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Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…

强关联电子 · 物理学 2009-11-07 Zhi-De Chen , J. -Q. Liang , Shun-Qing Shen

New Mn12 single-molecule magnets (SMM's) with the composition [Mn12O12(O2CR)16(H2O)4] were prepared and structurally characterized. Complexes of this type can exhibit two out-of-phase ac magnetic susceptibility signals, one in the 4-7 K…

We investigate the magnetic properties of three Mn$_6$ single molecule magnets by means of inelastic neutron scattering and frequency domain magnetic resonance spectroscopy. The experimental data reveal that small structural distortions of…

Single-molecule memory device based on a single-molecule magnet (SMM) is one of the ultimate goals of semiconductor nanofabrication technologies. Here, we study how to manipulate and readout the SMM's two spin-state of stored information…

介观与纳米尺度物理 · 物理学 2021-12-28 Hai-Bin Xue , Jiu-Qing Liang , Wu-Ming Liu

We report on the low temperature tunnel magnetoresistance (MR) in quasi one-dimensional (1D) nanofibers made of conjugated polymers. The MR voltage bias dependence reveals an enhancement (at low biases) and the oscillatory behavior at…

统计力学 · 物理学 2009-12-09 H. J. Lee , A. N. Aleshin , S. H. Jhang , H. S. Kim , M. J. Goh , K. Akagi , J. S. Brooks , Y. W. Park

The magnetic state of atomically thin semiconducting layered antiferromagnets such as CrI$_3$ and CrCl$_3$ can be probed by forming tunnel barriers and measuring their resistance as a function of magnetic field ($H$) and temperature ($T$).…

Spectroscopic measurements with low-temperature scanning tunneling microscopes have been used very successfully for studying not only individual atomic or molecular spins on surfaces but also complexly designed coupled systems. The symmetry…

介观与纳米尺度物理 · 物理学 2017-03-28 Markus Ternes

The three essential pillars of magnetic data storage devices are readability, writeability, and stability. However, these requirements compete as magnetic domain sizes reach the fundamental limit of single atoms and molecules. The proven…

A scanning tunneling microscope (STM) can probe the inelastic spin excitations of single magnetic atoms in a surface via spin-flip assisted tunneling. A particular and intriguing case is the Mn dimer case. We show here that the existing…

介观与纳米尺度物理 · 物理学 2022-08-31 F. Delgado , J. Fernández-Rossier

We characterize molecular magnet heterojunctions in which sublimated CoPc films as thin as 5 nm are sandwiched between transparent conducting bottom-layer indium tin oxide and top-layer soft-landing eutectic GaIn (EGaIn) electrodes. The…

We report here low temperature magnetization isotherms for the single molecule magnet, $(UO_2-L)_3$. By analyzing the low temperature magnetization in terms of $M= X_1*B + X_3*B^3$ we extract the linear susceptibility $X_1$ and the leading…

其他凝聚态物理 · 物理学 2017-05-10 B. S. Shivaram , Eric Colineau , Jean-Christophe Griveau , P. Kumar , V. Celli

We report spin-pair tunneling observed in Mn$_3$ single-molecule magnet, which is a crystal with 2D network of identical exchange coupling. We observed a series of extra quantum tunnelings by the ac susceptibility measurements, and…

介观与纳米尺度物理 · 物理学 2014-11-04 Yan-Rong Li , Rui-Yuan Liu , Yun-Ping Wang

Spin-dependent transport through a multilevel quantum dot weakly coupled to ferromagnetic leads is analyzed theoretically by means of the real-time diagrammatic technique. Both the sequential and cotunneling processes are taken into…

介观与纳米尺度物理 · 物理学 2009-11-13 I. Weymann , J. Barnas

We consider quantum transport and tunneling magnetoresistance (TMR) through an interacting quantum dot in the Coulomb blockade regime, attached to ferromagnetic leads. We show that there exist two kinds of anomalies of TMR, which have…

介观与纳米尺度物理 · 物理学 2009-11-13 Piotr Stefanski

We report resistance versus magnetic field measurements for a La0.65Sr0.35MnO3/SrTiO3/La0.65Sr0.35MnO3 tunnel junction grown by molecular-beam epitaxy, that show a large field window of extremely high tunneling magnetoresistance (TMR) at…

介观与纳米尺度物理 · 物理学 2015-05-27 Robert Werner , Alexandr Yu. Petrov , Lucero Alvarez Mino , Reinhold Kleiner , Dieter Koelle , Bruce A. Davidson

We report on magnetoconductance measurements through a weakly coupled quantum dot, containing roughly 900 electrons, in a wide magnetic field range from 0 T to 12 T. We find modulations of the conductance resonances in the quantum Hall…

A three barrier resonant tunneling structure in which the two quantum wells are formed by a dilute magnetic semiconductor material (ZnMnSe) with a giant Zeeman splitting of the conduction band is theoretically investigated. Self-consistent…

介观与纳米尺度物理 · 物理学 2007-05-23 Christian Ertler , Jaroslav Fabian

Controlling electronic transport through a single-molecule junction is crucial for molecular electronics or spintronics. In magnetic molecular devices, the spin degree-of-freedom can be used to this end since the magnetic properties of the…

The nonlinear dynamical response of Mn$_{12}$ single-molecule magnets is experimentally found to be very large, quite insensitive to the spin-lattice coupling constant, and displaying peaks reversed with respect to classical…

介观与纳米尺度物理 · 物理学 2016-08-31 F. Luis , V. Gonzalez , A. Millan , J. L. Garcia-Palacios

Direct evidence of quantum coherence in a single-molecule magnet in frozen solution is reported with coherence times as long as T2 = 630 ns. We can strongly increase the coherence time by modifying the matrix in which the single-molecule…

材料科学 · 物理学 2008-10-28 C. Schlegel , J. van Slageren , M. Manoli , E. K. Brechin , M. Dressel