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Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

The rare earth pyrochlore magnet Yb2Ti2O7 is among a handful of materials that apparently exhibit no long range order down to the lowest explored temperatures and well below the Curie-Weiss temperature. Paramagnetic neutron scattering on a…

Statistical Mechanics · Physics 2011-04-11 J. D. Thompson , P. A. McClarty , M. J. P. Gingras

We present an extensive powder and single-crystal neutron scattering investigation of the crystallographic structure and magnetic order of the frustrated metallic $f$-electron magnet UNi$_4$B. We carry out a full refinement of the…

Strongly Correlated Electrons · Physics 2021-06-02 J. Willwater , S. Süllow , M. Reehuis , R. Feyerherm , H. Amitsuka , B. Ouladdiaf , E. Suard , M. Klicpera , M. Vališka , J. Pospíšil , V. Sechovský

The nature of the low temperature ground state of the pyrochlore compound Tb2Ti2O7 remains a puzzling issue. Dynamic fluctuations and short-range correlations persist down to 50 mK, as evidenced by microscopic probes. In parallel,…

Strongly Correlated Electrons · Physics 2012-08-02 E. Lhotel , C. Paulsen , P. Dalmas de Réotier , A. Yaouanc , C. Marin , S. Vanishri

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

The recent determination of a robust spin Hamiltonian for the anti-ferromagnetic XY pyrochlore Er2Ti2O7 reveals a most convincing case of the "order by quantum disorder" (ObQD) mechanism for ground state selection. This mechanism relies on…

Strongly Correlated Electrons · Physics 2014-02-13 K. A. Ross , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

Fully relativistic first-principles electronic structure calculations based on a noncollinear local spin density approximation (LSDA) are performed for pyrochlore iridates Y$_2$Ir$_2$O$_7$ and Pr$_2$Ir$_2$O$_7$. The all-in, all-out…

Strongly Correlated Electrons · Physics 2015-06-22 Fumiyuki Ishii , Yo Pierre Mizuta , Takehiro Kato , Taisuke Ozaki , Hongming Weng , Shigeki Onoda

The consequences of nonmagnetic-ion dilution for the pyrochlore family Y$_{2}$($M_{1-x}N_{x}$)$_{2}$O$_{7}$ ($M$ = magnetic ion, $N$ = nonmagnetic ion) have been investigated. As a first step, we experimentally examine the magnetic…

Strongly Correlated Electrons · Physics 2017-10-04 L. Shen , C. Greaves , R. Riyat , T. C. Hansen , E. Blackburn

We report on the quasi-two-dimensional magnetism of the natural mineral diaboleite Pb2Cu(OH)4Cl2 with a tetragonal crystal structure, which is closely related to that of the frustrated spin-1/2 magnet PbVO3. Magnetic susceptibility of…

Materials Science · Physics 2013-02-15 Alexander A. Tsirlin , Oleg Janson , Stefan Lebernegg , Helge Rosner

The Ho2Ti2O7, Er2Ti2O7 and Yb2Ti2O7 pyrochlores were studied by synchrotron X-ray diffraction to determine whether the (002) peak, forbidden in the pyrochlore space group Fd-3m but observed in single crystal neutron scattering measurements,…

Materials Science · Physics 2015-04-24 Kristen Baroudi , Bruce D. Gaulin , Saul H. Lapidus , R. J. Cava

A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

The classical Heisenberg antiferromagnet on the pyrochlore lattice is macroscopically and continuously degenerate and the system remains disordered at all temperatures, even in the presence of weak dilution with nonmagnetic ions. We show…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Bellier-Castella , M. J. P. Gingras , P. C. W. Holdsworth , R. Moessner

We present a comprehensive experimental and theoretical study of the pyrochlore Tb$_2$Ge$_2$O$_7$, an exemplary realization of a material whose properties are dominated by competition between magnetic dipolar and electric quadrupolar…

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

The magnetic behavior of polycrystalline samples of Er$_2$Ir$_2$O$_7$ and Tb$_2$Ir$_2$O$_7$ pyrochlores is studied by magnetization measurements and neutron diffraction. Both compounds undergo a magnetic transition at 140 and 130 K…

Strongly Correlated Electrons · Physics 2015-07-30 E. Lefrançois , V. Simonet , R. Ballou , E. Lhotel , A. Hadj-Azzem , S. Kodjikian , P. Lejay , P. Manuel , D. Khalyavin , L. C. Chapon

We have studied the hidden long-range order (LRO) of the frustrated pyrochlore magnet Tb$_2$Ti$_2$O$_7$ by means of specific-heat experiments and Monte-Carlo (MC) simulations, which has been discussed as the LRO of quadrupole moments…

Strongly Correlated Electrons · Physics 2016-02-09 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

We report the growth of large high quality crystals of the frustrated magnet, Pr2Zr2O7 by the floating zone technique. Several crystals have been produced starting with varying levels of excess of Pr6O11 to compensate for the loss of Pr2O3…

Materials Science · Physics 2016-11-09 M. Ciomaga Hatnean , C. Decorse , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan

We present neutron diffraction analysis of BaFe$_2$(As$_{1-x}$P$_x$)$_2$ over a wide temperature (10 to 300 K) and compositional ($0.11 \leq x \leq 0.79$) range, including the normal state, the magnetically ordered state, and the…

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin
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