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Time-and-frequency resolved pump-probe optical spectroscopy is used to investigate the effect of the impulsive injection of delocalized excitations through a charge-transfer process in insulating CuGeO3. A large broadening of the…

A lighting-based multispectral imaging system using an RGB camera and a projector is one of the most practical and low-cost systems to acquire multispectral observations for estimating the scene's spectral reflectance information. However,…

Image and Video Processing · Electrical Eng. & Systems 2020-12-21 Hironori Hidaka , Yusuke Monno , Masatoshi Okutomi

The optoelectronic properties of nanoscale systems such as carbon nanotubes (CNTs), graphene nanoribbons and transition metal dichalcogenides (TMDCs) are determined by their dielectric function. This complex, frequency dependent function is…

Materials Science · Physics 2021-11-10 Oisín Garrity , Alvaro Rodriguez , Niclas S. Mueller , Otakar Frank , Patryk Kusch

Time-resolved optical spectroscopy represents an effective non-invasive approach to investigate the interplay of different degrees of freedom, which plays a key role in the development of novel functional materials. Here, we present…

Phase-sensitive coherent imaging exploits changes in the phases of backscattered light to observe tiny alterations of scattering structures or variations of the refractive index. But moving scatterers or a fluctuating refractive index…

The classical or quantum nature of optical spectroscopy signals is a topic that has attracted great attention recently. Spectroscopic techniques have been classified as quantum or classical depending on the light-source used in their…

Quantum Physics · Physics 2016-06-21 R. de J. León-Montiel , Zixuan Hu , Joel Yuen-Zhou

X-ray spectroscopy is one of the most powerful tools to access structure and properties of matter in different states of aggregation as it allows to trace atomic and molecular energy levels in course of various physical and chemical…

Chemical Physics · Physics 2019-06-12 Sergey I. Bokarev , Oliver Kühn

Spectroscopy is a unique experimental tool for measuring the fundamental Casimir-Polder interaction between excited state atoms, or other polarizable quantum objects, and a macroscopic surface. Spectroscopic measurements probe atoms at…

A numerical method to calculate optical conductivity based on a pump-probe setup is presented. Its validity and limits are tested and demonstrated via the concrete numerical simulations on the half-filled one-dimensional extended Hubbard…

Strongly Correlated Electrons · Physics 2016-05-26 Can Shao , Takami Tohyama , Hong-Gang Luo , Hantao Lu

We derive the two-time linear response theory for out-of-equilibrium pumped systems, generic pump-probe delays and probe frequencies. Such a theory enormously simplifies the numerical calculations, for instance, of the optical conductivity…

Optics · Physics 2024-12-10 Amir Eskandari-asl , Adolfo Avella

A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…

Chemical Physics · Physics 2009-11-13 F. Shikerman , E. Barkai

We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally-resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a nanomechanical…

A simple and novel setup for high-frequency dielectric spectroscopy of materials has been developed using a portable vector network analyzer. The measurement principle is based on radio-frequency reflectometry, and both its capabilities and…

Instrumentation and Detectors · Physics 2024-02-02 Aitor Erkoreka , Josu Martinez-Perdiguero

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental…

Deviation from perfect conical dispersion in Dirac materials, such as the presence of mass or tilting, enhances control and directionality of electronic transport. To identify these signatures, we analyze the thermal derivative spectra of…

Mesoscale and Nanoscale Physics · Physics 2024-02-22 M. A. Mojarro , R. Carrillo-Bastos , Jesús A. Maytorena

We study the intensity-intensity correlations of the radiation emitted on probe transition in a three level cascade electromagnetically induced transparency (EIT) scheme. By applying an incoherent pump, we also monitor further changes in…

Quantum Physics · Physics 2014-09-04 Shaik Ahmed , Preethi N. Wasnik , Suneel Singh , P. Anantha Lakshmi

Relaxation of electrons in a Hubbard model coupled to a dissipative bosonic bath is studied to simulate the pump-probe photoemission measurement. From this insight, we propose an experimental method of eliciting unoccupied part of the…

Strongly Correlated Electrons · Physics 2016-08-15 Youhei Yamaji , Masatoshi Imada

In pump-probe time and angle-resolved photoemission spectroscopy (TR-ARPES) experiments the presence of the pump pulse adds a new level of complexity to the photoemission process in comparison to conventional ARPES. This is evidenced by…

Using quantum theory, we study the propagation of an optical field in an inhomogeneous dielectric, and apply this scheme to traveling optical fields in a waveguide. We introduce a field-atom interaction Hamiltonian and derive the refractive…

Quantum Physics · Physics 2015-10-26 Akira Kitagawa

The real-time dynamics of interacting electrons out of equilibrium contains detailed microscopic information about electronically correlated materials, which can be read out with time-resolved optical spectroscopy. The reflectivity that is…

Strongly Correlated Electrons · Physics 2008-12-08 Martin Eckstein , Marcus Kollar