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The construction of accurate interatomic potentials, and related fields of forces, from equilibrium conformational distributions of molecules is a crucial step in coarse-grained modeling. In this work we show that in order to develop…

软凝聚态物质 · 物理学 2025-04-18 J. M. Hall , M. G. Guenza

The magnetic properties of a system of coexisting localized spins and conduction electrons are investigated within an extended version of the one dimensional Kondo lattice model in which effects stemming from the electron-lattice and…

强关联电子 · 物理学 2009-11-10 M. Gulacsi , A. Bussmann-Holder , A. R. Bishop

The local approach to computing electrostatic interactions proposed by Maggs and adapted by Pasichnyk for molecular dynamics simulations is extended to situations where the dielectric background medium is inhomogeneous. We furthermore…

计算物理 · 物理学 2014-12-10 Florian Fahrenberger , Christian Holm

Molecular design requires systematic and broadly applicable methods to extract structure-property relationships. The focus of this study is on learning thermodynamic properties from molecular-liquid simulations. The methodology relies on an…

材料科学 · 物理学 2023-07-04 Bernadette Mohr , Diego van der Mast , Tristan Bereau

A model for the adsorption of a binary mixture on a one-dimensional infinite lattice with nearest neighbour cooperative effects is considered. The particles of the two species are both monomers but differ in the repulsive interaction…

统计力学 · 物理学 2010-04-20 A. Prados , J. J. Brey

Graph neural networks (GNNs) demonstrate great performance in compound property and activity prediction due to their capability to efficiently learn complex molecular graph structures. However, two main limitations persist including…

生物大分子 · 定量生物学 2023-10-10 Apakorn Kengkanna , Masahito Ohue

A rigourous Monte Carlo method for protein folding simulation on lattice model is introduced. We show that a parameter which can be seen as the rigidity of the conformations has to be introduced in order to satisfy the detailed balance…

软凝聚态物质 · 物理学 2007-05-23 Olivier Collet

Coarse-grained molecular dynamics (CGMD) is a technique developed as a concurrent multiscale model that couples conventional molecular dynamics (MD) to a more coarse-grained description of the periphery. The coarse-grained regions are…

材料科学 · 物理学 2009-11-11 Robert E. Rudd , Jeremy Q. Broughton

Significant efforts have been devoted in the last decade towards improving the predictivity of coarse-grained models in molecular dynamics simulations and providing a rigorous justification of their use, through a combination of theoretical…

化学物理 · 物理学 2019-01-16 Nicodemo Di Pasquale , Thomas Hudson , Matteo Icardi

We report on the development of an original mesoscopic lattice model to predict structural, dynamical and capacitive properties of carbon-carbon supercapacitors. The model uses input from molecular simulations, such as free energy profiles…

材料科学 · 物理学 2019-10-08 Anouar Belhboub , El Hassane Lahrar , Patrice Simon , Celine Merlet

Molecular dynamics (MD) simulations provide detailed insight into atomic-scale mechanisms but are inherently restricted to small spatio-temporal scales. Coarse-grained molecular dynamics (CGMD) techniques allow simulations of much larger…

计算物理 · 物理学 2025-02-10 Yangshuai Wang , Gabor Csanyi , Christoph Ortner

Most experiments can only detect a set of coarse-grained clusters of a molecular system, while the internal microstates are often inaccessible. Here, based on an infinitely long coarse-grained trajectory, we obtain a set of sufficient…

统计力学 · 物理学 2024-12-16 Bingjie Wu , Chen Jia

We study a two species fermion mixture with different populations on a square lattice modeled by a Hubbard Hamiltonian with on-site inter-species repulsive interaction. Such a model can be realized in a cold atom system with fermionic atoms…

强关联电子 · 物理学 2013-02-25 Chen-Yen Lai , Chuntai Shi , Shan-Wen Tsai

The properties of polymer liquids on hard and soft substrates are investigated by molecular dynamics simulation of a coarse-grained bead-spring model and dynamic single-chain-in-mean-field (SCMF) simulations of a soft, coarse-grained…

软凝聚态物质 · 物理学 2015-05-18 F. Léonforte , J. Servantie , C. Pastorino , M. Müller

Kinetically-constrained models are lattice-gas models that are used for describing glassy systems. By construction, their equilibrium state is trivial and there are no equal-time correlations between the occupancy of different sites. We…

统计力学 · 物理学 2017-03-01 Eial Teomy , Yair Shokef

We focus here on the thermodynamic properties of adsorbates formed by two-species $A+B \to \oslash$ reactions on a one-dimensional infinite lattice with heterogeneous "catalytic" properties. In our model hard-core $A$ and $B$ particles…

统计力学 · 物理学 2020-09-17 Dmytro Shapoval , Maxym Dudka , Olivier Bénichou , Gleb Oshanin

Bottom-up coarse-grained molecular dynamics models are parameterized using complex effective Hamiltonians. These models are typically optimized to approximate high dimensional data from atomistic simulations. In contrast, human validation…

化学物理 · 物理学 2021-09-16 Aleksander Evren Paetzold Durumeric , Gregory A. Voth

We discuss recent theoretical developments in the study of simple lattice models of proteins. Such models are designed to understand general features of protein structures and mechanism of folding. Among the topics covered are (i) the use…

软凝聚态物质 · 物理学 2007-05-23 D. Thirumalai , D. K. Klimov

We introduce and implement a Monte Carlo scheme to study the equilibrium statistics of polymers in the globular phase. It is based on a model of "interacting elastic lattice polymers" and allows a sufficiently good sampling of long and…

统计力学 · 物理学 2014-06-25 M. Baiesi , E. Orlandini

Molecular Representation Learning (MRL) has proven impactful in numerous biochemical applications such as drug discovery and enzyme design. While Graph Neural Networks (GNNs) are effective at learning molecular representations from a 2D…

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