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Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

The preceding paper describes a strategy for externally influencing the course of short-time electronic excitation transfer (EET) in molecular dimers and observing the process by nonlinear wave-packet interferometry (nl-WPI). Within a…

Quantum Physics · Physics 2015-05-14 Jason D. Biggs , Jeffrey A. Cina

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

A theory of pump-probe spectroscopy is developed in which optical fields drive two-photon Raman transitions between ground states of an ensemble of three-level $\Lambda $ atoms. Effects related to the recoil the atoms undergo as a result of…

Atomic Physics · Physics 2009-11-06 C. P. Search , P. R. Berman

Superconducting circuits provide a versatile and controllable platform for studies of fundamental quantum phenomena as well as for quantum technology applications. A conventional technique to read out the state of a quantum circuit or to…

We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

X-ray energy spectrum plays an essential role in imaging and related tasks. Due to the high photon flux of clinical CT scanners, most of the spectrum estimation methods are indirect and are usually suffered from various limitations. The…

Medical Physics · Physics 2016-04-19 Wei Zhao , Qiude Zhang , Tianye Niu

Infrared pump-probe spectroscopy provides detailed information on the dynamics of hydrogen-bonded liquids. Due to dissipation of the absorbed pump pulse energy, also thermal equilibration dynamics contributes to the observed signal.…

Chemical Physics · Physics 2019-06-05 Riccardo Dettori , Michele Ceriotti , Johannes Hunger , Luciano Colombo , Davide Donadio

We report on key signal contributions in photothermal deflection spectroscopy (PDS) of semiconductors at photon energies below the bandgap energy and show how to extract the actual absorption properties from the measurement data. To this…

Materials Science · Physics 2019-07-24 Walter Dickmann , Johannes Dickmann , Florian Feilong Bruns , Stefanie Kroker

The concept of nonlinear quantum-beat pump-probe Auger spectroscopy is introduced by discussing a relatively simple four-level model system. We consider a coherent wave packet involving two low-lying states that was prepared by an…

Atomic Physics · Physics 2015-10-28 Song Bin Zhang , Nina Rohringer

Nonlinear selective reflection from the interface YAG window-high density rubidium vapor in the high-temperature cell is studied at the transition 5S$_{1/2}$-5P$_{3/2}$. In the experiment tunable pump and probe lasers are used. The…

Atomic Physics · Physics 2024-07-10 V. A. Sautenkov , S. A. Saakyan , A. A. Bobrov , B. B. Zelener

Electromagnetic interaction between a sub-wavelength particle (the `probe') and a material surface (the `sample') is studied theoretically. The interaction is shown to be governed by a series of resonances corresponding to surface polariton…

Mesoscale and Nanoscale Physics · Physics 2016-02-11 B. -Y. Jiang , L. M. Zhang , A. H. Castro Neto , D. N. Basov , M. M. Fogler

Based on the measurement of quantum correlation functions, the quantum statistical properties of spectral measurements are studied for broadband radiation fields. The spectral filtering of light before its detection is compared with the…

Quantum Physics · Physics 2015-01-15 P. Grünwald , D. Vasylyev , J. Häggblad , W. Vogel

While time-resolved pump-probe differential reflectivity and transmitivity measurements are routinely used to monitor the population relaxation dynamics on the subpicosecond time scale, it is also known that the signal in the negative delay…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Richarj Mondal , Basabendra Roy , Bipul Pal , Bhavtosh Bansal

This paper describes the impedance spectroscopy adapted for analysis of small electrochemical changes in fluids. To increase accuracy of measurements the differential approach with temperature stabilization of fluid samples and electronics…

Instrumentation and Detectors · Physics 2016-07-26 S. Kernbach , I. Kuksin , O. Kernbach

Several devices for substrate texture detection based on diffractive optics, for paper, textiles and non-wovens have been proposed in the past for direct inspection during the production processes. In spite of the presence of devices…

Popular Physics · Physics 2008-01-21 Amelia Sparavigna , Rory A. Wolf

The optical conductivity of freely suspended graphene was examined under non-equilibrium conditions using femtosecond pump-probe spectroscopy. We observed a conductivity transient that varied strongly with the electronic temperature,…

Mesoscale and Nanoscale Physics · Physics 2013-06-20 Leandro M. Malard , Kin Fai Mak , A. H. Castro Neto , N. M. R. Peres , Tony F. Heinz

Reflectometry is a technique that uses the light reflected by a sample to determine properties of the sample. Interferometric reflectometry uses interference between two beams, one of which is incident on ---and reflected back by--- a…

Optics · Physics 2019-10-10 Alexander Nahmad-Rohen , Wolfgang Langbein

A method is presented for modelling the optical properties of a photonic crystal structure mounted on a substrate which is thick enough that the light reflected from the back is incoherent with reflections from the front. Transmission and…

Optics · Physics 2010-12-17 D. M. Whittaker , G. A. Gehring
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