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Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…

It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…

An innovative inverse scattering (IS) method is proposed for the quantitative imaging of pixel-sparse scatterers buried within a lossy half-space. On the one hand, such an approach leverages on the wide-band nature of ground penetrating…

Information Theory · Computer Science 2021-08-04 Marco Salucci , Nicola Anselmi

An emission tomography of laser-induced plasmas employed in the laser induced breakdown spectroscopy (LIBS) requires long signal integration times during which the plasma cannot be considered stationary. To reduce the integration time, it…

Plasma Physics · Physics 2010-08-04 Sergei V. Shabanov , Igor B. Gornushkin

Inverse Compton scattering (ICS) is a unique mechanism for producing fast pulses - picosecond and below - of bright X- to gamma-rays. These nominally narrow spectral bandwidth electromagnetic radiation pulses are efficiently produced in the…

We report generation of an ultrafast supercontinuum extending into the mid- infrared in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF) pumped by 1.7 $\mu$m light from an optical parametric amplifier. The simple fiber…

Thanks to intrinsically short electronic relaxation on the ps time scale, III-V semiconductor unipolar devices are ideal candidates for ultrahigh-speed operation at mid-infrared frequencies. In this work, antenna-coupled, GaAs-based multi…

Instrumentation and Detectors · Physics 2024-06-13 Quyang Lin , Michael Hakl , Sylvie Lepillet , Hua Li , Jean-Francois Lampin , Emilien Peytavit , Stefano Barbieri

Interferometric scattering microscopy has been a very promising technology for highly sensitive label-free imaging of a broad spectrum of biological nanoparticles from proteins to viruses in a high-throughput manner. Although it can reveal…

Optics · Physics 2021-08-11 Celalettin Yurdakul , Haonan Zong , Yeran Bai , Ji-Xin Cheng , M. Selim Unlu

Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…

Chemical Physics · Physics 2025-05-07 Ashay N. Patel , Madison I. Howard , Timothy C. Steimle , Nicholas R. Hutzler

We investigate the spectral shape of the total continuum radiation, between 74 MHz and 5 GHz (400 to 6 cm in wavelength), for a large sample of bright galaxies. We take advantage of the overlapping survey coverage of the VLA Low-Frequency…

Astrophysics of Galaxies · Physics 2015-06-22 Joshua Marvil , Frazer Owen , Jean Eilek

Spectroscopy of whispering-gallery mode (WGM) microresonators has become a powerful scientific tool, enabling detection of single viruses, nanoparticles, and even single molecules. Yet the demonstrated timescale of these schemes has been…

Optics · Physics 2015-06-23 Serge Rosenblum , Yulia Lovsky , Lior Arazi , Frank Vollmer , Barak Dayan

Correlated rotational alignment spectroscopy correlates observables of ultrafast gas-phase spectroscopy with high-resolution, broad-band rotational Raman spectra. This article reviews the measurement principle of CRASY, existing…

Chemical Physics · Physics 2024-03-07 Thomas Schultz

Numerous molecules exhibit unique absorption bands in the fingerprint infrared (IR) region, allowing chemical identification and detection. This makes IR spectroscopy an essential tool in biomedical diagnostics, sensing, and material…

Optics · Physics 2022-02-04 Anna V. Paterova , Zi S. D. Toa , Hongzhi Yang , Leonid A. Krivitsky

X-ray photon correlation spectroscopy (XPCS) allows for the resolution of dynamic processes within a material across a wide range of length and time scales. X-ray speckle visibility spectroscopy (XSVS) is a related method that uses a single…

Numerical Analysis · Mathematics 2023-01-09 Shaswat Mohanty , Christopher B. Cooper , Hui Wang , Mengning Liang , Wei Cai

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…

We present a technique that uses noisy broadband pulse bursts generated by modulational instability to probe nonlinear processes, including infrared-inactive Raman transitions, in molecular gases. These processes imprint correlations…

Optics · Physics 2020-12-15 Mallika Irene Suresh , Philip St. J. Russell , Francesco Tani

The absorption and emission spectrum arising from the vibrational motion of a molecule is mostly in the infrared region. These fingerprint absorptions of polar bonds enable us to acquire bond-specific chemical information from specimens.…

Optics · Physics 2024-11-15 Govind Dayal , Dheeraj Pratap

Data-driven science requires data to drive it. Being able to make accurate and precise measurement of biomaterials in the body means that medical assessments can be more accurate. There are differences between how blood absorbs and how it…

Applied Physics · Physics 2023-01-05 Daniel J. Schwab , Clifton R. Haider , Gary S. Delp , Stefan K. Grebe , Barry K. Gilbert
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