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We present a derivation of the orbital and spin sum rules for magnetic circular dichroic spectra measured by electron energy loss spectroscopy in a transmission electron microscope. These sum rules are obtained from the differential cross…

其他凝聚态物理 · 物理学 2009-11-13 L. Calmels , F. Houdellier , B. Warot-Fonrose , C. Gatel , M. J. Hÿtch , V. Serin , E. Snoeck , P. Schattschneider

Polarization-dependent photon spectroscopy (dichroism) using signal-enhancing superchiral beams is shown to be sensitive to magnetic properties of the sample, whereas previous investigations explored charge-like electronic properties of…

材料科学 · 物理学 2019-03-06 S. W. Lovesey , J. T. Collins , S. P. Collins

We demonstrate electron magnetic linear dichroism as a quantitative probe of vectorial magnetic order parameters with nanometer resolution in transmission electron microscopy. Explicit inclusion of vectorial core-level exchange splitting…

介观与纳米尺度物理 · 物理学 2026-05-28 Jan Hajduček , Jáchym Štindl , Ján Rusz , Vojtěch Uhlíř

Use of electron vortex beams (EVB), that is convergent electron beams carrying an orbital angular momentum (OAM), is a novel development in the field of transmission electron microscopy. They should allow measurement of element-specific…

材料科学 · 物理学 2015-06-19 Jan Rusz , Somnath Bhowmick , Mattias Eriksson , Nikolaj Karlsson

It was claimed (Lloyd et al., PRL 108 (2012) 074802) that energy loss magnetic chiral dichroism (EMCD) with electron vortex beams is feasible, and has even advantages over the standard setup with Bragg diffracted waves. In this Comment, we…

量子物理 · 物理学 2017-02-16 Peter Schattschneider , Stefan Löffler , Johan Verbeeck

Photoemission electron microscopy (PEEM) has evolved into an indispensable tool for structural and magnetic characterization of surfaces at the nanometer scale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a leading…

Electronic circular dichroism (ECD) is a powerful spectroscopical method for investigating chiral properties at the molecular level. ECD calculations with the commonly used linear-response time-dependent density functional theory (LR-TDDFT)…

Imaging the magnetic configuration of thin-films has been a long-standing area of research. Since a few years, the emergence of two-dimensional ferromagnetic materials calls for innovation in the field of magnetic imaging. As the magnetic…

材料科学 · 物理学 2021-01-13 T. Guillet , A. Marty , C. Vergnaud , F. Bonell , M. Jamet

A new material characterization technique is emerging for the transmission electron microscope (TEM). Using electron energy-loss spectroscopy, real space mappings of the underlying electronic transitions in the sample, so called orbital…

材料科学 · 物理学 2023-05-26 Manuel Ederer , Stefan Löffler

In photoelectron circular dichroism (PECD) it is generally difficult to trace how and when the chirality of the molecule is imprinted onto the photoelectron. We present simulations of PECD in a simple model and employ chirality measures to…

原子物理 · 物理学 2025-03-04 Marec W. Heger , Daniel M. Reich

Recent quantitative measurements of the orbital to spin magnetic moment ratio $m_L/m_S$ in electron magnetic circular dichroism (EMCD) experiments have given a $m_L/m_S$ ratio that is larger than commonly accepted values. We demonstrate…

Electronic circular dichroism (ECD) spectroscopy captures the chiroptical response of molecules, enabling absolute configuration assignment that is vital for enantioselective synthesis and drug design. The practical use of ECD spectra in…

量子物理 · 物理学 2026-02-04 Amandeep Singh Bhatia , Sabre Kais

The emergence of optical circular dichroism in chiral nanoscale and molecular systems provides not only a way for analyzing the sample chirality itself but also additional degrees of freedom in manipulating light. Such manipulation can be…

介观与纳米尺度物理 · 物理学 2026-02-18 Marek Zálešák , Martin Ošmera , Martin Hrtoň , Andrea Konečná

The Scanning electron microscope (SEM) and Electron-Dispersive Spectroscope (EDS) are two highly effective instruments in the field of nanoscience and nanotechnology. The quality of these instruments is determined by various factors, with…

应用物理 · 物理学 2023-10-24 Hamidreza Moradi , Fatemeh Mehradnia

Magneto-optical microscopies, including optical measurements of magnetic circular dichroism, are increasingly ubiquitous tools for probing spin-orbit coupling, charge-carrier g-factors, and chiral excitations in matter, but the minimum…

X-ray magnetic circular dichroism (XMCD) has become an important and powerful tool because it allows the study of material properties in combination with elemental specificity, chemical state specificity, and magnetic specificity. A new…

仪器与探测器 · 物理学 2015-06-19 Zhi-Ying Guo , Cai-Hao Hong , Hai-Ying Xing , Kun Tang , Wei Xui , Dong-liang Chen , Ming-Qi Cui , YI-Dong Zhao

Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…

Chiral and axial materials offer platforms for intriguing phenomena, such as cross-correlated responses and chirality-induced spin selectivity. However, quantifying the properties of such materials has generally been considered challenging.…

材料科学 · 物理学 2025-10-07 Tatsuya Miki , Hiroaki Ikeda , Michi-To Suzuki , Shintaro Hoshino

Electromagnetic moments of particles carry important information on their internal structure, as well as on the structure of the effective Lagrangian describing their underlying field theory. One of the cleanest observable of such kind is…

广义相对论与量子宇宙学 · 物理学 2021-06-01 Andras Laszlo , Zoltan Zimboras

A light beam can carry both spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is commonly evidenced by circular dichroism (CD) experiments {\em i. e.} differential absorption of left and right-handed circularly polarized…