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Fluorescence microscopy is indispensable in nanoscience and biological sciences. The versatility of labeling target structures with fluorescent dyes permits to visualize structure and function at a subcellular resolution with a wide field…

We report on the resonant coupling between localized surface plasmon resonances (LSPRs) in nanostructured Ag films, and an adsorbed monolayer of Rhodamine 6G dye. Hybridization of the plasmons and molecular excitons creates new coupled…

介观与纳米尺度物理 · 物理学 2015-05-13 N. I. Cade , T. Ritman-Meer , D. Richards

Damping rates of multipolar, localized surface plasmons (SP) of gold and silver nanospheres of radii up to $1000nm$ were found with the tools of classical electrodynamics. The significant increase in damping rates followed by noteworthy…

光学 · 物理学 2012-11-21 Krystyna Kolwas , Anastasiya Derkachova

New type of plasmonic nanoparticles - silver octopods that can be synthesized with a variety of shapes - have been demonstrated to show versatile optical response using the discrete dipole approximation. The octopods show a complex behavior…

介观与纳米尺度物理 · 物理学 2015-05-13 Ivan I. Naumov , Zhiyong Li , Alexander M. Bratkovsky

Photoluminesce (PL) spectroscopy offers excellent methods for mapping the PL decay on the nanosecond time scale. However, capturing maps of emission dynamics on the microsecond time scale can be highly time-consuming. We present a new…

光学 · 物理学 2021-02-24 Jiri Junek , Karel Zidek

Stimulated amplification of fluorescence signals is obtained under conditions which approach biocompatibility by adding NanoParticles (NPs) to an aqueous solution of fluorescein. The conditions for the stability of the suspension and…

生物物理 · 物理学 2023-10-05 S. Bonnefond , J. Cazareth , S. Abelanet , A. Reynaud , M. Vassalli , F. Brau , G. L. Lippi

Collective responses of localized surface plasmon resonances, known as surface lattice resonances (SLRs) in metal nanoparticle arrays, can lead to high quality factors (~100), large local-field enhancements and strong light-matter…

光学 · 物理学 2018-05-23 Mikko J. Huttunen , Payman Rasekh , Robert W. Boyd , Ksenia Dolgaleva

The observation of intense visible fluorescence from silver and iron nanoparticles in different solution phases and surface capping is reported here. Metallic silver and iron nanoparticles were obtained by exploding pure silver and iron…

材料科学 · 物理学 2007-05-23 Abdullah Alqudami , S. Annapoorni

The strong spatial confinement of a nanocavity plasmonic field has made it possible to visualize the inner structure of a single molecule and even to distinguish its vibrational modes in real space. With such ever-improved spatial…

The spontaneous fluorescence rates of single-molecule emitters are typically on the order of nanoseconds. However coupling them with plasmonic nanostructures can substantially increase their fluorescence yields. The confinement between the…

介观与纳米尺度物理 · 物理学 2024-02-01 Jiří Doležal , Amandeep Sagwal , Rodrigo Cezar de Campos Ferreira , Martin Švec

We demonstrated remote plasmonic enhancement (RPE) by a dense random array of Ag nanoislands (AgNIs) that were partially gold-alloyed and attached with column-structured silica (CSS) overlayer of more than 100 nm in thickness. The physical…

This article reviews the new developments in Tip-enhanced Raman scattering (TERS). The fundamental mechanisms underlying the Raman enhancement are discussed, including the role of the plasmonic character of the metallic tips, the nature of…

化学物理 · 物理学 2008-04-01 Catalin C. Neacsu , Samuel Berweger , Markus B. Raschke

The interest of micro and tip-enhanced Raman spectroscopy to analyze nanosized and nanostructured materials, chiefly semiconductors, oxides and pristine or functionalized carbon nanotubes, is reviewed at the light of the contributions to…

材料科学 · 物理学 2007-06-07 Philippe Colomban , Gwénael Gouadec

Microscopic pyramidal pits in a reflective surface, a geometry similar to a retroreflector, are frequently used to enhance signal strength. The enhancement effect is generally attributed to surface plasmons, however, the sub-wavelength to…

光学 · 物理学 2009-12-18 M. Mechler , S. V. Kukhlevsky , A. Mechler , D. McNaughton

Often only small amounts of sample are available for spectroscopic analytical determinations. This work investigates the enhancement of signal in columns packed with silica particles. We propose that silica particles cause the light to…

光学 · 物理学 2024-11-20 Nathan A. Giauque , Callum E. Flowerday , Steven R. Goates

Raman scattering experiments from silver nanocrystals embedded in films of amorphous silica are reported. In addition to the low-frequency peak due to vibrational quadrupolar modes, a broadband is observed in the high-frequency range, with…

凝聚态物理 · 物理学 2007-05-23 H. Portales , E. Duval , L. Saviot , M. Fujii , M. Sumitomo , S. Hayashi

Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour…

Surface plasmon polaritons (SPPs) are locally excited at silver surfaces using (~100) nm-sized nanodiamonds (NDs) with multiple nitrogen-vacancy (NV) centers (~400). The fluorescence from an externally illuminated (at 532 nm) ND and from…

介观与纳米尺度物理 · 物理学 2016-09-16 Cesar E. Garcia-Ortiz , Shailesh Kumar , Sergey I. Bozhevolnyi

Atomically thin boron nitride (BN) nanosheets have been found an excellent substrate for noble metal particles enabled surface enhanced Raman spectroscopy (SERS), thanks to their good adsorption of aromatic molecules, high thermal stability…

材料科学 · 物理学 2015-03-13 Qiran Cai , Lu Hua Li , Yuanlie Yu , Yun Liu , Shaoming Huang , Ying Chen , Kenji Watanabe , Takashi Taniguchi

We propose and theoretically analyze a new vibrational spectroscopy, termed electron- and light-induced stimulated Raman (ELISR) scattering, that combines the high spatial resolution of electron microscopy with the molecular sensitivity of…

光学 · 物理学 2020-08-12 Amr A. E. Saleh , Daniel K. Angell , Jennifer A. Dionne