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The effect of film morphology on its surface chemistry and band structure has been analyzed for gallium nitride epitaxial films grown by molecular beam epitaxy. The film morphology has been studied using scanning electron microscopy and…

材料科学 · 物理学 2018-01-09 Abhijit Chatterjee , S. P. Swathi , S. M. Shivaprasad

Water-soluble sacrificial layers based on epitaxially-grown, single crystalline (Ca, Sr, Ba)3Al2O6 layer are widely used for creating free-standing perovskite oxide membranes. However, obtaining these sacrificial layers with intricate…

材料科学 · 物理学 2024-05-20 Shivasheesh Varshney , Martí Ramis , Sooho Choo , Mariona Coll , Bharat Jalan

We present a first-principles study of electronic and magnetic properties of thin Co films on a BaTiO$_3$(001) single crystal. The crystalline structure of 1, 2, and 3 monolayer thick Co films was determined and served as input for…

Epitaxial single-crystalline CsPbBr3 perovskite films on mica, prepared ex-situ, are explored using a low-temperature scanning tunneling microscope (STM) by probing the unoccupied electronic states of their surface in ultra-high vacuum…

材料科学 · 物理学 2026-02-20 Eric Duverger , Vladimir Bruevich , Vitaly Podzorov , Damien Riedel

We present our study of (0001) oriented Mn$_3$Sn (c-Mn$_3$Sn) thin films synthesized directly on an MgO (111) substrate via molecular beam epitaxy. We identify a growth window where Mn$_3$Sn growth can be controlled through slight…

The topographic and electronic structure of cleaved SrTiO3(001) surfaces were studied, employing samples that either had or had not been coated with Ti on their outer surfaces prior to fracture. In both cases, SrO- and TiO2-terminated…

材料科学 · 物理学 2015-09-16 Wattaka Sitaputra , Marek Skowronski , Randall M. Feenstra

Ultrathin films of Na3Bi on insulating substrates are desired for opening a bulk band gap and generating the quantum spin Hall effect from a topological Dirac semimetal, though continuous films in the few nanometer regime have been…

In present study, Tetragonal Mn$_3$O$_4$ thin films of different coating layers of 2, 4, 6, 8, and 10 were prepared on the microscopic glass slides by the spin-coating method. X-ray diffraction, Raman spectroscopy, and ultra-violet visible…

应用物理 · 物理学 2023-08-13 Vidit Pandey , Mohd Salman Siddiqui , Sandeep Munjal , Tufail Ahmad

Bi$_2$Se$_3$ is a widely studied 3D topological insulator having potential applications in optics, electronics, and spintronics. When the thickness of these films decrease to less than approximately 6 nm, the top and bottom surface states…

材料科学 · 物理学 2024-06-19 Saadia Nasir , Walter J. Smith , Thomas E. Beechem , Stephanie Law

Thin film synthesis methods developed over the past decades have unlocked emergent interface properties ranging from conductivity to ferroelectricity. However, our attempts to exercise precise control over interfaces are constrained by a…

材料科学 · 物理学 2017-11-15 Steven R. Spurgeon , Peter V. Sushko , Ryan B. Comes , Scott A. Chambers

A structural transition in an ABO$_{3}$ perovskite thin film involving the change of the BO$_{6}$ octahedral rotation pattern can be hidden under the global lattice symmetry imposed by the substrate and often easily overlooked. We carried…

强关联电子 · 物理学 2019-11-04 W. T. Jin , H. Gretarsson , S. Y. Jang , Chang-Yong Kim , T. W. Noh , Young-june Kim

We have investigated how the recently-developed water-leaching method for atomically-flat SrTiO3 (STO) substrates affects the transport properties of LaAlO3 (LAO) and STO heterointerfaces. Using pulsed laser deposition at identical growth…

材料科学 · 物理学 2016-04-04 J. G. Connell , J. Nichols , J. H. Gruenewald , D. -W. Kim , S. S. A. Seo

We model the remarkable thin-film Ba-Ti-O structures formed by heat treatment of an initial perovskite BaTiO$_3$ thin film on a Pt(111) surface. All structures contain a rumpled Ti-O network with all Ti threefold coordinated with O, and…

材料科学 · 物理学 2016-01-13 Eric Cockayne , Marek Mihalkovic , Christopher L. Henley

The recent emergence of topological insulators (TI) has spurred intensive efforts to grow TI thin films on various substrates. However, little is known about how robust the topological surface states (TSS) are against disorders and other…

We report the formation and observation of an electron liquid in Sr$_{2-x}$La$_{x}$TiO$_4$, the quasi-two-dimensional counterpart of SrTiO$_3$, through reactive molecular-beam epitaxy and {\it in situ} angle-resolved photoemission…

强关联电子 · 物理学 2015-09-01 Y. F. Nie , D. Di Sante , S. Chatterjee , P. D. C. King , M. Uchida , S. Ciuchi , D. G. Schlom , K. M. Shen

The influence of oxygen stoichiometry on the uranium local environment is explored in epitaxial single crystal uranium oxide thin films grown by DC magnetron sputtering. Through post-growth annealing, the stoichiometry of as-grown UO$_{2}$…

We report comprehensive x-ray diffraction studies of the crystal structure and epitaxy of thin films of the topological insulator Bi2Te3 grown on Si (1 1 1). The films are single crystals of high crystalline quality, which strongly depends…

材料科学 · 物理学 2012-12-04 Jihwey Park , Yeong-Ah Soh , G. Aeppli , S. R. Bland , Xie-Gang Zhu , Xi Chen , Qi-Kun Xue , Francois Grey

Nowadays it has become feasible to perform angle-resolved photoemission spectroscopy (ARPES) measurements of transition-metal oxides with three-dimensional perovskite structures owing to the availability of high-quality single crystals of…

强关联电子 · 物理学 2007-05-23 H. Wadati , T. Yoshida , A. Chikamatsu , H. Kumigashira , M. Oshima , H. Eisaki , Z. -X. Shen , T. Mizokawa , A. Fujimori

We report on the synthesis of perovskite SrIrO3 thin films using sputtering technique. Single phase (110) oriented SrIrO$_3$ thin films were epitaxially grown on SrTiO3 (001) substrate. Using off-axis XRD $\theta-2\theta$ scans, we…

材料科学 · 物理学 2016-10-14 Z. Z. Li , O. Schneegans , L. Fruchter

Macroscopic properties of materials stem from fundamental atomic-scale details, yet for insulators, resolving surface structures remains a challenge. The basal (0001) plane of ${\alpha}$-Al$_{2}$O$_{3}$ was imaged with noncontact atomic…