原子物理
Molecules with heavy, radioactive nuclei promise extreme sensitivity to fundamental nuclear and particle physics. However, these nuclei are available in limited quantities, which challenges their use in precision measurements. Here we…
The collective interaction of electronic excitations with the electromagnetic field in atomic arrays can lead to reduced decay rates, forming subradiant states with applications in quantum information and memories. By including quantized…
Excluding the very shallow potential minimum of the electronic ground state, all bound electronic states of He$_2$ have Rydberg character. Their potential-energy functions are similar to those of the He$_2^+$ states to which the Rydberg…
RaOCH$_3$ molecule is one of the most sensitive systems for the electron electric dipole moment ($e$EDM) searches. Its hyperfine and $K-$doubling structure in the external electric field is of key importance for preparing and interpreting…
Control of the polarization of microwave fields is a key experimental capability for a number of atomic physics platforms. However, producing high-fidelity microwaves requires a well-controlled microwave environment, where reflections that…
Heavy polar molecules are sensitive probes of physics Beyond the Standard Model. However, uncontrolled external electromagnetic fields pose challenges to achieving precise and accurate measurements. Minimizing susceptibility to these fields…
High-lying Rydberg and autoionizing (AI) states of thorium (Th) have been studied via resonance laser ionization spectroscopy at both TRIUMF Canada's particle accelerator centre and Oak Ridge National Lab (ORNL). Multiple Rydberg series…
The finite operators are derived for the recoil $m\alpha^6(m/M)$ order relativistic corrections (to spin-averaged energy levels) in hydrogen-like atoms and ions in the two- and three-body formalism beyond the adiabatic approximation.…
We present a Rydberg-atom interferometry-based technique for voltage measurement between electrodes embedded in an atomic vapor cell, enabling the detection of weak voltages ($<0.1$V) and unambiguous discrimination between positive and…
Detailed comparisons between theory and experiment for quantum electrodynamics (QED) effects in He-like ions have been performed in the literature to search for hints of new physics. Different frequentist statistical analyses of the…
A soft ferromagnetic plate uniformizes Tesla-level fields generated by attached permanent magnets, producing a smooth and electronically tunable surface field on the opposite side. By arranging $n$ precisely fabricated rectangular plates, a…
Isomerization, i.e. the rearrangement between distinct molecular configurations, is a fundamental process in chemistry. Here we demonstrate that two-dimensional Coulomb crystals can emulate molecular isomerization and be used to…
The relativistic Fock-space coupled-cluster methods are applied to the cadmium atom. A large number of transition energies and matrix elements are calculated for the $5s^{2}\:$$ ^{1}S \to 5snp\: ^{1,3} P^{o}$, $5s6s\: ^{1}S \to 5snp\:…
The simulation of vibrational energy transport and quantum thermodynamics with trapped ions requires good methods for the estimation of temperatures. One valuable tool for this purpose is based on the fit of dark resonances in the…
We calculate the bound-electron $g$ factor for a wide range of rovibrational states of the molecular hydrogen ions H$_2^+$ and HD$^+$. Relativistic and QED corrections of orders up to $\alpha^5$ are taken into account. All contributions are…
Stabilized optical frequency references (OFRs) are indispensable for atom-based quantum technologies, optical communications, and precision metrology. As these systems become more sophisticated, demands for compactness, robustness, and…
This Technical Design Report presents AION-10, a 10-meter atom interferometer to be located at Oxford University using ultracold strontium atoms to make precision measurements of fundamental physics. AION-10 serves as both a prototype for…
The decay of core-excited states is a sensitive probe of autoionization dynamics and correlation effects in many-electron systems, occurring on the fastest timescales. Xenon, with its dense manifold of autoionizing resonances that can be…
A scattering resonance is one of the most striking quantum effects in low-temperature molecular collisions. Predicted decades ago theoretically, they have only been resolved experimentally for systems involving at most four atoms. Extension…
We perform a systematic analysis of intra-channel quantum interference in laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI)…