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Fe K-edge and Se K-edge x-ray absorption near edge structure (XANES) measurements are used to study FeSe$_{1-x}$Te$_{x}$ electronic structure of chalcogenides. An intense Fe K-edge pre-edge peak due to Fe 1s$\to$3d (and admixed Se/Te $p$…

超导电性 · 物理学 2010-12-08 B. Joseph , A. Iadecola , L. Simonelli , Y. Mizuguchi , Y. Takano , T. Mizokawa , N. L. Saini

The growing interest in tin-halide semiconductors for photovoltaic applications demands an in-depth knowledge of the fundamental properties of its constituents, starting from the smallest monomers entering the initial stages of formation.…

材料科学 · 物理学 2024-02-21 Freerk Schütt , Ana M. Valencia , Caterina Cocchi

The structural properties of the ROFeM (R=La, Nd; M=As, P) materials have been analyzed by means of electron diffraction, high-resolution transmission-electron microscopy (TEM) and in-situ cooling TEM observations. The experimental results…

超导电性 · 物理学 2009-11-13 C. Ma , L. J. Zeng , H. X. Yang , H. L Shi , R. C. Che , C. Y. Liang , Y. B. Qin , G. F. Chen , Z. A. Ren , J. Q. Li

Experiments on rare-earth filled skutterudites demonstrate an intriguing array of thermodynamic, transport and superconducting properties, and bring to fore theoretical challenges posed by f-electron systems. First principle calculations…

强关联电子 · 物理学 2019-09-11 Gheorghe Lucian Pascut , Michael Widom , Kristjan Haule , Khandker F. Quader

We have carried out a first principles study of the elastic properties and electronic structure for two room-temperature stable Pt silicide phases, tetragonal alpha-Pt_2Si and orthorhombic PtSi. We have calculated all of the equilibrium…

材料科学 · 物理学 2009-10-31 O. Beckstein , J. E. Klepeis , G. L. W. Hart , O. Pankratov

We present first-principles investigation of the electronic structure and magnetic properties of uranium monochalcogenides: US, USe, UTe. The calculations were performed by using recently developed LDA+U+SO method in which both Coulomb and…

强关联电子 · 物理学 2015-05-14 A. O. Shorikov , J. E. Medvedeva , A. I. Poteryaev , V. V. Mazurenko , V. I. Anisimov

Using first-principles density functional calculations, we have studied the structural stability of stoichiometric as well as non-stoichiometric CdS nanoclusters at ambient pressure with diameters ranging up to about 2.5 nm. Our study…

原子与分子团簇 · 物理学 2011-06-07 Soumendu Datta , Mukul Kabir , Tanusri Saha-Dasgupta , D. D. Sarma

The latest discovery of a new iron-chalcogenide superconductor A$_x$Fe$_{2-y}$Se$_2$(A=K, Cs, Rb, Tl and etc.) has attracted much attention due to a number of its unique characteristics, such as the possible insulating state of the parent…

超导电性 · 物理学 2012-01-04 Daixiang Mou , Lin Zhao , Xingjiang Zhou

The electronic structure of some europium chalcogenides and pnictides is calculated using the {\it ab-initio} self-interaction corrected local-spin-density approximation (SIC-LSD). This approach allows both a localised description of the…

强关联电子 · 物理学 2016-08-31 M. Horne , P. Strange , W. M. Temmerman , Z. Szotek , A. Svane , H. Winter

The structure of chalcogenide glassy semiconductors in three-component systems of Ge-As-Se and As-Sb-Se has been studied by means of both NQR and EPR spectroscopy. Investigation of mutual local coordination of atoms has been performed. The…

The first-principles calculations have been performed to investigate the ground state properties of cubic scandium trifluoride (ScF$_3$) perovskite. Using modified hybrid exchange-correlation functionals within the density functional theory…

材料科学 · 物理学 2012-11-27 P. Zhgun , D. Bocharov , S. Piskunov , A. Kuzmin , J. Purans

The structural, electronic, mechanical and thermal properties of Ir$_{1-x}$Rh$_{x}$ alloys were studied systematically using ab initio density functional theory at different concentrations (x = 0.00, 0.25, 0.50, 0.75, 1.00). A Special…

材料科学 · 物理学 2015-06-15 S. Ahmed , M. Zafar , M. Shakil , M. A. Choudhary

Employing first-principle electronic structure calculations, we study the magnetic and electronic properties of the XY (X= Mg, Ca, Sr and Y= N, P, As, Sb) compounds crystallizing in the zincblende structure. The Ca and Sr alkaline-earth…

材料科学 · 物理学 2012-10-30 K. Ozdogan , I. Galanakis

The finding of superconductivity in Ba0.6K0.4Fe2As2 put the attention on the investigation of compounds that crystallize with ThCr2Si2 structure type such as AT2X2 (A = alkali/ alkaline earth/ rare earth element; T = transition metal and X…

超导电性 · 物理学 2012-12-10 Andrea V. Hoffmann , Viktor Hlukhyy , Thomas F. Fässler

In this work, we explore the electronic properties and chemical bonding in the recently discovered mineral zaykovite, the first natural rhodium selenide Rh$_3$Se$_4$. We comprehensively studied the bulk electronic structure, hybridization…

材料科学 · 物理学 2024-10-08 Leonid S. Taran , Sergey V. Eremeev , Sergey V. Streltsov

Small clusters of the As/Sb-S/Se system that is of importance for simulation of elementary structure units of chalcogenide glasses are calculated using DFT technique. Different structures of As2Xn- and Sb2Xn- (X=S,Se) with proper hydrogen…

材料科学 · 物理学 2015-04-02 V. Gurin , O. Shpotyuk , V. Boyko

First-principles-based materials screening is systematically performed to discover new combinations of chemical elements possibly making shape-memory alloys (SMAs). The B2, D03, and L21 crystal structures are considered as the parent…

材料科学 · 物理学 2017-12-15 Joohwi Lee , Yuji Ikeda , Isao Tanaka

Novel ordered intermetallic compounds have stimulated much interest. Ru-Al alloys are a prominent class of high-temperature structural materials, but the experimentally reported crystal structure of the intermetallic Ru2Al5 phase remains…

材料科学 · 物理学 2024-09-02 Jing Luo , Meiguang Zhang , Xiaofei Jia , Xuanmin Zhu , Qun Wei

Boosted by the relentless increase of available computational resources, high-throughput calculations based on first principles methods have become a powerful tool to screen a huge range of materials. The backbone of these studies are…

材料科学 · 物理学 2022-03-23 Holger-Dietrich Saßnick , Caterina Cocchi

The typical two-dimensional semiconductors, group \uppercase\expandafter{\romannumeral3A} chalcogenides, have garnered tremendous interest for their outstanding electronic, mechanical, and chemical properties. However, so far, there have…

材料科学 · 物理学 2020-09-10 Dong Fan , Chuncheng Yang , Shaohua Lu , Xiaojun Hu