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Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…

Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…

To meet the challenges of high-resolution molecular spectroscopy, increasingly sophisticated spectroscopic techniques were developed. For a long time FTIR and laser-based spectroscopies were used for these studies. The recent development of…

Coherent Anti-Stokes Raman Scattering (CARS) processes are ``coherent,'' but the phase of the anti-Stokes radiation is usually lost by most incoherent spectroscopic CARS measurements. We propose a novel Raman microscopy imaging method…

Optics · Physics 2009-11-10 D. L. Marks , S. A. Boppart

Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…

Optics · Physics 2025-01-20 Xiaoshuai Ma , Tianjian Lv , Xudong Zhu , Ming Yan , Heping Zeng

Infrared (IR) spectroscopy can be used as an important and effective tool for probing periodic networks of quantum wires or nanotubes (quantum crossbars, QCB) at finite frequencies far from the Luttinger liquid fixed point. Plasmon…

Strongly Correlated Electrons · Physics 2009-11-10 I. Kuzmenko , S. Gredeskul , K. Kikoin , Y. Avishai

A new method for highly selective remote sensing of atmospheric trace polar molecular gases is described. Based on infrared/terahertz double resonance spectroscopic techniques, the molecule- specific coincidence between the lines of a CO2…

Atomic Physics · Physics 2012-05-15 Dane J. Phillips , Elizabeth A. Tanner , Frank C. De Lucia , Henry O. Everitt

We demonstrate incoherent broadband cavity enhanced absorption spectroscopy in the mid-infrared wave- length range from 3000 to 3450 nm using an all-fiber based supercontinuum source. Multi-components gas detection is performed and…

Instrumentation and Detectors · Physics 2017-09-13 Caroline Amiot , Antti Aalto , Piotr Ryczkowski , Juha Toivonen , Goëry Genty

We present an overview of the Velocity Coordinate Spectrum (VCS), a new technique for studying astrophysical turbulence that utilizes the line-of-sight statistics of Doppler-broadened spectral lines. We consider the retrieval of turbulence…

Astrophysics of Galaxies · Physics 2009-02-03 D. Pogosyan , A. Lazarian

Diffuse Correlation Spectroscopy (DCS) allows the label-free investigation of microvascular dynamics deep within living tissue. However, common implementations of DCS are currently limited to measurement depths of $\sim 1-1.5cm$, which can…

Spectral imaging in the mid-infrared (MIR) range provides simultaneous morphological and chemical information of a wide variety of samples. However, current MIR technologies struggle to produce high-definition images over a broad spectral…

A novel ultra-long distributed vibration sensing (DVS) system using forward transmission and coherent detection is proposed and experimentally demonstrated. In the proposed scheme, a pair of multi-span optical fibers are deployed for…

Signal Processing · Electrical Eng. & Systems 2019-07-19 Yaxi Yan , Changjian Guo , Xiong Wu , Ziqi Lin , Xian Zhou , Faisal Nadeem Khan , Alan Pak Tao Lau , Chao Lu

Absorption spectroscopy is a fundamental tool for probing molecular structure. However, performing absorption spectroscopy on individual molecules is challenging due to the low signal-to-noise ratio. Here, we report on a nondestructive…

Broadband mid-infrared (MIR) molecular spectroscopy demands a bright and broadband light source in the molecular fingerprint region. To this end, intra-pulse difference frequency generation (IDFG) has shown excellent properties among…

We report molecular detection using dual frequency-comb spectroscopy with highly coherent broadband (6.6-11.4 {\m}m) long-wavelength infrared (LWIR) combs. The combs were produced via intra-pulse difference frequency generation (IDFG) in…

Vibrational spectroscopy is key for probing the interplay between the structure and dynamics of aqueous systems. In order to map different regions of experimental spectra to the microscopic structure of a system, it is important to combine…

Chemical Physics · Physics 2021-08-09 Sam Shepherd , Jinggang Lan , David M. Wilkins , Venkat Kapil

Frequency comb assisted diode laser spectroscopy, employing both the accuracy of an optical frequency comb and the broad wavelength tuning range of a tunable diode laser, has been widely used in many applications. In this letter we present…

Intravascular ultrasound (IVUS) is the preferred modality for capturing real-time and high resolution cross-sectional images of the coronary arteries, and evaluating the stenosis. Accurate and real-time segmentation of IVUS images involves…

Image and Video Processing · Electrical Eng. & Systems 2023-02-01 Shaofeng Yuan , Feng Yang

Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency…