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We report on atom probe tomography analyses of Pd and Pd@Au nanoparticles embedded in a Ni matrix and the effects of local evaporation field variations on the atom probe data. In order to assess the integrity of the reconstructed atom maps,…

Low energy electron diffraction (LEED), scanning tunneling microscopy (STM), and photoelectron spectroscopy have been used to study an ordered structure formed by Ge atoms deposited onto the Au(111) surface. Based on a careful analysis of…

材料科学 · 物理学 2018-01-03 W. Wang , R. I. G. Uhrberg

We report a study of structural and electronic properties of a germanium layer on Al(111) using scanning tunneling microscopy (STM), low energy electron diffraction and core-level photoelectron spectroscopy. Experimental results show that a…

材料科学 · 物理学 2017-12-08 W. Wang , R. I. G. Uhrberg

The electronic structure of Au-Sn intermetallic layers of different compositions grown on Au(111) to the thickness of several nanometers has been studied in this work. The layer, interface and the substrate related components in the Au 4$f$…

We report on the structure and adsorption properties of Pd$_n$ ($n=1-4$) clusters supported on the rutile TiO$_2$ (110) surfaces with the possible presence of a surface oxygen vacancy or a subsurface Ti-interstitial atom. As predicted by…

材料科学 · 物理学 2012-04-12 Jin Zhang , Anastassia N. Alexandrova

The morphology of epitaxial structures formed in solidification of liquid Au films on the Au(110) surface was studied by molecular dynamics simulation based on a many--body interatomic potential. The (1x2) reconstructed and smooth phase at…

mtrl-th · 物理学 2009-10-28 G. Bilalbegovic

We apply Density Functional Theory (DFT) and the DFT+U technique to study the adsorption of transition metal porphine molecules on atomistically flat Au(111) surfaces. DFT calculations using the Perdew-Burke-Ernzerhof (PBE) exchange…

We have investigated the atomic and electronic structure of the ($\sqrt{3}\times \sqrt{3}$)$R30^{\circ}$ SnAu$_2$/Au(111) surface alloy. Low energy electron diffraction and scanning tunneling microscopy measurements show that the native…

Stable organic radicals serve as model systems for investigating metal-free magnetic phenomena at (sub)nanometer length scales. We have investigated at the single-molecule level the stable $\pi$-radical 2,2-diphenyl-1-picrylhydrazyl (DPPH)…

仪器与探测器 · 物理学 2021-01-13 Radovan Vranik , Vitalii Stetsovych , Simon Feigl , Stefan Müllegger

The self-assembly of submonolayer amounts of Au on the densely stepped Si(553) surface creates an array of closely spaced \atomic wires" separated by 1.5 nm. At low temperature, charge transfer between the terraces and the row of silicon…

介观与纳米尺度物理 · 物理学 2020-01-15 B. Hafke , C. Brand , T. Witte , B. Sothmann , M. Horn-von Hoegen , S. C. Erwin

Growth of atomic indium chains - 1D islands - on the Si(100)-2x1 surface was observed by scanning tunneling microscopy (STM) at room temperature and simulated by means of a kinetic Monte Carlo method. Density of indium islands and island…

材料科学 · 物理学 2015-05-13 Jakub Javorský , Martin Setvín , Ivan Ošt'ádal , Pavel Sobotík , Miroslav Kotrla

Hetero-epitaxial growth on a strain-relief vicinal patterned substrate has revealed unprecedented 2D long range ordered growth of uniform cobalt nanostructures. The morphology of a Co sub-monolayer deposit on a Au(111) reconstructed vicinal…

On-surface metal-organic coordination provides a promising way for synthesizing different two-dimensional lattice structures that have been predicted to possess exotic electronic properties. Using scanning tunneling microscopy (STM) and…

材料科学 · 物理学 2019-10-04 Linghao Yan , Ilona Pohjavirta , Benjamin Alldritt , Peter Liljeroth

We use in situ transmission electron microscopy with automated tracking to study supported gold nanoparticles (NPs) during high-temperature vacuum annealing. \rev{The average mass loss per NP is governed by a flat, nearly size-independent…

We present the growth morphology, the long range ordering, and the evolution of the valence band electronic states of ultra-thin films of copper phthalocyanine (CuPc) deposited on the Au(110)-(1x2) reconstructed surface, as a function of…

材料科学 · 物理学 2009-11-10 F. Evangelista , A. Ruocco , V. Corradini , M. P. Donzello , C. Mariani , M. G. Betti

In our earlier study of Ag island coarsening on Ag(111) surface using kinetic Monte Carlo (KMC) simulations we found that during early stages coarsening proceeds as a sequence of selected island sizes resulting in peaks and valleys in the…

材料科学 · 物理学 2014-04-22 Giridhar Nandipati , Abdelkader Kara , Syed Islamuddin Shah , Talat S. Rahman

Surface reconstructions of Au film on Pd(110) substrate are studied using a local Einstein approximation to quasiharmonic theory with the Sutton-Chen interatomic potential. Temperature dependent surface free energies for different coverages…

凝聚态物理 · 物理学 2009-10-28 J. A. Nieminen

Using scanning tunneling microscopy and spectroscopy, we demonstrate that the adsorption of a minute amount of Cs on a Pb mesa grown in the quantum regime can induce dramatic morphological changes of the mesa, characterized by the…

We identify the atomic structure of the Au/Si(111)-5x2 surface by using density functional theory calculations. With seven Au atoms per unit cell, our model forms a bona fide 5x2 atomic structure, which is energetically favored over the…

材料科学 · 物理学 2014-08-20 Se Gab Kwon , Myung Ho Kang

In situ low-energy electron microscopy was used to study interlayer mass transport kinetics during annealing of three-dimensional (3D) TiN(111) mounds, consisting of stacked 2D islands, at temperatures T between 1550 and 1700 K. At each T,…

材料科学 · 物理学 2009-11-10 S. Kodambaka , Navot Israeli , J. Bareno , W. Swiech , Kenji Ohmori , I. Petrov , J. E. Greene