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$^{77}$Se-NMR spectrum and frequency shift measurements in the paramagnetic metal (PM) and antiferromagnetic insulating (AFI) phases are reported for a small single crystal of the organic conductor $\lambda-$(BETS)$_{2}$FeCl$_{4}$ as a…

强关联电子 · 物理学 2009-11-13 Guoqing Wu , W. G. Clark , S. E. Brown , J. S. Brooks , A. Kobayashi , H. Kobayashi

The highly insulating antiferromagnetic phase of the magnetic- organic conductor lambda-(BETS)2FeCl4 has been probed by resonant mm wave methods vs. magnetic field, temperature, and frequency. Our results show evidence for magnetic…

强关联电子 · 物理学 2007-05-23 I. Rutel , S. Okubo , H. Ohta , H. Tanaka , H. Kobayashi , J. Brooks

We have performed high-field Electron Magnetic Resonance (EMR) measurements of lamda-(BETS)2FexGa1-xCl4 to clarify the role of Pi- and d-electrons in the paramagnetic (PM) and field-induced superconducting (FISC) phases. We found that this…

In the organic charge transfer salt k-(BETS)2Mn[N(CN)2]3 the metallic conductivity is provided by itinerant pi-electrons in the layers of BETS molecules, whereas magnetization is largely dominated by the localized d-electrons of the Mn2+…

强关联电子 · 物理学 2017-12-06 O. M. Vyaselev , W. Biberacher , N. D. Kushch , M. V. Kartsovnik

The low-temperature electronic state of the layered organic charge-transfer salt $\kappa$-(BETS)$_2$FeCl$_4$ was probed by interlayer electrical resistance measurements under magnetic field. Both above and below $T_{\mathrm{N}}=0.47\,$K,…

强关联电子 · 物理学 2016-11-09 Michael Kunz , Werner Biberacher , Natalia D. Kushch , Akira Miyazaki , Mark V. Kartsovnik

The experimental studies of the paramagnetic-antiferromagnetic phase transition through M\"{o}ssbauer spectroscopy and measurements of temperature and field dependencies of magnetic susceptibility in the layered Cu$_{0.15}$Fe$_{0.85}$PS$_3$…

计算物理 · 物理学 2023-01-05 V. Pashchenko , O. Bludov , D. Baltrunas , K. Mazeika , S. Motria , K. Glukhov , Yu. Vysochanskii

We report results of 77Se NMR frequency shift in the normal state of the organic charge-transfer-salt k-(BETS)2FeBr4 which shows magnetic field-induced superconductivity (FISC). From a simple mean field analysis, we determined the field and…

超导电性 · 物理学 2011-11-09 S. Fujiyama , M. Takigawa , J. Kikuchi , H-B. Cui , H. Fujiwara , H. Kobayashi

A complex study of magnetic properties including dc magnetization, 1H NMR and magnetic torque measurements has been performed for the organic conductor kappa-(BETS)2Mn[N(CN)2]3 which undergoes a metal-insulator transition at T_MI~25K. NMR…

强关联电子 · 物理学 2012-04-17 O. M. Vyaselev , M. V. Kartsovnik , W. Biberacher , L. V. Zorina , N. D. Kushch , E. B. Yagubskii

The two-dimensional organic conductor lambda-(BETS)2FeCl4 has an unusual phase diagram as a function of temperature and magnetic field that includes a paramagnetic metal (PM) phase, an antiferromagnetic insulating (AFI) phase, and a…

强关联电子 · 物理学 2007-05-23 W. G. Clark , Guoqing Wu , P. Ranin , L. K. Montgomery , L. Balicas

The synthetic organic compound lambda-(BETS)2FeCl4 undergoes successive transitions from an antiferromagnetic insulator to a metal and then to a superconductor as a magnetic field is increased. We use a Hubbard-Kondo model to clarify the…

强关联电子 · 物理学 2009-11-07 O. Cepas , Ross H. McKenzie , J. Merino

Submillimeter and millimeter wave electron spin resonance (ESR) measurements of the pi-d correlated organic conductor lambda-(BETS)2Fe0.6Ga0.4Cl4 have been performed. Antiferromagnetic resonance (AFMR) has been observed in the insulating…

We study the transition from paramagnetic metal to paramagnetic insulator by finite temperature Quantum Monte-Carlo simulations for the 2D Hubbard model at half-filling. Working at the moderately high temperature T=0.33*t where the spin…

强关联电子 · 物理学 2007-05-23 C. Groeber , M. G. Zacher , R. Eder

We have performed $^{77}$Se NMR on a single crystal sample of the field induced superconductor $\lambda$-(BETS)$_{2}$FeCl$_{4}$. Our results obtained in the paramagnetic state provide a microscopic insight on the exchange interaction $J$…

Superconducting FeSe has been investigated by measurements of the magnetic susceptibility versus temperature and Moessbauer spectroscopy at various temperatures including strong external magnetic fields applied to the absorber. It was found…

超导电性 · 物理学 2010-03-11 A. Blachowski , K. Ruebenbauer , J. Zukrowski , J. Przewoznik , K. Wojciechowski , Z. M. Stadnik

FeSe has been extensively explored as a quantum material, primarily due to the observed highest superconducting transition temperature among Fe-based unconventional superconductors. Nonetheless, the electronic structure and the electron…

强关联电子 · 物理学 2023-10-31 Byungkyun Kang , Maengsuk Kim , Chul Hong Park , Anderson Janotti

We study the unconventional insulating state in A_4C_{60} with a variety of approaches, including density functional calculations and dynamical mean-field theory. While the former predicts a metallic state, in disagreement with experiment,…

强关联电子 · 物理学 2007-08-07 M. Capone , M. Fabrizio , P. Giannozzi , E. Tosatti

We present a coordinated study of the paramagnetic-to-antiferromagnetic, rhombohedral-to-monoclinic, and metal-to-insulator transitions in thin-film specimens of the classic Mott insulator V$_2$O$_3$ using low-energy muon spin relaxation,…

The thermal conductivity kappa of the quasi-two-dimensional (Q2D) organic superconductor lambda-(BETS)_2 GaCl_4 was studied in the magnetic field H applied parallel to the Q2D plane. The phase diagram determined from this bulk measurement…

超导电性 · 物理学 2009-11-07 M. A. Tanatar , T. Ishiguro , H. Tanaka , H. Kobayashi

We study the magnetic, structural, and electronic properties of the recently discovered iron- based superconductor BaFe2S3 based on density functional theory with the generalized gradient approximation. The calculations show that the…

强关联电子 · 物理学 2015-08-19 Michi-To Suzuki , Ryotaro Arita , Hiroaki Ikeda

We report on investigations of the complex magnetostructural and spin-state transitions in the breathing pyrochlore LiFeCr$_{4}$O$_{8}$ by means of magnetization, M\"ossbauer spectroscopy, and density functional theory (DFT) calculations.…

强关联电子 · 物理学 2023-12-05 Bo Zhang , Wei Ren , Shengyu Yang , Qifeng Kuang , Da Li , Xin Liu , Anmin Zhang , Hua Pang , Liyun Tang , Liang Qiao , Fashen Li , Zhiwei Li
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