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Low temperature magnetic and structural behavior of the extended Kagome system YBaCo4O7 has been studied by single crystal neutron diffraction and high-resolution powder X-ray diffraction. Long-range magnetic ordering associated with a…

Materials Science · Physics 2015-05-19 D. D. Khalyavin , P. Manuel , B. Ouladdiaf , A. Huq , H. Zheng , J. F. Mitchell , L. C. Chapon

We have investigated the effect of synthesis and growth conditions on the magnetic, structural, and compositional properties of pyrochlore oxide holmium titanate and demonstrate a method for growing high quality stoichiometric single…

Materials Science · Physics 2018-09-26 Alireza Ghasemi , Allen Scheie , Jonas Kindervater , Seyed M. Koohpayeh

We have investigated the physical properties of a pyrochlore hafnate Nd2Hf2O7 using ac magnetic susceptibility \chi_ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements, and…

Strongly Correlated Electrons · Physics 2015-12-09 V. K. Anand , A. K. Bera , J. Xu , T. Herrmannsdörfer , C. Ritter , B. Lake

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

Partially-ordered magnets are distinct from both spin liquids and conventional ordered magnets because order and disorder coexist in the same magnetic phase. Here, we determine the nature of partial order in the canonical frustrated…

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

We have investigated the 89Y NMR spectrum and spin lattice relaxation, T1, in the magnetically frustrated pyrochlore Y2Mo2O7. We find that upon cooling the spectrum shifts, and broadens asymmetrically. A detailed examination of the low T…

Strongly Correlated Electrons · Physics 2009-11-07 Amit Keren , Jason S. Gardner

The origin of the spin liquid state in Tb$_2$Ti$_2$O$_7$ has challenged experimentalists and theorists alike for nearly 20 years. To improve our understanding of the exotic magnetism in Tb$_2$Ti$_2$O$_7$, we have synthesized a chemical…

We report the basic thermodynamic properties of the new geometrically frustrated beta-pyrochlore bulk superconductor RbOs2O6 with a critical temperature Tc = 6.4 K. Specific heat measurements are performed in magnetic fields up to 12 T. The…

Superconductivity · Physics 2009-11-10 M. Brühwiler , S. M. Kazakov , N. D. Zhigadlo , J. Karpinski , B. Batlogg

We report magnetization data for several titanium pyrochlore systems measured down to 0.5 K. The measurements, performed on single crystal samples in fields of up to 7 T, have captured the essential elements of the previously reported phase…

Strongly Correlated Electrons · Physics 2014-08-18 O. A. Petrenko , M. R. Lees , G. Balakrishnan

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

Strongly Correlated Electrons · Physics 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville

We report the anisotropic magnetic properties of Ho2Ge2O7 determined from dc and ac magnetization, specific heat and powder neutron diffraction experiments. The magnetic lanthanide sublattice, seen in our refinement of the tetragonal…

Other Condensed Matter · Physics 2009-11-13 E. Morosan , J. A. Fleitman , Q. Huang , J. W. Lynn , Y. Chen , X. Ke , M. L. Dahlberg , P. Schiffer , C. R. Craley , R. J. Cava

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

A single crystal of the Co2+ based pyrochlore NaCaCo2F7 was studied by inelastic neutron scattering. This frustrated magnet with quenched exchange disorder remains in a strongly correlated paramagnetic state down to one 60th of the…

Strongly Correlated Electrons · Physics 2016-02-03 Kate A. Ross , Jason W. Krizan , Jose A. Rodriguez-Rivera , Robert J. Cava , Collin L. Broholm

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

It is shown that both structural phase transitions in Cd2Re2O7, which occur at T_{s1}=200 K and T_{s2}=120 K, are due to an instability of the Re tetrahedral network with respect to the same doubly degenerate long-wavelength phonon mode.…

Superconductivity · Physics 2009-11-10 I. A. Sergienko , S. H. Curnoe

We present time-of-flight inelastic neutron scattering measurements at low temperature on powder samples of the magnetic pyrochlore oxides Tb2Ti2O7 and Tb2Sn2O7. These two materials possess related, but different ground states, with…

Strongly Correlated Electrons · Physics 2014-05-01 J. Zhang , K. Fritsch , Z. Hao , B. V. Bagheri , M. J. P. Gingras , G. E. Granroth , P. Jiramongkolchai , R. J. Cava , B. D. Gaulin

A unique type of frustrated lattice is found in two A-site ordered spinel oxides, LiGaCr4O8 and LiInCr4O8. Because of the large size mismatch between Li+ and Ga3+/In3+ ions at the A site, the pyrochlore lattice, made up of Cr3+ ions…

Materials Science · Physics 2015-06-12 Yoshihiko Okamoto , Gøran J. Nilsen , J. Paul Attfield , Zenji Hiroi