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We study the all-optical switching behavior of one-dimensional metal-dielectric photonic crystals due to the nonlinearity of the free metal electrons. A polychromatic pump-probe setup is used to determine the wavelength and pump intensity…

Other Condensed Matter · Physics 2015-05-13 Tolga Ergin , Tilman Höner zu Siederdissen , Harald Giessen , Markus Lippitz

In pump-probe spectroscopy, one often needs to analyse the transmission or reflection of electromagnetic waves through optically pumped media. Here, it is common practice to approximate the analysis in order to extract non-equilibrium…

Optics · Physics 2019-02-26 Peter Karlsen , Euan Hendry

Transient absorption microscopy measures excited-state kinetics based on the imaginary part of the pump-induced perturbation to the complex refractive index, i.e. $\Im \{\Delta\mathcal N\}$, with applications in both materials and…

Optics · Physics 2026-03-17 Cameron N. Coleal , Randy A. Bartels , Jesse W. Wilson

A major limitation of transient optical spectroscopy is that relatively high laser fluences are required to enable broadband, multichannel detection with acceptable signal-to-noise levels. Under typical experimental conditions, many…

Optics · Physics 2023-05-03 Siedah J. Hall , Peter J. Budden , Anne Zats , Matthew Y. Sfeir

As a label-free imaging technique, quantitative phase imaging (QPI) provides optical path length information of transparent specimens for various applications in biology, materials science, and engineering. Multispectral QPI measures…

Optics · Physics 2023-08-29 Che-Yung Shen , Jingxi Li , Deniz Mengu , Aydogan Ozcan

Ultrafast pump-probe spectroscopy is a powerful tool to study the nonequilibrium dynamics in high-Tc cuprate superconductors. The photo-induced quasiparticle (QP) dynamics revealed by pump-probe spectroscopy are sensitive to the near-Fermi…

Superconductivity · Physics 2015-06-22 Wei Li , Chunfeng Zhang , Xiaoyong Wang , Jak Chakhalian , Min Xiao

Dielectric spectroscopy is one of the most commonly used techniques for the investigation of the dynamic response of glass-forming materials. The tremendous slow-down of the particle motions when approaching the glass transition and…

Disordered Systems and Neural Networks · Physics 2007-05-23 U. Schneider , P. Lunkenheimer , A. Pimenov , R. Brand , A. Loidl

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…

Quantum Physics · Physics 2020-11-03 Haowei Shi , Zheshen Zhang , Stefano Pirandola , Quntao Zhuang

We report on cw measurements of probe beam absorption and four-wave-mixing spectra in a $^{85}$Rb magneto-optical trap taken while the trap is in operation. The trapping beams are used as pump light. We concentrate on the central feature of…

A novel technique for measuring plasma conditions using monochromatic pump-broadband probe laser interactions has been experimentally demonstrated. Originally proposed in [J. Ludwig et al., Phys. Plasmas \textbf{26}, 113108 (2019)], this…

We use frequency entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive index sensing of a…

Quantum Physics · Physics 2014-03-27 Dmitry A. Kalashnikov , Zhenying Pan , Arseniy I. Kuznetsov , Leonid A. Krivitsky

Ultrafast dynamical processes in photoexcited molecules can be observed with pump-probe measurements, in which information about the dynamics is obtained from the transient signal associated with the excited state. Background signals…

Atomic Physics · Physics 2018-06-11 M. Rumetshofer , P. Heim , B. Thaler , W. E. Ernst , M. Koch , W. von der Linden

Selective reflection is a high-resolution spectroscopic method that allows the probing of atomic and molecular gases in the near field of dielectric cell windows. It is a sensitive technique for measuring interactions between excited atoms…

Quantum Physics · Physics 2025-07-09 B. Dutta , C. Boldt , G. Garcia-Arellano , M. Ducloy , P. Pedri , S. Scheel , A. Laliotis

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

We present a method for recovery of narrow homogeneous spectral features out of broad inhomogeneous overlapped profile based on second-derivative processing of the absorption spectra of alkali metal atomic vapor nanocells. The method is…

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…

Quantum Physics · Physics 2015-06-22 Allan S. Johnson , Joel Yuen-Zhou , Alán Aspuru-Guzik , Jacob J. Krich

Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however,…

Optics · Physics 2019-05-01 Ondřej Denk , Kaibo Zheng , Donatas Zigmantas , Karel Žídek

We analyze theoretically and experimentally how nonlinear differential-transmission spectroscopy of a lambda-system medium can provide quantitative understanding of the optical dipole moments and transition energies. We focus on the…

Materials Science · Physics 2015-01-07 J. P. de Jong , A. R. Onur , D. Reuter , A. D. Wieck , C. H. van der Wal

Optical images of transparent three-dimensional objects can be different from a replica of the object's cross section in the image plane due to refraction at the surface or in the body of the object. Simulations of the object's image are…