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A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An…

介观与纳米尺度物理 · 物理学 2007-05-23 D. Galetti , B. M. Pimentel , C. L. Lima , E. C. Silva

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…

介观与纳米尺度物理 · 物理学 2009-11-11 W. Wernsdorfer , N. E. Chakov , G. Christou

High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…

介观与纳米尺度物理 · 物理学 2022-02-17 Sascha Brinker , Felix Küster , Stuart S. P. Parkin , Paolo Sessi , Samir Lounis

Temperature dependence of the tunnel magnetoresistance (TMR) was calculated in range of the quantum-ballistic model in the magnetic tunnel junctions (MTJs) with embedded nanoparticles (NPs). The electron tunnel transport through NP was…

介观与纳米尺度物理 · 物理学 2016-03-28 Arthur Useinov , Chih-Huang Lai

Spin tunneling in molecular magnets has attracted much attention, however theoretical considerations of this phenomenon up to now have not taken into account the many-spin nature of molecular magnets. We present, to our knowledge, the first…

材料科学 · 物理学 2009-10-31 M. Al-Saqer , V. V. Dobrovitski , B. N. Harmon , M. I. Katsnelson

We show that the nuclear spin dynamics in the single-molecule magnet Mn12-ac below 1 K is governed by quantum tunneling fluctuations of the cluster spins, combined with intercluster nuclear spin diffusion. We also obtain the first…

介观与纳米尺度物理 · 物理学 2007-05-23 Andrea Morello , Oleg N. Bakharev , Hans B. Brom , Roberta Sessoli , L. Jos de Jongh

Quantum-well (QW) devices have been extensively investigated in semiconductor structures. More recently, spin-polarized QWs were integrated into magnetic tunnel junctions (MTJs). In this work, we demonstrate the spin-based control of the…

Spin-polarized transport through bistable magnetic adatoms or single-molecule magnets (SMMs), which exhibit both uniaxial and transverse magnetic anisotropy, is considered theoretically. The main focus is on the impact of transverse…

介观与纳米尺度物理 · 物理学 2014-07-22 Maciej Misiorny , Józef Barnaś

Magnetization measurements of a molecular clusters Mn12 with a spin ground state of S = 10 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field…

介观与纳米尺度物理 · 物理学 2009-11-07 W. Wernsdorfer , M. Soler , G. Christou , D. N. Hendrickson

A comprehensive study of a force detected single-spin magnetic resonance measurement concept with atomic spatial resolution is presented. The method is based upon electrostatic force detection of spin-selection rule controlled…

介观与纳米尺度物理 · 物理学 2015-06-11 A. Payne , K. Ambal , C. Boehme , C. C. Williams

Quantum tunneling of the magnetization is a phenomenon that impedes the use of small anisotropic spin systems for storage purposes even at the lowest temperatures. Phonons, usually considered for temperature dependent relaxation of…

强关联电子 · 物理学 2021-04-07 K. Irländer , H. -J. Schmidt , J. Schnack

We investigate single molecule magnet transistors (SMMTs) with ligands that support transport resonances. We find the lowest unoccupied molecular orbitals of Mn12-benzoate SMMs (with and without thiol or methyl-sulfide termination) to be on…

介观与纳米尺度物理 · 物理学 2011-11-23 Fatemeh Rostamzadeh Renani , George Kirczenow

We study low temperature resonant spin tunneling in molecular magnets induced by a field sweep with account of dipole-dipole interactions. Numerical simulations uncovered formation of self-organized patterns of the magnetization and of the…

统计力学 · 物理学 2012-02-21 D. A. Garanin , E. M. Chudnovsky

The Landau Zener model has recently been used to measure very small tunnel splittings in molecular clusters of Fe8, which at low temperature behaves like a nanomagnet with a spin ground state of S = 10. The observed oscillations of the…

介观与纳米尺度物理 · 物理学 2009-10-31 W. Wernsdorfer , I. Chiorescu , R. Sessoli , D. Gatteschi , D. Mailly

Magnetic hysteresis has become a crucial aspect for characterizing single-molecule magnets, but the comprehension of the coercivity mechanism is still a challenge. By using analytical derivation and quantum dynamical simulations, we reveal…

材料科学 · 物理学 2023-09-08 Lei Gu , Qiancheng Luo , Guoping Zhao , Yan-Zhen Zheng , Ruqian Wu

In high spin molecules metal ions are coupled by ferro or antiferromagnetic short range interactions so that their magnetic moments are parallel or antiparallel to each other at temperatures (T) much smaller than the coupling constant J.…

凝聚态物理 · 物理学 2009-09-25 A. Keren , P. Mendels , A. Kratzer , A. Scuiller , M. Verdaguer , Z. Slaman , C. Baines

Single molecular magnet (SMM) like paramagnetic molecules interacting with the ferromagnetic electrodes of a magnetic tunnel junction (MTJ) produce a new system that differs dramatically from the properties of isolated molecules and…

材料科学 · 物理学 2021-05-26 Andrew Grizzle , Christopher DAngelo , Pawan Tyagi

We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic…

统计力学 · 物理学 2007-05-23 J. F. Fernandez , J. J. Alonso

Spin-resolved electron symmetry filtering is a key mechanism behind giant tunneling magnetoresistance (TMR) in Fe/MgO/Fe and similar magnetic tunnel junctions (MTJs), providing room temperature functionality in modern spin electronics.…

介观与纳米尺度物理 · 物理学 2021-10-12 César González-Ruano , Coriolan Tiusan , Michel Hehn , Farkhad G. Aliev

Single-molecule magnets (SMMs) are promising elements for quantum informatics. In the presence of strong magnetic anisotropy, they exhibit magnetization blocking - a magnetic memory effect at the level of a single molecule. Recent studies…