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We investigate the thermal Hall effect in a Kitaev-Heisenberg system, a model for Kitaev candidate $\alpha$-RuCl$_3$, in the presence of the coupling between spin and phonon arising from chlorine atoms' vibration. We observe that the…

Strongly Correlated Electrons · Physics 2022-07-27 Shaozhi Li , Satoshi Okamoto

We present first-principles results on the magnetoelastic coupling in $\alpha$-RuCl$_3$ and uncover a striking dependence of the magnetic coupling constants on strain effects. Different magnetic interactions are found to respond very…

Strongly Correlated Electrons · Physics 2021-04-14 David A. S. Kaib , Sananda Biswas , Kira Riedl , Stephen M. Winter , Roser Valenti

Thermodynamics of the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ is studied for different directions of in-plane magnetic field using measurements of the magnetic Gr\"uneisen parameter $\Gamma_B$ and specific heat $C$. We identify two…

Strongly Correlated Electrons · Physics 2021-03-03 S. Bachus , D. A. S. Kaib , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valentí , P. Gegenwart

The Kitaev honeycomb model provides a paradigmatic example of an exactly solvable quantum spin liquid (QSL), in which the spin degrees of freedom fractionalize into itinerant Majorana fermions coupled to a static background of…

Strongly Correlated Electrons · Physics 2024-06-28 Vitor Dantas , Wen-Han Kao , Natalia B. Perkins

Magnetoelastic interaction couples spin and lattice degrees of freedom and plays a key role in thermal transport properties of magnetic insulators. In the Kitaev quantum spin liquid, the low energy excitations are charge neutral Majorana…

Strongly Correlated Electrons · Physics 2021-12-06 Haoxiang Li , A. Said , J. Q. Yan , D. M. Mandrus , H. N. Lee , S. Okamoto , Gábor B. Halász , H. Miao

We present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material $\alpha$-RuCl$_3$, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered…

Kitaev's honeycomb spin-liquid model and its proposed realization in materials such as $\alpha$-RuCl$_3$, Li$_2$IrO$_3$ and Na$_2$IrO$_3$ continue to present open questions about how the dynamics of a spin-liquid are modified in the…

Strongly Correlated Electrons · Physics 2020-02-12 R. Sarkar , Z. Mei , A. Ruiz , G. Lopez , H. -H. Klauss , J. G. Analytis , I. Kimchi , N. J. Curro

$\alpha$-RuCl$_3$ has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a…

Strongly Correlated Electrons · Physics 2025-07-15 Jiefu Cen , Hae-Young Kee

The ruthenium halide $\alpha$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $\alpha$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for…

$\alpha$-RuCl$_3$ has been proposed recently as an excellent playground for exploring Kitaev physics on a two-dimensional (2D) honeycomb lattice. However, structural clarification of the compound has not been completed, which is crucial in…

Materials Science · Physics 2016-04-27 Heung-Sik Kim , Hae-Young Kee

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction…

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

We present high-resolution thermal-expansion and specific-heat measurements of single crystalline alpha-RuCl3. An extremely hysteretic structural transition expanding over 100 K is observed by thermal- expansion along both crystallographic…

Strongly Correlated Electrons · Physics 2018-09-26 Mingquan He , Xiao Wang , Liran Wang , Frédéric Hardy , Thomas Wolf , Peter Adelmann , Thomas Brückel , Yixi Su , Christoph Meingast

In the search for experimental realizations of bond-anisotropic Kitaev interactions and resulting spin-liquid phases, the layered magnet $\alpha$-RuCl$_3$ is a prime candidate. Its modelling typically involves Heisenberg, Kitaev, and…

Strongly Correlated Electrons · Physics 2020-06-01 Lukas Janssen , Stefan Koch , Matthias Vojta

Magnetic exchange interactions are mediated via orbital overlaps across chemical bonds. Thus, modifying the bond angles by physical pressure or strain can tune the relative strength of competing interactions. Here we present a remarkable…

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

Strongly Correlated Electrons · Physics 2017-12-12 P. Lampen-Kelley , A. Banerjee , A. A. Aczel , H. B. Cao , M. B. Stone , C. A. Bridges , J. -Q. Yan , S. E. Nagler , D. Mandrus

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

We report a polarized Raman scattering study of the lattice dynamics of $\beta$-Li$_2$IrO$_3$ under hydrostatic pressures up to 7.62 GPa. At ambient pressure, $\beta$-Li$_2$IrO$_3$ exhibits the hyperhoneycomb crystal structure and a…

Quantum triangular-lattice antiferromagnets are important prototype systems to investigate phenomena of the geometrical frustration in condensed matter. Apart from highly unusual magnetic properties, they possess a rich phase diagram…

Strongly Correlated Electrons · Physics 2019-03-13 S. A. Zvyagin , D. Graf , T. Sakurai , S. Kimura , H. Nojiri , J. Wosnitza , H. Ohta , T. Ono , H. Tanaka