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Experiments with cold ion-atom mixtures have recently opened the way for the production and application of ultracold molecular ions. Here, in a comparative study, we theoretically investigate ground and several excited electronic states and…

原子物理 · 物理学 2020-08-12 Wissem Zrafi , Hela Ladjimi , Halima Said , Hamid Berriche , Michał Tomza

We have produced ultracold, polar RbCs* molecules via photoassociation in a laser-cooled mixture of Rb and Cs atoms. Using a model of the RbCs* molecular interaction which reproduces the observed rovibrational structure, we infer decay…

原子物理 · 物理学 2009-11-10 Andrew J. Kerman , Jeremy M. Sage , Sunil Sainis , David DeMille , Thomas Bergeman

We investigate pump-dump photoassociation of ultracold molecules with amplitude- and phase-modulated femtosecond laser pulses. For this purpose a perturbative model for the light-matter interaction is developed and combined with a genetic…

We predict that pairs of polar molecules can be weakly bound together in an ultracold environment, provided that a dc electric field is present. The field that links the molecules together also strongly influences the basic properties of…

原子物理 · 物理学 2009-11-07 A. V. Avdeenkov , J. L. Bohn

Photoassociation of ultracold atoms is a resonant light-assisted collision process, in which two colliding atoms absorb a photon and form an excited molecule. Since the first observation about three decades ago, the photoassociation of…

原子物理 · 物理学 2024-03-19 Jin Cao , Bo-Yuan Wang , Huan Yang , Zhi-Jie Fan , Zhen Su , Jun Rui , Bo Zhao , Jian-Wei Pan

The light scattered by cold atoms induces mutual optical forces between them, which can lead to bound states. In addition to the trapping potential, this light-induced interaction generates a velocity-dependent force which damps or…

原子物理 · 物理学 2020-07-01 Angel T. Gisbert , Nicola Piovella , Romain Bachelard

Mergoassociation of two ultracold atoms to form a weakly bound molecule can occur when two optical traps that each contain a single atom are merged. Molecule formation occurs at an avoided crossing between a molecular state and the lowest…

原子物理 · 物理学 2023-10-04 Robert C. Bird , C. Ruth Le Sueur , Jeremy M. Hutson

Photoassociation with short laser pulses has been proposed as a technique to create ultracold ground state molecules. A broad-band excitation seems the natural choice to drive the series of excitation and deexcitation steps required to form…

原子物理 · 物理学 2010-09-21 Christiane P. Koch , Mamadou Ndong , Ronnie Kosloff

The formation of ultracold molecules via stimulated emission followed by a radiative deexcitation cascade in the presence of a static electric field is investigated. By analyzing the corresponding cross sections, we demonstrate the…

量子物理 · 物理学 2007-06-06 Rosario González-Férez , Michael Mayle , Peter Schmelcher

We develop the theory for the Adiabatic Raman Photoassociation (ARPA) of ultracold atoms to form ultracold molecules in the presence of scattering resonances. Based on a computational method in which we replace the continuum with a discrete…

原子物理 · 物理学 2012-11-27 Alex C. Han , Evgeny A. Shapiro , Moshe Shapiro

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

介观与纳米尺度物理 · 物理学 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

We study the expansion of a strongly coupled, non-neutral, and cylindrically arranged ion plasma into the vacuum. The plasma is made from cold rubidium atoms in a magneto-optical trap (MOT) and is formed via ultraviolet photoionization.…

原子物理 · 物理学 2020-09-09 Michael A. Viray , Stephanie A. Miller , Georg Raithel

Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an…

量子气体 · 物理学 2026-04-17 Yun Chen , Yuqi Wang , Jingjun You , Yingqi Liu , Su Yi , Yuangang Deng

We show theoretically that it is possible to create and manipulate a pair of bound states in continuum in ultracold atoms by two lasers in the presence of a magnetically tunable Feshbach resonance. These bound states are formed due to…

原子与分子团簇 · 物理学 2016-09-15 Bimalendu Deb , G. S. Agarwal

We present a theoretical analysis of optical pathways for formation of cold Ca($^1$S)Na$^+$($^1$S) molecular ions via an intermediate state. The formation schemes are based on ab initio potential energy curves and transition dipole moments…

原子物理 · 物理学 2016-08-03 Marko Gacesa , John A. Montgomery , H. Harvey Michels , Robin Côté

The strong evanescent field around ultra-thin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold atom cloud, we investigate the interaction of a small…

量子物理 · 物理学 2009-11-13 G. Sagué , E. Vetsch , W. Alt , D. Meschede , A. Rauschenbeutel

Collective off resonant scattering of coherent light by a cold gas induces long-range interactions via interference of light scattered by different particles. In a 1D configuration these interactions grow particularly strong for particles…

量子物理 · 物理学 2015-06-15 Tobias Grießer , Helmut Ritsch

We investigate theoretically the molecular yield in photoassociation of Bose-Einstein condensed sodium atoms for light intensities of the order of and above those applied in a recent experiment. Our results show that the rate at which…

其他凝聚态物理 · 物理学 2008-09-08 Thomas Gasenzer

We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…

量子气体 · 物理学 2012-05-15 Sebastian D. Huber , Hans Peter Büchler

We discuss the production of ultracold molecules in their electronic ground state by photoassociation employing electronically excited states with ion-pair character and strong spin-orbit interaction. A short photoassociation laser pulse…