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We report a study of the geometrically frustrated magnetic material Tb2Sn2O7 by the positive muon spin relaxation technique. No signature of a static magnetically ordered state is detected while neutron magnetic reflections are observed in…

Strongly Correlated Electrons · Physics 2009-11-11 P. Dalmas de Reotier , A. Yaouanc , L. Keller , A. Cervellino , B. Roessli , C. Baines , A. Forget , C. Vaju , P. C. M. Gubbens , A. Amato , P. J. C. King

Superconducting and structural phase transitions in a pyrochlore oxide Cd2Re2O7 are studied under high pressure by x-ray diffraction and electrical resistivity measurements. A rich P-T phase diagram is obtained, which contains at least two…

We study the magnetic structure of the "stuffed" (Tb-rich) pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$, using resonant elastic x-ray scattering (REXS). In order to disentangle contributions from Tb and Ir magnetic sublattices,…

We report results of NMR experiments on the ruthenium oxide Hg2Ru2O7 with the pyrochlore structure, which exhibits a metal-insulator transition at TMI = 107 K. In the metallic phase above TMI, the nuclear spin-lattice relaxation rate 1/T1…

Strongly Correlated Electrons · Physics 2017-12-01 Makoto Yoshida , Masashi Takigawa , Ayako Yamamoto , Hidenori Takagi

NaCaNi$_2$F$_7$ is an insulating, frustrated A$_2$B$_2$F$_7$ pyrochlore with magnetic S = 1 Ni$^{2+}$ on the pyrochlore B site. Non-magnetic Na and Ca are disordered on the A-site. Magnetic susceptibility measurements made on an oriented…

Materials Science · Physics 2015-04-30 J. W. Krizan , R. J. Cava

The oxide pyrochlore Bi$_2$Ti$_2$O$_6$O$^\prime$ is known to be associated with large displacements of Bi and O$^\prime$ atoms from their ideal crystallographic positions. Neutron total scattering, analyzed in both reciprocal and real…

Materials Science · Physics 2010-04-19 D. P. Shoemaker , A. L. Hector , C. J. Fennie , A. Llobet , Th. Proffen , R. Seshadri

Electronic properties of the metallic pyrochlore oxide Cd2Re2O7 are studied by means of electrical resistivity and Hall measurements. Semimetallic band structures are revealed as expected from band structure calculations. It is found that…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hiroi , M. Hanawa , Y. Muraoka , H. Harima

Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a prototypical example of the pyrochlore iridates. The density of states, the Fermi surface, and the near Fermi level band dispersion in the plane…

Strongly Correlated Electrons · Physics 2013-11-14 Q. Wang , Y. Cao , X. G. Wan , J. D. Denlinger , T. F. Qi , O. B. Korneta , G. Cao , D. S. Dessau

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

We study the finite-temperature transition in a model XY antiferromagnet on a pyrochlore lattice, which describes the pyrochlore material Er2Ti2O7. The ordered magnetic structure selected by thermal fluctuations is six-fold degenerate.…

Strongly Correlated Electrons · Physics 2014-04-15 M. E. Zhitomirsky , P. C. W. Holdsworth , R. Moessner

Despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K, the Tb2Ti2O7 pyrochlore magnetic material lacks long range magnetic order down to at least $T^*\approx 50$ mK. It has recently been proposed that the low temperature collective…

Statistical Mechanics · Physics 2009-05-07 Hamid R. Molavian , Michel J. P. Gingras

From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…

Statistical Mechanics · Physics 2010-11-30 Paul A. McClarty , Pawel Stasiak , Michel J. P. Gingras

Spin ordering in TbBaCo2O5.5 and its temperature transformation is studied. Polymorphism due to the oxygen ordering with the average content close to 5.5 is investigated. One of ceramic samples (I), in addition to the main phase ap x 2ap x…

Frustrated rare-earth pyrochlore titanates, Yb$_2$Ti$_2$O$_7$, and Tb$_2$Ti$_2$O$_7$ have been proposed as promising candidates to realize quantum spin ice (QSI). Multiple exotic quantum phases, including Coulombic ferromagnet, quantum…

Strongly Correlated Electrons · Physics 2021-01-12 Fangdi Wen , Tsung-Chi Wu , Xiaoran Liu , Michael Terilli , Mikhail Kareev , Jak Chakhalian

Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…

Strongly Correlated Electrons · Physics 2022-04-20 Sheetal , A. Elghandour , R. Klingeler , C. S. Yadav

A detailed study of the structural and magnetic properties of a spin-$5/2$ triangular lattice antiferromagnet RbFe(HPO$_{3}$)$_{2}$ is presented using x-ray diffraction, magnetization, heat capacity, and $^{31}$P nuclear magnetic resonance…

Materials Science · Physics 2025-11-24 V. Nagpal , Sebin J. Sebastian , Surya P. Patra , S. Shibash , Q. -P. Ding , Y. Furukawa , R. Nath

The crystal and magnetic structures and underlying magnetic interactions of Bi4Fe5O13F, a model system for studying the physics of the Cairo pentagonal spin lattice, are investigated by transmission electron microscopy, low-temperature…

The very nature of the ground state of the pyrochlore compound Yb$_2$Ti$_2$O$_7$ is much debated, as experimental results demonstrate evidence for both a disordered or a long-range ordered ground state. Indeed, the delicate balance of…

Strongly Correlated Electrons · Physics 2014-05-13 E. Lhotel , S. R. Giblin , M. R. Lees , G. Balakrishnan , L. J. Chang , Y. Yasui

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

Superconductivity · Physics 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…