with vast potential across energy storage, electronics, etc. Here, we present a novel mechanical approach utilizing ultrasonic high-energy intercalation exfoliation to extract monolayer graphene from…

材料科学 · 物理学 2025-01-15 Kaitong Sun , Si Wu , Junchao Xia , Yinghao Zhu , Guanping Xu , Hai-Feng Li

We have demonstrated a method to disperse and exfoliate graphite to give graphene suspended in water-surfactant solutions. Optical characterisation of these suspensions allowed the partial optimisation of the dispersion process.…

材料科学 · 物理学 2008-09-17 Y Hernandez , M Lotya , V Nicolosi , FM Blighe , S De , G Duesberg , JN Coleman

Inkjet printable graphene inks are very attractive for applications in flexible and foldable electronics, such as wearable electronics and the Internet of Things. However, the ink preparation is still very time consuming as high…

应用物理 · 物理学 2019-04-19 Khaled Parvez , Robyn Worsley , Adriana Alieva , Alexandre Felten , Cinzia Casiraghi

We use molecular dynamics simulation to study the exfoliation of graphene and fluorographene in molecular and ionic liquids, by performing computer experiments in which one layer of the 2D nanomaterial is peeled from a stack, in vacuum and…

介观与纳米尺度物理 · 物理学 2018-02-07 Emilie Bordes , Joanna Szala-Bilnik , Agílio A. H. Pádua

Liquid-phase exfoliation is one of the most promising routes for large scale production of multilayer graphene dispersions. These dispersions, which may be used in coatings, composites or paints, are believed to contain disorder-free…

介观与纳米尺度物理 · 物理学 2014-09-05 M. V. Bracamonte , G. I. Lacconi , S. Urreta , L. E. F. Foa Torres

Dispersing graphite in water to obtain true (single layer) graphene (SLG) in bulk quantity in a liquid has been an unreachable goal for materials scientists in the last decade. Likewise, a diagnostic tool for identifying solubilized SLG in…

Graphene is an intriguing material with properties that are distinct from those of other graphitic systems. The first samples of pristine graphene were obtained by peeling off and epitaxial growth. Recently, the chemical reduction of…

材料科学 · 物理学 2015-05-13 Xiaolin Li , Guangyu Zhang , Xuedong Bai , Xiaoming Sun , Xinran Wang , Enge Wang , Hongjie Dai

An efficient route to synthesize macroscopic amounts of graphene is highly desired and a bulk characterization of such samples, in terms of the number of layers, is equally important. We present a Raman spectroscopy-based method to…

A simple solvent exchange method is introduced to prepare high-concentration and surfactant-free graphene liquid dispersion. Natural graphite flakes are first exfoliated into graphene in dimethylformamide (DMF). DMF is then exchanged by…

材料科学 · 物理学 2012-05-10 Jiantong Li , Fei Ye , Sam Vaziri , Mamoun Muhammed , Max C. Lemme , Mikael Östling

Few layer graphene (FLG) was synthesized by $\mu$-wave assisted exfoliation of expanded graphite in toluene with an overall yield from c.a. 7% to 20%. A significant difference in the absorption of $\mu$-waves by the expanded graphite and…

Liquid-phase exfoliation, the use of a sheared liquid to delaminate graphite into few-layer graphene, is a promising technique for the large-scale production of graphene. But the micro and nanoscale fluid-structure processes controlling the…

软凝聚态物质 · 物理学 2020-04-22 Simon Gravelle , Catherine Kamal , Lorenzo Botto

We show that by using an original method, bulk graphite can be bonded onto borosilicate glass or potentially any insulating substrate with ionic conductivity and then cleaved off to leave single or few layer graphene on the substrate,…

材料科学 · 物理学 2009-04-06 Abhay Shukla , Rakesh Kumar , Javed Mazher , Adrian Balan

In this work, linear polystyrene-poly(2-vinylpyridine) (PS-b-P2VP) and heteroarm star PS_22P2VP_22 ionizable block copolymers were used as dispersing agents for the liquid-phase exfoliation of pristine graphene. Various strategies such as…

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