English

Intermediate phases in $\alpha$-RuCl$_3$ under in-plane magnetic field via interlayer spin interactions

Strongly Correlated Electrons 2025-07-15 v2

Abstract

α\alpha-RuCl3_3 has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a moderate in-plane magnetic field. The intermediate regime of the field has exotic behaviors, some of which are claimed to originate from a Kitaev spin liquid. In resolving debates surrounding these behaviors, interlayer interactions in α\alpha-RuCl3_3 have been largely overlooked due to their perceived weakness in van der Waals materials. However, near the transition, they may become significant as the field energy approaches the interlayer coupling scale. Here we investigate the effects of interlayer couplings in α\alpha-RuCl3_3 with R3ˉR\bar{3} and C2/mC2/m structures. We first examine their effects on the transition temperature (TNT_N) using classical Monte Carlo simulations. We found that the interlayer couplings have minimal effects on TNT_N, and the different TNT_N between the two structures are mainly due to the anisotropy in intralayer interactions. Focusing on the R3ˉR{\bar 3} structure, we show that the nearest neighbor interlayer interaction is the XXZ type due to the symmetry, and the next nearest neighbor interaction of the Kitaev type is crucial for the transition between two zigzag orders under an in-plane field. Furthermore, an intermediate phase with a large unit cell emerges due to the interlayer interactions. Our findings provide insights into the exotic behaviors and sample dependence reported in α\alpha-RuCl3_3.

Keywords

Cite

@article{arxiv.2504.11458,
  title  = {Intermediate phases in $\alpha$-RuCl$_3$ under in-plane magnetic field via interlayer spin interactions},
  author = {Jiefu Cen and Hae-Young Kee},
  journal= {arXiv preprint arXiv:2504.11458},
  year   = {2025}
}

Comments

13 pages, 11 figures

R2 v1 2026-06-28T22:59:32.294Z