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Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

强关联电子 · 物理学 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

We analyse the scattering operator associated with the defocusing nonlinear Schr{\"o}dinger equation which captures the evolution of solutions over an infinite time-interval under the nonlinear flow of this equation. The asymptotic nature…

偏微分方程分析 · 数学 2026-04-08 Rémi Carles , Georg Maierhofer

Resonant inelastic x-ray scattering (RIXS) has become a powerful tool in the study of the electronic structure of condensed matter. Although the linewidths of many RIXS features are narrow, the experimental broadening can often hamper the…

强关联电子 · 物理学 2012-02-13 J. Laverock , A. R. H. Preston , D. Newby , K. E. Smith , S. B. Dugdale

High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4. In combination with linear dichroism X-ray absorption spectroscopy, the ruthenium…

We report resonant inelastic x-ray scattering (RIXS) excited by circularly polarized x-rays on Mn-Zn ferrite at the Mn L2,3-resonances. We demonstrate that crystal field excitations, as expected for localized systems, dominate the RIXS…

材料科学 · 物理学 2012-01-04 M. Magnuson , L. -C. Duda , S. M. Butorin , P. Kuiper , J. Nordgren

Angle-resolved soft x-ray measurements made at the boron K-edge in single crystal MgB2 provide new insights into the B-2p local partial density of both unoccupied and occupied band states. The strong variation of absorption with incident…

We describe how improvements in methodology and instrumentation for meV-resolved inelastic x-ray scattering (IXS), coupled with a fresh examination of older theory, allow identification of interaction between the quasi-elastic and acoustic…

软凝聚态物质 · 物理学 2022-05-18 Alfred Q. R. Baron , Daisuke Ishikawa

Resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge is a possible tool to detect charge excitations in cuprate superconductors. We theoretically investigate the possibility for observing a collective charge excitation by the…

强关联电子 · 物理学 2015-08-03 Takami Tohyama , Kenji Tsutsui , Michiyasu Mori , Shigetoshi Sota , Seiji Yunoki

A two-dimensional resonant inelastic x-ray scattering (2D-RIXS) microscopy system has been developed at the beamline BL02U of NanoTerasu. The instrument combines a Wolter type-I mirror for spatial imaging with a varied-line-spacing grating…

材料科学 · 物理学 2026-05-07 Kohei Yamamoto , Hakuto Suzuki , Jun Miyawaki

We present an ab initio theory of core- and valence resonant inelastic x-ray scattering (RIXS) based on a real-space multiple scattering Green's function formalism and a quasi-boson model Hamiltonian. Simplifying assumptions are made which…

材料科学 · 物理学 2011-01-25 J. J. Kas , J. J. Rehr , J. A. Soininen , P. Glatzel

A new method is presented for describing vibrational effects in x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using a combination of the classical Franck-Condon (FC) approximation and classical…

材料科学 · 物理学 2017-12-20 Mathias P. Ljungberg

The use of inelastic x-ray scattering (IXS) to investigate phonons and phonon dispersion in crystals opens the field of phonon spectroscopy, allowing measurements on tiny samples: micrograms of material, or single crystals ~10 to 100 micron…

材料科学 · 物理学 2009-11-02 Alfred Q. R. Baron

Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitations of these materials hold great promise for understanding and…

强关联电子 · 物理学 2019-04-02 Y. Cao , D. G. Mazzone , D. Meyers , J. P. Hill , X. Liu , S. Wall , M. P. M. Dean

The (electromagnetic or weak) current operator responsible for deep inelastic scattering (DIS) should be local and satisfy the well-known commutation relations with the representation operators of the Poincare group. The problem whether…

高能物理 - 唯象学 · 物理学 2007-05-23 Felix M. Lev

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

材料科学 · 物理学 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

强关联电子 · 物理学 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

化学物理 · 物理学 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

We provide a semiquantitative explanation of a recent experiment on the resonant inelastic x-ray scattering (RIXS) in insulating cuprate La2CuO4 (Y.J. Kim et al., Phys. Rev. Lett. 89, 177003 (2002).). We show theoretically that there are…

强关联电子 · 物理学 2009-11-10 Takuji Nomura , Jun-ichi Igarashi

Resonant (elastic) soft x-ray scattering (RSXS) offers a unique element, site, and valence specific probe to study spatial modulations of charge, spin, and orbital degrees of freedom in solids on the nanoscopic length scale. It cannot only…

材料科学 · 物理学 2013-04-12 J. Fink , E. Schierle , E. Weschke , J. Geck

Measurements of spin excitations are essential for an understanding of spin-mediated pairing for superconductivity; and resonant inelastic X-ray scattering (RIXS) provides a considerable opportunity to probe high-energy spin excitations.…