We report a 35Cl nuclear magnetic resonance study in the honeycomb lattice, α-RuCl3, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct evidence that α-RuCl3 exhibits a magnetic field-induced QSL. For fields larger than ∼10 T a spin-gap opens up while resonance lines remain sharp, evidencing that spins are quantum disordered and locally fluctuating. The spin gap increases linearly with increasing magnetic field, reaching ∼50 K at 15 T, and is nearly isotropic with respect to the field direction. The unusual rapid increase of the spin gap with increasing field and its isotropic nature are incompatible with conventional magnetic ordering and in particular exclude that the ground state is a fully polarized ferromagnet. The presence of such a field-induced, gapped QSL phase has indeed been predicted in the Kitaev model.
@article{arxiv.1702.01671,
title = {Evidence for a Field-induced Quantum Spin Liquid in $\alpha$-RuCl$_3$},
author = {S. -H. Baek and S. -H. Do and K. -Y. Choi and Y. S. Kwon and A. U. B. Wolter and S. Nishimoto and Jeroen van den Brink and B. Büchner},
journal= {arXiv preprint arXiv:1702.01671},
year = {2017}
}