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"Single-shot" ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics using chirped probe pulses is analyzed theoretically. FDSS has an advantage over pump-probe spectroscopy in a situation where the "noise"…

Optics · Physics 2007-05-23 Ilya A. Shkrob , Stanislas Pommeret

Attosecond science has been transforming our understanding of electron dynamics in atoms, molecules and solids. However, to date almost all of the attoscience experiments have been based on spectroscopic measurements because attosecond…

We present ultra-fast quantum chemical methods for the calculation of infrared and ultraviolet-visible spectra designed to provide fingerprint information during autonomous and interactive explorations of molecular structures.…

Chemical Physics · Physics 2022-08-30 Francesco Bosia , Thomas Weymuth , Markus Reiher

Materials combining both a high refractive index and a wide band gap are of great interest for optoelectronic and sensor applications. However, these two properties are typically described by an inverse correlation with high refractive…

The ability to manipulate and measure the time-frequency structure of quantum light is useful for information processing and metrology. Measuring this structure is also important when developing quantum light sources with high modal purity…

Quantum Physics · Physics 2022-01-12 G. S. Thekkadath , B. A. Bell , R. B. Patel , M. S. Kim , I. A. Walmsley

A novel approach for measuring fast oscillations of an absolute value of interferometer optical path difference (OPD) has been developed. The principles of frequency-scanning interferometry are utilized for registration of the…

Instrumentation and Detectors · Physics 2019-05-01 Nikolai Ushakov , Leonid Liokumovich

To design semiconductor-based optical devices, the optical properties of the used semiconductor materials must be precisely measured over a large band. Transmission spectroscopy stands out as an inexpensive and widely available method for…

This paper presents a simple and effective wideband method for the determination of material properties, such as the complex index of refraction and the complex permittivity and permeability. The method is explicit (non-iterative) and…

Instrumentation and Detectors · Physics 2010-12-02 Khattiya Chalapat , Kari Sarvala , Jian Li , G. S. Paraoanu

Transient field-resolved spectroscopy enables studies of ultrafast dynamics in molecules, nanostructures, or solids with sub-cycle resolution, but previous work has so far concentrated on extracting the dielectric response at frequencies…

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

Optical spectrum analysis is the cornerstone of spectroscopic sensing, optical network performance monitoring, and hyperspectral imaging. While conventional high-performance spectrometers used to perform such analysis are often large…

Applied Physics · Physics 2018-03-19 Derek M. Kita , Brando Miranda , David Favela , David Bono , Jerome Michon , Hongtao Lin , Tian Gu , Juejun Hu

The spectrogram is a classical DSP tool used to view signals in both time and frequency. Unfortunately, the Heisenberg Uncertainty Principal limits our ability to use them for detecting and measuring narrowband signal modulation in wideband…

Information Theory · Computer Science 2014-01-22 Ray Maleh , Frank A. Boyle

The spectral properties of a multilevel atomic system interacting with multiple electromagnetic fields, a modified inverted-Y system, have been theoretically investigated. In this study, a numerical matrix propagation method has been…

Atomic Physics · Physics 2019-05-22 Charu Mishra , A. Chakraborty , S. R. Mishra

The spectrophotometric characterization of high efficiency, optically-active samples such as light-emitting organic bulks and thin films can be problematic because their broad-band luminescence is detected together with the monochromatic…

Instrumentation and Detectors · Physics 2012-03-20 R. M. Montereali , M. A. Vincenti , E. Nichelatti , F. Di Pompeo , E. Segreto , N. Canci , F. Cavanna

The characteristics of an x-ray spectrum can greatly influence imaging and related tasks. In practice, due to the pile-up effect of the detector, it's difficult to directly measure the spectrum of a CT scanner using an energy resolved…

Medical Physics · Physics 2015-03-09 Wei Zhao , Kai Niu , Sebastian Schafer , Kevin Royalty

The redistribution of electrons in an ultrafast pump-probe experiment causes significant changes to the effective interaction between electrons and bosonic modes. We study the influence of these changes on pump-probe photoemission…

Mesoscale and Nanoscale Physics · Physics 2014-08-25 A. F. Kemper , M. A. Sentef , B. Moritz , J. K. Freericks , T. P. Devereaux

Many important phenomena in quantum devices are dynamic, meaning that they cannot be studied using time-averaged measurements alone. Experiments that measure such transient effects are collectively known as fast readout. One of the most…

We present measurements of the hyperfine coefficients and isotope shifts of the Dy I $683.731 $nm transition, using saturated absorption spectroscopy on an atomic beam. A King Plot is drawn resulting in an updated value for the specific…

Atomic Physics · Physics 2014-02-27 M. Schmitt , E. A. L. Henn , J. Billy , H. Kadau , T. Maier , A. Griesmaier , T. Pfau

The problem of calculation of the reflectivity of non-ideal shock-compressed plasmas is revisited. The dielectric formalism based on the method of moments incorporating exact asymptotic forms and sum rules is applied to the new experimental…

Plasma Physics · Physics 2007-05-23 D. Ballester , A. M. Fuentes , I. M. Tkachenko

Complex field imaging, which captures both the amplitude and phase information of input optical fields or objects, can offer rich structural insights into samples, such as their absorption and refractive index distributions. However,…

Optics · Physics 2024-05-30 Jingxi Li , Yuhang Li , Tianyi Gan , Che-Yung Shen , Mona Jarrahi , Aydogan Ozcan