中文

Diffusion-Limited Aggregation Processes with 3-Particle Elementary Reactions

凝聚态物理 2009-10-22 v1

摘要

A diffusion-limited aggregation process, in which clusters coalesce by means of 3-particle reaction, A+A+A->A, is investigated. In one dimension we give a heuristic argument that predicts logarithmic corrections to the mean-field asymptotic behavior for the concentration of clusters of mass mm at time tt, c(m,t) m1/2(log(t)/t)3/4c(m,t)~m^{-1/2}(log(t)/t)^{3/4}, for 1<<m<<t/log(t)1 << m << \sqrt{t/log(t)}. The total concentration of clusters, c(t)c(t), decays as c(t) log(t)/tc(t)~\sqrt{log(t)/t} at t>t --> \infty. We also investigate the problem with a localized steady source of monomers and find that the steady-state concentration c(r)c(r) scales as r1(log(r))1/2r^{-1}(log(r))^{1/2}, r1r^{-1}, and r1(log(r))1/2r^{-1}(log(r))^{-1/2}, respectively, for the spatial dimension dd equal to 1, 2, and 3. The total number of clusters, N(t)N(t), grows with time as (log(t))3/2(log(t))^{3/2}, t1/2t^{1/2}, and t(log(t))1/2t(log(t))^{-1/2} for dd = 1, 2, and 3. Furthermore, in three dimensions we obtain an asymptotic solution for the steady state cluster-mass distribution: c(m,r)r1(log(r))1Φ(z)c(m,r) \sim r^{-1}(log(r))^{-1}\Phi(z), with the scaling function Φ(z)=z1/2exp(z)\Phi(z)=z^{-1/2}\exp(-z) and the scaling variable z m/log(r)z ~ m/\sqrt{log(r)}.

关键词

引用

@article{arxiv.cond-mat/9403041,
  title  = {Diffusion-Limited Aggregation Processes with 3-Particle Elementary Reactions},
  author = {P. L. Krapivsky},
  journal= {arXiv preprint arXiv:cond-mat/9403041},
  year   = {2009}
}

备注

12 pages, plain TeX