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Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain…

Here we present a study of the phonon dynamics in the honeycomb Kitaev spin model at finite temperatures. We show that the fractionalized spin excitations of the Kitaev spin liquid, the itinerant Majorana fermions and static $Z_2$ fluxes,…

Strongly Correlated Electrons · Physics 2021-08-24 Kexin Feng , Mengxing Ye , Natalia B. Perkins

The Kitaev quantum spin liquid (QSL) on the two-dimensional honeycomb lattice epitomizes an entangled topological state, where the spins fractionalize into Majorana fermions. This state has aroused tremendous interest because it harbors…

Strongly Correlated Electrons · Physics 2022-12-12 S. Suetsugu , Y. Ukai , M. Shimomura , M. Kamimura , T. Asaba , Y. Kasahara , N. Kurita , H. Tanaka , T. Shibauchi , J. Nasu , Y. Motome , Y. Matsuda

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

The Kitaev quantum spin liquid (KSL) is a theoretically predicted state of matter whose fractionalized quasiparticles are distinct from bosonic magnons, the fundamental excitation in ordered magnets. The layered honeycomb antiferromagnet…

We present high-pressure (2 GPa) $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyper-honeycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. The spectra show evidence for a structural phase transition around 200 K…

Strongly Correlated Electrons · Physics 2025-12-16 Aimé Verrier , Vikram Nagarajan , Louis-Thomas Gendron , James G. Analytis , Jeffrey A. Quilliam

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

The layered compound $\alpha$-RuCl$_3$ is composed of a honeycomb lattice of magnetic Ru$^{3+}$ ions with the $4d^5$ electronic state. We have investigated the magnetic properties of $\alpha$-RuCl$_3$ via magnetization and specific heat…

Strongly Correlated Electrons · Physics 2015-06-24 Yumi Kubota , Hidekazu Tanaka , Toshio Ono , Yasuo Narumi , Koichi Kindo

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

We study on transport and magnetic properties of hydrated and lithium-intercalated $\alpha$-RuCl$_3$, Li$_x$RuCl$_3 \cdot y$H$_2$O, for investigating the effect on mobile-carrier doping into candidate materials for a realization of a Kitaev…

Strongly Correlated Electrons · Physics 2019-06-26 Yoshinori Imai , Katsuya Konno , Yoshinao Hasegawa , Takuya Aoyama , Kenya Ohgushi

The material $\alpha$-RuCl$_3$ has been the subject of intense scrutiny as a potential Kitaev quantum spin liquid, predicted to display Majorana fermions as low energy excitations. In practice, $\alpha$-RuCl$_3$ undergoes a transition to a…

In the Kitaev honeycomb model, spins coupled by strongly-frustrated anisotropic interactions do not order at low temperature but instead form a quantum spin liquid with spin fractionalization into Majorana fermions and static fluxes. The…

Hydrostatic pressure effects on the temperature- and magnetic field dependencies of the in-plane and out-of-plane magnetization of the bi-layered perovskite Sr3Ru2O7 have been studied by SQUID magnetometer measurements under a hydrostatic…

Materials Science · Physics 2009-11-10 Yuri V. Sushko , Bruno DeHarak , Gang Cao , G. Shaw , D. K. Powell , J. W. Brill

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

We present an analytical study of the exchange interactions between pseudospin one-half $d^{5}$ ions in honeycomb lattices with edge-shared octahedra. Various exchange channels involving Hubbard U, charge-transfer excitations, and cyclic…

Strongly Correlated Electrons · Physics 2022-06-10 Huimei Liu , Jiri Chaloupka , Giniyat Khaliullin

Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. In the quest of finding a pertinent material, $\alpha$-RuCl$_{3}$ recently emerged as…

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however,…