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The emerging field of complex oxide interfaces is generically built on one of the most celebrated substrates - strontium titanate (SrTiO3). This material hosts a range of phenomena, including ferroelasticity, incipient ferroelectricity, and…

Mesoscale and Nanoscale Physics · Physics 2013-12-13 Maayan Honig , Joseph A. Sulpizio , Jonathan Drori , Arjun Joshua , Eli Zeldov , Shahal Ilani

We present a comprehensive first-principles study of the electronic charge redistribution in atomically sharp LaAlO$_3$/SrTiO$_3$(001) heterointerfaces of both n- and p-types allowing for non-stoichiometric composition. Using two different…

Materials Science · Physics 2012-11-13 Alexandre Sorokine , Dmitry Bocharov , Sergei Piskunov , Vyacheslavs Kashcheyevs

The oxide interface between LaAlO3 and KTaO3(111) can host an electron gas that condenses into superconductivity at low temperatures. In this work, we demonstrate a local and non-volatile control of this electron gas using a biased…

Superconductivity · Physics 2022-08-25 Siyuan Hong , Yanqiu Sun , Yuan Liu , Yishuai Wang , Yanwu Xie

Atomically sharp oxide heterostructures exhibit a range of novel physical phenomena that do not occur in the parent bulk compounds. The most prominent example is the appearance of highly conducting and superconducting states at the…

Intriguingly conducting perovskite interfaces between ordinary band insulators are widely explored, whereas similar interfaces with Mott insulators are still not quite understood. Here we address the (001), (110), and (111) interfaces…

The interface superconductivity in LaAlO$_{3}$-SrTiO$_{3}$ heterostructures reveals a non-monotonic behavior of the critical temperature as a function of the two-dimensional density of charge carriers. We develop a theoretical description…

Superconductivity · Physics 2014-07-22 S. N. Klimin , J. Tempere , J. T. Devreese , D. van der Marel

The properties of single-crystal SrTiO$_{3}$ substrates and homoepitaxial SrTiO$_{3}$ films grown by pulsed laser deposition have been compared, in order to understand the loss of interfacial conductivity when more than a critical thickness…

We present calculations of the charge density profile, subband occupancy and ellipsometry spectra of the electron gas at the LaAlO3/SrTiO3 interface. The calculations employ self-consistent Hartree and random phase approximations, a tight…

Strongly Correlated Electrons · Physics 2015-06-15 Se Young Park , Andrew J. Millis

We present an x-ray absorption study of the dependence of the V oxidation state on the thickness of LaVO$_3$ (LVO) and capping LaAlO$_3$ (LAO) layers in the multilayer structure of LVO sandwiched between LAO. We found that the change of the…

Strongly Correlated Electrons · Physics 2009-07-15 H. Wadati , D. G. Hawthorn , J. Geck , T. Z. Regier , R. I. R. Blyth , T. Higuchi , Y. Hotta , Y. Hikita , H. Y. Hwang , G. A. Sawatzky

We investigate the electronic properties of the LaAlO3/SrTiO3 interface using density functional theory. In contrast to previous studies, which relied on (semi-)local functionals and the GGA+U method, we here use a recently developed hybrid…

Strongly Correlated Electrons · Physics 2013-07-18 F. Cossu , U. Schwingenschlögl , V. Eyert

The electronic properties of the polar interface between insulating oxides is a subject of great current interest. An exciting new development is the observation of robust magnetism at the interface of two non-magnetic materials LaAlO_3…

Strongly Correlated Electrons · Physics 2013-10-03 Sumilan Banerjee , Onur Erten , Mohit Randeria

In this paper we use density functional theory combined with dynamical mean-field theory (DFT+DMFT) to study interface effects between thin films of the correlated metal CaVO$_3$ and the two typical substrate materials SrTiO$_3$ and…

Strongly Correlated Electrons · Physics 2021-01-04 Sophie Beck , Claude Ederer

We used x-ray photoemission spectroscopy to investigate the electronic structure of the Mott insulator LaVO3 embedded in LaAlO3. By limiting the upper layer of LaAlO3 to 3 unit cells, the underlying LaVO3 could be probed. The V 2p…

Materials Science · Physics 2015-06-25 Y. Hotta , H. Wadati , A. Fujimori , T. Susaki , H. Y. Hwang

Oxide interfaces provide an opportunity for electronics. However, patterning of electron gases at complex oxide interfaces is challenging. In particular, patterning of complex oxides while preserving a high electron mobility remains…

We investigate the role of lattice polarization in determination of induced carrier density at the $n$-type interface of LaAlO$_3$ overlayer on SrTiO$_3$ (001) by carrying out density-functional-theory calculations. When no oxygen vacancy…

Materials Science · Physics 2015-05-13 Yun Li , Jaejun Yu

We report the formation of a non-magnetic band insulator at the isopolar interface between the antiferromagnetic Mott-Hubbard insulator LaTiO3 and the antiferromagnetic charge transfer insulator LaFeO3. By density functional theory…

Strongly Correlated Electrons · Physics 2014-12-10 J. E. Kleibeuker , Z. Zhong , H. Nishikawa , J. Gabel , A. Müller , F. Pfaff , M. Sing , K. Held , R. Claessen , G. Koster , G. Rijnders

We investigate the structural, electronic, transport, and thermoelectric properties of LaNiO$_3$/SrTiO$_3(001)$ superlattices containing either exclusively $n$- or $p$-type interfaces or coupled interfaces of opposite polarity by using…

Materials Science · Physics 2017-03-03 Benjamin Geisler , Ariadna Blanca-Romero , Rossitza Pentcheva

The realization of ambient-pressure superconductivity in La$_3$Ni$_2$O$_7$ thin films raises a fundamental question: is the metallic ground state driven by lattice strain or interfacial charge reconstruction? Using fully self-consistent…

Superconductivity · Physics 2025-12-22 Guanlin Li , Cui-Qun Chen , Haoliang Shi , Zhengtao Liu , Hao Ma , Fubo Tian , Dao-Xin Yao , Defang Duan

Dimensionality control in the LaNiO3 (LNO) heterostructure has attracted attention due to its two-dimensional (2D) electronic structure was predicted to have an orbital ordered insulating ground state, analogous to that of the parent…

The recent observation of superconductivity at the interfaces between KTaO3 and EuO (or LaAlO3) offers a new example of emergent phenomena at oxide interfaces. This superconductivity exhibits an unusual strong dependence on the crystalline…

Superconductivity · Physics 2022-08-25 Tianshuang Ren , Miaocong Li , Xikang Sun , Lele Ju , Yuan Liu , Siyuan Hong , Yanqiu Sun , Qian Tao , Yi Zhou , Zhu-An Xu , Yanwu Xie