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Interfaces between dissimilar materials control the transport of energy in a range of technologies including solar cells (electron transport), batteries (ion transport), and thermoelectrics (heat transport). Advances in computer power and…

材料科学 · 物理学 2018-12-06 Ji-Sang Park , Young-Kwang Jung , Keith T. Butler , Aron Walsh

In the present study, two-different reduced-order models are proposed for $\text{H}_2\left(\text{X}^1\Sigma_g^+\right)$+$\text{H}\left({}^2\text{S}\right)$ system by leveraging first-principle quasi-classical trajectory simulations and…

化学物理 · 物理学 2026-01-29 Hye Su Jeong , Tae Woong Jeong , Sung Min Jo

The possible formation of oxides or thin oxide films (surface oxides) on late transition metal surfaces is recently being recognized as an essential ingredient when aiming to understand catalytic oxidation reactions under technologically…

材料科学 · 物理学 2009-11-13 Jutta Rogal , Karsten Reuter , Matthias Scheffler

We investigate limit models resulting from a dimensional analysis of quite general heterogeneous catalysis models with fast sorption (i.e.\ exchange of mass between the bulk phase and the catalytic surface of a reactor) and fast surface…

偏微分方程分析 · 数学 2021-05-10 Björn Augner , Dieter Bothe

A new two-layer model has been proposed to study microscale heat transfer associated with a developing flow boundary layer. As an example, a cold, microscale film of liquid impinging on an isothermal hot, horizontal surface has been…

流体动力学 · 物理学 2014-03-18 Jian-Jun Shu

Estimating the heat loads on re-entry vehicles is a crucial part of preparing for atmospheric re-entry manoeuvres. Re-entry flows at high altitudes are in the rarefied regime and are governed by high enthalpies and thermodynamic…

计算物理 · 物理学 2020-07-14 Wladimir Reschke , Marcel Pfeiffer , Stefanos Fasoulas

We present a multi-lattice kinetic Monte Carlo (kMC) approach that efficiently describes the atomistic dynamics of morphological transitions between commensurate structures at crystal surfaces. As an example we study the reduction of a…

介观与纳米尺度物理 · 物理学 2015-01-09 Max J. Hoffmann , Matthias Scheffler , Karsten Reuter

We present a density-functional theory based kinetic Monte Carlo study of CO oxidation at the (111) facet of RuO$_2$. We compare the detailed insight into elementary processes, steady-state surface coverages and catalytic activity to…

材料科学 · 物理学 2015-12-09 Tongyu Wang , Karsten Reuter

Fabrication, handling and disposal of nuclear fuel materials require comprehensive knowledge of their surface morphology and reactivity. Due to unavoidable contact with air components (even at low partial pressures), UN samples contain…

In this opinion piece, we discuss recent advances in experimental methods for characterizing phase change heat transfer. We begin with a survey of techniques for high-resolution measurements of temperature and heat flux at the solid surface…

介观与纳米尺度物理 · 物理学 2014-08-04 Jacopo Buongiorno , David G. Cahill , Carlos H. Hidrovo , Saeed Moghaddam , Aaron J. Schmidt , Li Shi

In fire spread simulations, heat transfer and pyrolysis are processes to describe the thermal degradation of solid material. In general, the necessary material parameters cannot be directly measured. They are implicitly deduced from micro-…

流体动力学 · 物理学 2023-06-28 Tristan Hehnen , Lukas Arnold

The incredible thermo-mechanical properties of biological materials arise from the microscopic scale due to a complex hierarchical mechanism, regulated by microinstabilities at the molecular level. The description of such complex structures…

生物物理 · 物理学 2022-10-26 Luca Bellino

As an aid to the development of hydrogen separation membranes, we predict the temperature dependent phase diagrams using first principles calculations combined with thermodynamic principles. Our method models the phase diagram without…

材料科学 · 物理学 2014-08-07 William Paul Huhn , Michael Widom , Michael C. Gao

A quantum interatomic scattering is implemented in the direct simulation Monte Carlo (DSMC) method applied to transport phenomena in rarefied gases. In contrast to the traditional DSMC method based on the classical scattering, the proposed…

计算物理 · 物理学 2025-07-16 Felix Sharipov

The theoretical description of materials' properties driven out of equilibrium has important consequences in various fields such as semiconductor spintronics, nonlinear optics, continuous and discrete quantum information science and…

材料科学 · 物理学 2025-09-18 Jacopo Simoni , Gabriele Riva , Yuan Ping

Understanding how properties of materials change due to nuclear transmutations is a major challenge for the design of structural components for a fusion power plant. In this study, by combining a first-principles matrix Hamiltonian approach…

A study of a reacting boundary layer flow with heat transfer at conditions typical for configurations at elevated pressures has been performed using a set of direct numerical simulations. Effects of wall temperatures are investigated,…

流体动力学 · 物理学 2021-02-16 Nikolaos Perakis , Oskar Haidn , Matthias Ihme

We use a general circulation model to study the three-dimensional (3-D) flow and temperature distributions of atmospheres on tidally synchronized extrasolar planets. In this work, we focus on the sensitivity of the evolution to the initial…

地球与行星天体物理 · 物理学 2015-05-18 Heidar Th. Thrastarson , James Y-K. Cho

First principles calculations based on density functional theory, with generalised gradient corrections and ultrasoft pseudopotentials, have been used to simulate solid and liquid aluminium in direct coexistence at zero pressure.…

材料科学 · 物理学 2009-11-10 Dario Alfè

A series of First Principles calculations is undertaken to characterize and explain the enhancement of the catalytic activity of oxygen on top of very disordered nanomaterials of Pt. As the adsorption of OH fragment on top of the surfaces…

材料科学 · 物理学 2024-02-02 Olivier Le Bacq