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Density-functional-theory (DFT) calculations have been performed on the Li-Si and Li-Ge systems. Lithiated Si and Ge, including their metastable phases, play an important technological r\^ole as Li-ion battery (LIB) anodes. The calculations…

材料科学 · 物理学 2015-06-18 Andrew J. Morris , C. P. Grey , C. J Pickard

The optical and electronic properties of crystalline Li2TeO3, which is a tellurite glass, is studied in the framework of density functional theory (DFT) implemented software SIESTA. The material has monoclinic symmetrized structure and the…

材料科学 · 物理学 2021-08-04 Aditya Dey

In the present work, we study the structural, electronic and optical properties of Sodium Based Cubic Fluoro-perovskites: NaBF$_3$ (B= Ca, Mg or Zn) using DFT and TDDFT methods. We performed the density functional theory DFT calculations…

材料科学 · 物理学 2024-08-20 S. Idrissi , A. Jabar , H. Labrim , L. Bahmad , S. Benyoussef

In contrast to the original Kohn-Sham (KS) formalism, we propose a density functional theory (DFT) with fractional orbital occupations for the study of ground states of many-electron systems, wherein strong static correlation is shown to be…

化学物理 · 物理学 2015-06-03 Jeng-Da Chai

Effects of the structural distortion associated with the $\rm OsO_6$ octahedral rotation and tilting on the electronic band structure and magnetic anisotropy energy for the $5d^3$ compound NaOsO$_3$ are investigated using the density…

强关联电子 · 物理学 2018-05-02 Shubhajyoti Mohapatra , Churna Bhandari , Sashi Satpathy , Avinash Singh

Accurately modeling the electronic structure of materials is a persistent challenge to high-throughput screening. A promising means of balancing accuracy against computational cost are non-self-consistent calculations with hybrid…

材料科学 · 物理学 2020-05-04 Jonathan M. Skelton , David S. D. Gunn , Sebastian Metz , Stephen C. Parker

In this work, the electronic and optical properties of a Nitrogen (N) or a Boron (B) doped BeO monolayer are investigated in the framework of density functional theory. It is known that the band gap of a BeO monolayer is large leading to…

X-ray absorption fine-structure (XAFS) measurements supported by {\em ab initio} computations within the density functional theory (DFT) are employed to systematically characterize Fe-doped as well as Fe and Si-co-doped films grown by…

We present a first-principles investigation of structural, electronic and optical properties of bulk crystalline Ag3N, AgN and AgN2 based on density functional theory (DFT) and many-body perturbation theory. The equation of state (EOS),…

材料科学 · 物理学 2015-09-15 Mohammed S. H. Suleiman , Daniel P. Joubert

Density functional theory (DFT) is an essential building block for modern theoretical physics, chemistry, and engineering, especially those concerning electronic properties. Through decades of development, various program packages for…

材料科学 · 物理学 2022-11-21 Yusuke Nomura , Ryosuke Akashi

The atomic structure, energy of formation, and electronic states of vacancies in H-passivated Ge nanocrystals are studied by density functional theory (DFT) methods. The competition between quantum self-purification and the free surface…

材料科学 · 物理学 2015-05-19 Kenneth Bayus , O. Paz , S. P. Beckman

The exploring and understanding the electronic properties of molecules connected to metallic leads is a vital part of nanoscience if molecule is to have a future. This thesis documents a study for various families of organic and…

计算物理 · 物理学 2016-12-13 Oday A. Al-Owaedi

The electronic energy gap and total dipole moment of chemically functionalized hexagonal and triangular graphene quantum dots are investigated by the density functional theory. It has been found that the energy gap can be efficiently tuned…

介观与纳米尺度物理 · 物理学 2018-03-14 Hazem Abdelsalam , Hanan Elhaes , Medhat A. Ibrahim

We present a Density Functional Theory (DFT) study of the structural and electronic properties of bare rutile VO$_{2}$(110) surfaces and its oxygen-rich terminations. We discuss the performance of various DFT functionals, including PBE,…

材料科学 · 物理学 2021-08-31 Jakub Planer , Florian Mittendorfer , Josef Redinger

First-principles simulations of electronic properties of hybrid inorganic/organic interfaces are challenging, as common density-functional theory (DFT) approximations target specific material classes like bulk semiconductors or gas-phase…

材料科学 · 物理学 2023-02-13 Jannis Krumland , Caterina Cocchi

The electronic properties of chemically functionalized nanodiamonds are studied using density functional theory calculations. HOMO-LUMO gap and relative stabilities are calculated for different surface functionalization schemes and diamond…

材料科学 · 物理学 2014-03-26 Noam Brown , Oded Hod

The self consistent version of the density functional theory (DFT) is presented, which allows to calculate the ground state and dynamic properties of finite multi-electron systems such as atoms, molecules and clusters. The exact functional…

凝聚态物理 · 物理学 2007-05-23 M. Ya. Amusia , V. R. Shaginyan

We study the electronic properties of the $\textrm{Fe}\textrm{Se}_{1-x}\textrm{Te}_x$ system ($x=0$, 0.25, 0.5, 0.75, and 1) from the perspective of X-ray spectroscopy and density functional theory (DFT). The analysis performed on the…

超导电性 · 物理学 2014-11-10 I. Perez , J. A. Mcleod , R. J. Green , R. Escamilla , V. Ortiz , A. Moewes

The electronic structure of high-quality van der Waals NiPS$_3$ crystals was studied using near-edge x-ray absorption spectroscopy (NEXAFS) and resonant photoelectron spectroscopy (ResPES) in combination with density functional theory (DFT)…

The exciton binding energy, the energy required to dissociate an excited electron-hole pair into free charge carriers, is one of the key factors to the optoelectronic performance of organic materials. However, it remains unclear whether…

化学物理 · 物理学 2015-12-08 Jui-Che Lee , Jeng-Da Chai , Shiang-Tai Lin