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In present work we calculated the three components of polarization in phenomenological theory framework by consideration of three Euler-Lagrange equations, which include mismatch effect and influence of misfit dislocations, surface…

软凝聚态物质 · 物理学 2015-06-25 M. D. Glinchuk , A. N. Morozovska , E. A. Eliseev

The origin of the unusual 90^o ferroelectric / ferroelastic domains, consistently observed in recent studies on meso and nanoscale free-standing single crystals of BaTiO3 [Schilling et al., Physical Review B, 74, 024115 (2006); Schilling et…

材料科学 · 物理学 2009-04-13 I. A. Luk'yanchuk , A. Schilling , J. M. Gregg , G. Catalan , J. F. Scott

For the first time we proposed the model for the calculations of the relaxor ferroelectrics films properties in the framework of the random field theory. We took into account the misfit strain between film and substrate as well as surface…

材料科学 · 物理学 2007-05-23 E. A. Eliseev , M. D. Glinchuk

Recent observations of unusual ferroelectricity in thin films of HfO_2 and related materials have attracted broad interest to the materials and led to the emergence of a number of competing models for observed behaviors. Here we develop the…

材料科学 · 物理学 2018-11-27 Maya D. Glinchuk , Anna N. Morozovska , Yunseok Kim , Sergei V. Kalinin

The interaction of electric field with charged domain walls in ferroelectrics is theoretically addressed. A general expression for the force acting per unit area of a charged domain wall carrying free charge is derived. It is shown that, in…

材料科学 · 物理学 2012-01-31 Maxim Y. Gureev , Pavel Mokry , Alexander K. Tagantsev , Nava Setter

We theoretically explore mechanisms that can potentially give rise to the steady-state and transient negative capacitance in a uniaxial ferroelectric film stabilized by a dielectric layer. The analytical expressions for the steady-state…

To minimize their electrostatic energy, insulating ferroelectric films tend to break up into nanoscale ``Kittel'' domains of opposite polarization that are separated by uncharged 180$^\circ$ domain walls. Here, I report on self-consistent…

介观与纳米尺度物理 · 物理学 2022-10-14 W. A. Atkinson

Using direct variational method with 2-parametric trial function and Landau-Ginzburg-Devonshire thermodynamical approach, we derived analytical expressions for polarization spatial redistribution in the ferroelectrics caused by the biased…

材料科学 · 物理学 2010-04-16 Anna N. Morozovska

We study theoretically and by means of molecular dynamics (MD) simulations the generation of mechanical force by grafted polyelectrolytes in an external electric field, which favors its adsorption on the grafting plane. The force arises in…

软凝聚态物质 · 物理学 2016-03-18 N. V. Brilliantov , Yu. A. Budkov , C. Seidel

The wealth of complex polar topologies recently found in nanoscale ferroelectrics result from a delicate balance between the materials intrinsic tendency to develop a homogeneous polarization and the electric and mechanic boundary…

The theory of size effects of the properties of nanocrystalline ferroelectric ceramic or nanoparticle powder allowing for surface tension and depolarization field is proposed. Surface tension was included into free energy functional and…

材料科学 · 物理学 2015-06-24 M. D. Glinchuk , A. N. Morozovskaya

Using the plasma model for the metal dielectric function we have calculated the electromagnetic fluctuation induced forces on a free standing metallic film in vacuum as a function of the film size and the plasma frequency. The force for…

量子物理 · 物理学 2009-11-13 Andrea Benassi , Carlo Calandra

We explore the force generation and surface interactions arising when electric fields are applied across fluid films. Using a surface force balance (SFB) we measure directly the force between two electrodes in crossed-cylinder geometry…

软凝聚态物质 · 物理学 2019-04-09 Carla Perez-Martinez , Susan Perkin

Phase decomposition is a well-known process leading to the formation of two-phase mixtures. Here we show that a strain imposed on a ferroelastic crystal promotes the formation of mixed phases and domains, i.e., domain and phase de-strain…

材料科学 · 物理学 2016-12-21 Fei Xue , Yongjun Li , Yijia Gu , Jinxing Zhang , Long-Qing Chen

Ferroelectrics form domain patterns that minimize their energy subject to imposed boundary conditions. In a linear, constrained theory, that neglects domain wall energy, periodic domain patterns in the form of multi-rank laminates can be…

材料科学 · 物理学 2018-03-20 Ananya Renuka Balakrishna , John E. Huber , Ingo Münch

The electrostatics arising in ferroelectric/dielectric two-dimensional heterostructures and superlatitices is revisited here within a simplest Kittel model, in order to define a clear paradigmatic reference for domain formation. The…

介观与纳米尺度物理 · 物理学 2022-08-12 Daniel Bennett , Maitane Muñoz-Basagoiti , Emilio Artacho

A thermodynamic theory of ferroelectric thin film multilayers is developed. The free energy function is written down using a multilayer model in which c-domain layers of one ferroelectric material alternate with a-domain layers of a second…

材料科学 · 物理学 2007-05-23 M. D. Glinchuk , E. A. Eliseev , V. A. Stephanovich , M. G. Karkut , R. Farhi

The calculation of the polarization in ferroelectric thin films is performed using an analytical solution of the Euler-Lagrange differential equation with boundary conditions with different extrapolation lengths of positive sign on the…

材料科学 · 物理学 2007-05-23 M. D. Glinchuk , E. A. Eliseev , V. A. Stephanovich , R. Farhi

We report first-principle atomistic simulations on the effect of local strain gradients on the nanoscale domain morphology of free-standing PbTiO$_3$ ultrathin films. First, the ferroelectric properties of free films at the atomic level are…

材料科学 · 物理学 2015-06-22 G. D. Belletti , S. D. Dalosto , Silvia Tinte

We analyze theoretically and by means of molecular dynamics (MD) simulations the generation of mechanical force by a polyelectrolyte (PE) chain grafted to a plane. The PE is exposed to an external electric field that favors its adsorption…

软凝聚态物质 · 物理学 2016-11-23 N. V. Brilliantov , Yu. A. Budkov , C. Seidel